Cited by 963High Entropy Alloys StudiesElectrocatalysts for Energy ConversionMachine Learning in Materials Science

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High-entropy energy materials: challenges and new opportunities

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Ma, Yanjiao, Ma, Yuan, Wang, Qingsong, Schweidler, Simon, Botros, Miriam, Fu, Tongtong, Hahn, Horst, Brezesinski, Torsten, Breitung, Ben·2021·Energy & Environmental Science

DOI 10.1039/d1ee00505g

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Abstract

An overview of high-entropy materials for energy applications, including H 2 catalysis and storage, CO 2 conversion, O 2 catalysis and electrochemical energy storage, is given and the challenges and opportunities within this field are discussed.

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Wu, Q., Alkemper, A., Lauterbach, S., Hofmann, J., & Einert, M. (2024) · Energy Advances · doi:10.1039/d4ya00026a · Cited by 14
“1,2 The principal concept of entropy-stabilized alloys was expanded to multicationic oxide systems in 2015.”
Self-adhesive high-entropy oxide sub-nanowire monolithic electrocatalysts
Huang, Y., Wang, Z., Chen, X., Gu, L., Xiao, H. Y., Liu, Q., & Wang, X. (2026) · Nature Nanotechnology · doi:10.1038/s41565-026-02175-4 · Cited by 18
“…), where Δ G is the Gibbs free energy, Δ H mix is the enthalpy of mixing, T is the absolute temperature, Δ S configuration is the configurational entropy and Δ S surface is the surface entropy, which enables low-temperature synthesis with precise control over composition and morphology 17,18,32 .”
Influential
High-entropy alloys as advanced electrocatalysts: Structural engineering and performance optimization for sustainable energy conversion
Zhu, A., Pan, Y., Chang, Z., Cao, X., & Gao, J. (2025) · Chemical Engineering Journal · doi:10.1016/j.cej.2025.171157 · Cited by 15
High-entropy hexacyanoferrates as robust cathode active materials for sodium storage
Ma, Y., Brezesinski, T., Breitung, B., & Ma, Y.-J. (2023) · Matter · doi:10.1016/j.matt.2023.01.008 · Cited by 13
Self-citation
Emerging Pd-based electrocatalysts and supports for ethanol oxidation reaction: High-entropy and single-atom materials
Fakude, C. T., Haruna, A. B., & Ozoemena, K. I. (2024) · Inorganica Chimica Acta · doi:10.1016/j.ica.2024.122377 · Cited by 14
High-entropy alloy electrocatalysts for water splitting: A systematic review with perspectives on machine learning and future design strategies
Naz, S., Saeed, A., Khoja, A. H., Younis, H., Azeem, H., Naeem, N., Anwar, M., & Baig, M. M. (2025) · Fuel · doi:10.1016/j.fuel.2025.137920 · Cited by 13
Amorphous scaly high-entropy borides with electron traps for efficient catalysis in solid-state hydrogen storage
Wang, L., Wu, F., Chen, D., Bian, T., Senin, P. V., & Zhang, L. (2025) · International Journal of Minerals Metallurgy and Materials · doi:10.1007/s12613-024-3033-2 · Cited by 9
High-Entropy Ceramics: From Disorder to Emerging Functionalities
Hingangavkar, G. M. (2025) · Ceramics International · doi:10.1016/j.ceramint.2025.10.444 · Cited by 12
Investigation into the design and application of alloy anodes for lithium-ion batteries
Han, T., Sun, Q., He, P., Han, D., Xin, Y., Li, G., Yu, W., Zhao, Y., Yang, P., & Liu, Z. (2025) · Chemical Engineering Journal · doi:10.1016/j.cej.2025.169018 · Cited by 14
High-entropy lead-free perovskite nanoparticles as efficient photocatalysis with a wide visible-light absorption band
An, X., Guo, X., Zhu, S., Fan, B., Zhu, J., Shao, G., Xu, H., Wang, H., & Lu, H. (2025) · Journal of Alloys and Compounds · doi:10.1016/j.jallcom.2025.181680 · Cited by 13
Synthesis and characterization of (Fe0.2Ni0.2Co0.2Al0.2Zn0.2)3O4 high entropy oxide as electrocatalyst for oxygen evolution reaction
Vasconcelos, G. S., Raimundo, R., Lima, M. J., Galvão, K. F., da Silva, M. D., Macedo, D. A., Karimi, M., Huaman, R. C., Gastelois, P., Gomes, U. U., et al. (2025) · Journal of Alloys and Compounds · doi:10.1016/j.jallcom.2025.179776 · Cited by 12
Electrochemical energy storage and rectification performance of high-entropy oxide (CrMnFeCoNi)3O4
Chen, B., Zhang, W.-B., Yin, Y., Feng, J., Yang, F., Yang, K., Liu, X.-Y., Ma, X., & Peng, Y. (2025) · Journal of Energy Storage · doi:10.1016/j.est.2024.115228 · Cited by 12
Effects of irradiation damage on the hardness and elastic properties of quaternary and high entropy transition metal diborides
Khanolkar, A., Datye, A., Zhang, Y., Dennett, C., Guo, W., Liu, Y., Weber, W., Lin, H.-T., & Zhang, Y.-W. (2024) · Journal of Applied Physics · doi:10.1063/5.0206224 · Cited by 12
Role of Oxygen Vacancy in High-entropy Cu1Zn1Al0.5Ce5Zr0.5Ox for CO2 Hydrogenation Reaction
Li, J.-T., Yuan, X., Tian, F.-P., Wang, M., Hu, T., Xiong, G., & Wang, X. (2024) · Applied Catalysis A : General · doi:10.1016/j.apcata.2024.119781 · Cited by 12
Hydrogen technologies and policies for sustainable future: a review
Agbadaola, O., Qadir, D., Ahmad, F., Suleman, H., Karousos, D. S., & Favvas, E. (2024) · Chemické zvesti · doi:10.1007/s11696-024-03403-8 · Cited by 12
“…in underdevel-oped nations (iii) Growing population of the world (iv) Environmental issues around the world Effective expansion of HE will have significant positive effects on the economy, energy security, environment, and final consumer (Ishfaq et al. 2022; Ma et al. 2021; Abe et al. 2019).”
Low-temperature synthesized amorphous quasi-high-entropy carbonate electrocatalyst with superior surface self-optimization for efficient water oxidation
Lü, C., Li, M., Zhang, X., Hou, H., Li, X., Yang, X., Liu, X., Ding, Y., Hou, J., & Wang, Y. (2022) · Ceramics International · doi:10.1016/j.ceramint.2022.12.067 · Cited by 13
Constructing Multilevel Structure with Microdomains of Oxides on Three-Dimensional High-Entropy Alloy Support Toward Efficient Oxygen Evolution
Zhang, S., Guo, J., Li, T.-T., Sun, J.-F., Meng, Y.-Q., Kang, J.-L., Tan, L., & Zhang, Z.-J. (2022) · Social Science Research Network · doi:10.2139/ssrn.4181327 · Cited by 12
Noble-metal-free high-entropy spinel oxides as an efficient and long-lasting bifunctional electrocatalyst for seawater electrolysis under industrial conditions
Balasubramanian, P., Shen, R., He, S., Han, S.-T., & Zhang, M. (2025) · Journal of Power Sources · doi:10.1016/j.jpowsour.2025.238329 · Cited by 11
Dynamic atomic-scale electron avalanche breakdown in solid dielectrics
Wang, J., Shen, Z.-H., Li, W., Liu, R., Duan, Y.-L., Shen, Y., Liu, H.-X., & Nan, C.-W. (2025) · Nature Communications · doi:10.1038/s41467-025-61866-z · Cited by 11
“Recently, high-entropy strategy has been recognized as a feasible and effective method to easily modulate the local atomic heterogeneity to realize near-ideal lattice distortion 4,19,47 – 49 .”
Yolk-Shell-Structured (CrMnFeCoNi)3O4 High-Entropy Oxide Anode for High-Performance Lithium-Ion Batteries
Patra, J., Nguyen, T., Panda, A., Hsieh, C.-T., Wang, F.-M., Wu, T.-Y., Yang, C.-C., Bresser, D., Ting, J., & Chang, J.-K. (2025) · Electrochimica Acta · doi:10.1016/j.electacta.2025.146545 · Cited by 11
High entropy oxides as a rising star in pollutant disposal and resource recycling: Emerging advancements and future challenges
Hua, Y.-K., Su, G.-J., Li, Q., Pang, J., Sun, B.-H., Zhang, Y., Chen, X., Shi, B., & Meng, J. (2024) · Critical reviews in environmental science and technology · doi:10.1080/10643389.2024.2379028 · Cited by 11
“…with diverse structures have been reported, such as rock-salt, fluorite, spinel and perovskite type HEO (R-HEO, F-HEO, S-HEO and P-HEO) (Figure 1d) (Ma et al., 2021), mainly falling into the following two categories: The first type is R-HEO (AB) and F-HEO (AB 2 ) with a single cationic Wyckoff…”
Fabrication of porous high-entropy Mn-Fe-Co-Ni-Cu-Zn alloys by vapor phase dealloying
Yakovenko, O. М., Sokol’skii, V. È., Švec, P., Janotová, I., Švec, P., Kulik, T., Cieślak, G., & Roik, O. S. (2024) · Journal of Alloys and Compounds · doi:10.1016/j.jallcom.2024.175312 · Cited by 22
Powder metallurgical process to enhance the critical current density and critical magnetic field in high entropy alloy superconductors
Hidayati, R., Kim, J. H., Kim, G., Yun, J. H., & Rhyee, J. (2024) · Current Applied Physics · doi:10.1016/j.cap.2023.10.019 · Cited by 13
Local cation ordering in compositionally complex Ruddlesden–Popper n = 1 oxides
Jiang, B., Pitike, K., Lin, D., Purdy, S., Wang, X., Zhao, Y.-F., Zhang, Y.-P., Metz, P., Macias, A., Meyer, H. M., et al. (2023) · APL Materials · doi:10.1063/5.0144766 · Cited by 11
Deuterium induced defects and embrittlement behavior of a Co-free high entropy alloy
An, X., Zhang, D., Zhang, H., Wang, Q.-Q., Zhu, T., Wu, Z., Zhang, W., Deng, H., Hu, W.-Y., Cao, X.-Z., et al. (2023) · Journal of Alloys and Compounds · doi:10.1016/j.jallcom.2023.168800 · Cited by 11
Self-citation
Preparation of graphene-coated high entropy alloy nanoparticles by double pulse carbothermal shock
Wang, G.-J., Li, L., Zhang, S., Zhu, L., Zhang, Y., Huang, Z.-F., Cao, Z.-H., & Meng, X. (2023) · Scripta Materialia · doi:10.1016/j.scriptamat.2023.115668 · Cited by 11
High-entropy oxides anode: Exploring the high-performance application from composition design to modification strategy in lithium ion battery
Yao, J., Wang, D., Liu, S.-M., Zhang, J.-L., Ding, W.-Y., & Dong, C. (2026) · Journal of Energy Storage · doi:10.1016/j.est.2025.120192 · Cited by 10
Ultrasmall high-entropy alloy-nanolabels based immunochromatographic test strip for rapid, ultrasensitive, and catalytic detection of Staphylococcus aureus
Huang, W., Ren, Z. X., Li, X., Chen, R., Fan, D., Da, J., Zha, Y., & Yongjie, X. (2025) · Microchimica Acta · doi:10.1007/s00604-025-07213-x · Cited by 10
“As a result, HEAs are considered strong candidates for applications in energy systems [30–32], therapeutics [33], and various other fields [34].”
Electrolyte Formulation with Improved Ion Desolvation and Diffusion Kinetics, and Superior Anti-Corrosion Properties for Ultrawide-Temperature Supercapacitors (–70∼100°C)
Qi, Y.-H., Bao, C., Qiu, J., Hu, Z., Lu, S., Yan, J.-H., Cen, K.-F., Bo, Z., & Yang, H.-C. (2024) · Energy Storage Materials · doi:10.1016/j.ensm.2024.103782 · Cited by 10
Porous high-entropy spinel oxides templated by in situ generated polypyrrole microspheres toward enhanced peroxymonosulfate activation
Zhang, L., Song, S., Han, X., & Du, Y. (2024) · Separation and Purification Technology · doi:10.1016/j.seppur.2024.129083 · Cited by 6
New-Generation Materials for Hydrogen Storage in Medium-Entropy Alloys
Varcholová, D., Kušnírová, K., Oroszová, L., Möllmer, J., Lange, M., Gáborová, K., Buľko, B., Demeter, P., & Saksl, K. (2024) · Materials · doi:10.3390/ma17122897 · Cited by 10
“This growing interest stems from their remarkable characteristics, including their impressive mechanical properties [13,14], strong corrosion resistance [15,16], and notable structural stability [17].”
BackgroundInfluential
Rigid structural battery: Progress and outlook
Chen, X.-H., Xiang, Y., Wu, J., Wu, F., Mei, S., Ye, X., Pan, H., Xiang, Y., Liu, X.-C., Li, F., et al. (2024) · Journal of Energy Storage · doi:10.1016/j.est.2024.112070 · Cited by 10
Anomalies in the short-range local environment and atomic diffusion in single crystalline equiatomic CrMnFeCoNi high-entropy alloy
Smekhova, A., Gaertner, D., Kuzmin, A., Buzanich, A. G., Schuck, G., Žižak, I., Wilde, G., Yusenko, K. V., & Divinski, S. V. (2024) · Nano Research · doi:10.1007/s12274-024-6443-6 · Cited by 10
Advanced high entropy LDHs electrocatalysts: Synthesis and performance enhancement strategies for alkaline oxygen evolution reaction
Yin, S., Fu, S., Wang, Y., Zhao, R., & Liu, L. (2025) · Sustainable materials and technologies · doi:10.1016/j.susmat.2025.e01829 · Cited by 5
One-step, binder-free and rapid synthesis of high-entropy oxide anode materials for the lithium-ion batteries
Lin, Y., Chen, S., Ma, Y.-Z., Wang, S., Ma, Z., Sun, L., Cao, R., Song, G., Yu, Z., Yao, J.-H., et al. (2025) · Next Materials · doi:10.1016/j.nxmate.2025.100855 · Cited by 9
Self-citation
Progress in the fabrication and catalytic utilization of high entropy alloys particles
Xiao, M., Sun, H., & Hong, Z. (2025) · International Journal of Hydrogen Energy · doi:10.1016/j.ijhydene.2025.06.200 · Cited by 10
High-entropy argyrodite glass–ceramic electrolytes for all-solid-state batteries
Lin, J., Schaller, M., Zhang, R.-Z., Baran, V., Liu, H., Ding, Z., Indris, S., Kondrakov, A., Brezesinski, T., & Strauss, F. (2025) · Materials Futures · doi:10.1088/2752-5724/adde76 · Cited by 9
“This threshold criterion is met when at least five different elements occupy a single crystallographic site at equimolar ratios [31, 32].”
Self-citation
Multifunctional high entropy metal/metal oxide hybrid nanostructures-embedded carbon nanofiber composites for electrochemical energy storage
Kim, D.-Y., Song, J.-W., Kim, Y. A., Kim, M. H., & Kim, B.-H. (2025) · Carbon · doi:10.1016/j.carbon.2025.120414 · Cited by 9
Tuning the oxygen vacancy concentration in n-type TiO2 group oxides through Nb5+/Ga3+ for high-dielectric La2(TiZrSnHfGe)2O7 high-entropy oxides
Zhou, Z.-X., Ma, K., Li, S., Dong, L., Li, P., Li, J., & Qi, X. (2025) · Rare Metals · doi:10.1007/s12598-025-03356-1 · Cited by 9
“The diversity of materials design, provided by the entropy-mediated phase-stabilization concept, allows engineering of new oxide candidates for practical applications, warranting further studies in this emerging ﬁeld of materials science [32–36].”
Dual-doped medium-entropy phosphides for complete urea electrolysis.
Sheng, W., Zhou, X., Ajmal, S., Chen, X., Ma, Y.-H., Chen, P., Zhu, M.-Z., & Li, P. (2024) · Journal of Colloid and Interface Science · doi:10.1016/j.jcis.2024.09.142 · Cited by 9
Self-citation
Studies on supercapacitor electrode performance of novel (AlCuCoFeMnNi)3O4 high entropy spinel oxide admixed with different carbon‐based additives
Gupta, A. K., Kumar, A., Marndi, M., Giri, N. K., & Shahi, R. R. (2024) · Energy Storage · doi:10.1002/est2.70002 · Cited by 9
“17 High entropy oxide (HEO) possesses diverse metal cations within the crystal structure, and their interaction results in intriguing functional properties.”
Elevating energy storage: High-entropy materials take center stage
Mishra, M., & Kumar, M. (2024) · Journal of Energy Storage · doi:10.1016/j.est.2024.112186 · Cited by 9
Recent advances and understanding of high-entropy materials for lithium-ion batteries
Feng, S., & Liu, H. (2024) · Nanotechnology · doi:10.1088/1361-6528/ad40b4 · Cited by 9
“S conf achieves its maximum [ 26 ] : As a result, Δ S mix solely relates to the number of elements in HEAs, thus increasing the Δ S mix with the increase of the number of elements.”
High entropy oxides: New superior supports for single atom catalysts
Tukur, P., Tukur, F., Mo, Y., Yan, Q., Dun, C., & Wei, J.-J. (2024) · Next Materials · doi:10.1016/j.nxmate.2024.100192 · Cited by 9
Varying interfacial reaction patterns in (VNbTaMoW)C ceramic joints brazed with Ti-Zr-Ni-Cu filler alloy
Niu, S.-Y., Yang, Z.-W., Mu, R.-J., Sun, K.-B., & Wang, Y. (2024) · Journal of the European Ceramic Society · doi:10.1016/j.jeurceramsoc.2024.03.023 · Cited by 9
Development and Research of New Hybrid Composites in Order to Increase Reliability and Durability of Structural Elements
Rusinov, P., Blednova, Z., Rusinova, A., Kurapov, G., & Semadeni, M. (2023) · Metals · doi:10.3390/met13071177 · Cited by 9
Synthesis and Characterization of High-Entropy Dawsonite-Type Structures
Knorpp, A. J., Allegri, P., Huangfu, S., Vogel, A., & Stuer, M. (2023) · Inorganic Chemistry · doi:10.1021/acs.inorgchem.3c00179 · Cited by 9
Synthesis of nanostructured spinel (NiFeCrZnMg)3O4 as potential cathode material for solid oxide fuel cells via a high entropy strategy
Li, Y.-C., Ye, X.-L., Guo, S.-H., Hou, M., Yang, L., Gao, L., Chen, K., Li, M., & Xue, Z. (2025) · Journal of Power Sources · doi:10.1016/j.jpowsour.2025.237502 · Cited by 8
Valorization of polyethylene waste via chemical looping gasification using high-entropy oxide oxygen carriers
Wang, L., Xie, M., Zhao, W., Wu, X., Yao, W. F., Wei, G., Yao, Y., Yang, X., He, Z., & Huang, Z. (2025) · Journal of environmental chemical engineering · doi:10.1016/j.jece.2025.118937 · Cited by 3
Configurational-entropy driven formation of single-phase high entropy carbide nanoparticles for efficient hydrogen evolution
Feng, L., Meng, Y., Chen, Y., Zhu, Z., Zou, Y.-M., Zhang, W.-B., Xiang, C., Liu, E., Chen, D.-J., Tang, Y., et al. (2025) · Rare Metals · doi:10.1007/s12598-025-03468-8 · Cited by 8
High-entropy oxide for enhanced supercapacitors and precise electrochemical detection of dopamine at nanomolar levels
Sivasurya, E., Ashamary, F., Elancheziyan, M., Harathi, J., Monika, M., Arivazhagan, M., Bhuvanendran, N., Mary, S., Atchudan, R., Kalambate, P. K., et al. (2025) · Next Materials · doi:10.1016/j.nxmate.2025.100699 · Cited by 8
Enhanced energy-storage performance of equimolar high-entropy ceramics under moderate electric field by NaNbO3 modulation
Zhu, W.-J., Cao, W., Cheng, C., Zheng, J., & Wang, C.-C. (2025) · Ceramics International · doi:10.1016/j.ceramint.2025.07.306 · Cited by 8
Rational design of large-scale high-entropy alloy nanosheets anode with excellent lithium storage performance
Li, J., Xu, W., Yin, W., Cui, Q., Xia, S., Tao, Z., Hu, F. X., Wang, N., Zhu, Y., Wei, H. A., et al. (2025) · Materials Chemistry and Physics · doi:10.1016/j.matchemphys.2025.130450 · Cited by 7
Alkaline hydrogen evolution reaction catalyzed by atomically dispersed ruthenium on phosphorus-nitrogen co-doped porous carbon
Liu, S., Shen, L., Tang, Y., Guo, C., Francesco Ciucci, A., & Tang, Z. (2024) · International Journal of Hydrogen Energy · doi:10.1016/j.ijhydene.2024.07.374 · Cited by 9
Anchoring magic NiCo2O4/NiO on Ni foam as an effective and binder-free electrocatalyst for boosting hydrogen evolution reaction
Faraji, H., Hemmati, K., Mirabbaszadeh, K., & Ebrahimi, M. (2024) · Colloids and Surfaces A Physicochemical and Engineering Aspects · doi:10.1016/j.colsurfa.2024.134863 · Cited by 9
Structural modeling of high-entropy oxides battery anodes using x-ray absorption spectroscopy
Marques, O. J., & Segre, C. (2024) · Journal of Applied Physics · doi:10.1063/5.0206316 · Cited by 8
First principles calculation and corrosion resistance study of Fe60CrxNi40-x medium entropy alloy
Wang, W., Wu, D.-T., Gao, Y., Zhu, Z.-H., & Zou, Y. (2024) · Materials Today Communications · doi:10.1016/j.mtcomm.2024.109232 · Cited by 8
Facile synthesis of self-supported (NiCoZnCrFe)Se materials for supercapacitors and oxygen evolution reaction
Liu, X., Dong, J., Li, H., Lv, N., Guo, Z., Li, T., & Luo, J. (2024) · Materials Research Bulletin · doi:10.1016/j.materresbull.2024.112914 · Cited by 9
Advancing zinc-based batteries for next-generation energy storage: Key challenges, mitigation strategies, and future perspectives
Zhang, Y., Li, H., Qiu, S., Qian, J., Wu, F., Bai, Y., Wu, C. K., & Li, Y. (2026) · eScience · doi:10.1016/j.esci.2026.100567 · Cited by 9
High‐Entropy 2D MXenes: A New Paradigm for Energy Storage
Awan, H. T. A., Aboalhassan, A. A., Abdah, M. A. A. M., Mustafa, M. N., Saidi, N. M., Walvekar, R., & Khalid, M. (2026) · Battery Energy · doi:10.1002/bte2.70086 · Cited by 7
“These reinforced properties make HE‐MX promising for use in corrosive, high‐temperature, high‐pressure and thermally demanding environments [43].”
Entropy engineering strategies in nickel-based layered cathode materials: Advances in structural stabilization and electrochemical performance
Abulimiti, A., Zhang, Y., Hua, Y., Cui, C., Dai, W., Zhao, C., & Huang, S. (2026) · Applied Energy · doi:10.1016/j.apenergy.2025.127054 · Cited by 7
Nanostructured high-entropy alloys: Cutting-edge frontiers in sustainable electrocatalysis
Wang, W., & Tong, Y. (2025) · Materials Today Energy · doi:10.1016/j.mtener.2025.102174 · Cited by 4
Toward high entropy material discovery for energy applications using computational and machine learning methods
Mashhadimoslem, H., Karimi, P., Elkamel, A., & Yu, A. (2025) · npj Computational Materials · doi:10.1038/s41524-025-01918-6 · Cited by 13
“…and electrodes for rechargeable B/S. Computational methods are necessary to fully understand the complex behavior of HEMs, particularly in electrochemical systems where experimental methods are hindered by the complexity of the materials ’ reaction and the conditions under which they operate 35 .”
Platinum-free medium-entropy FeCoNiCu selenide/N-CNT electrocatalyst with superior ORR activity and long-term stability in alkaline medium
Wang, Z.-M., Yan, H., Liu, Z., Wang, K., Zhou, M., Tong, Z., Shi, H., Wang, F., Liu, G., Ni, Z., et al. (2025) · International Journal of Hydrogen Energy · doi:10.1016/j.ijhydene.2025.151899 · Cited by 8
Structural insights and electrochemical applications of high-entropy oxides: A comprehensive review
Sheikh, K. A., & Khan, M. M. (2025) · Progress in Engineering Science · doi:10.1016/j.pes.2025.100105 · Cited by 11
Tuning High-Entropy Oxides for Oxygen Evolution Reaction Through Electrocatalytic Water Splitting: Effects of (MnFeNiCoX)3O4 (X = Cr, Cu, Zn, and Cd) on Electrocatalytic Performance
Salmasi, M. Z., Narimani, A., Omidkar, A., & Song, H. (2025) · Catalysts · doi:10.3390/catal15090827 · Cited by 7
A Medium-Entropy Li-Garnet Solid Electrolyte with Ultrahigh Ionic Conductivity and Outstanding Electrochemical Stability for Solid-State Batteries
Umair, M., Rana, H. T. H., Yu, S.-Z., & Wei, J. (2025) · Energy Storage Materials · doi:10.1016/j.ensm.2025.104484 · Cited by 7
High entropy alloy/graphite composite as a new strategy to enhance the performance of lithium-ion batteries
Xiao, W., Xu, H., Pei, Y.-R., Hu, L., & Yang, Z. (2025) · Inorganic Chemistry Communications · doi:10.1016/j.inoche.2025.114594 · Cited by 7
Breaking the pH limitation by Mo modulated amorphous medium-entropy alloys as efficient advanced oxidation catalysts
Wu, X.-L., Liang, S., Jia, L., Liu, Y.-F., Huang, Y., Liu, Y.-J., Chen, L.-Y., Yang, Y., & Tao, P.-J. (2025) · Journal of Environmental Chemical Engineering · doi:10.1016/j.jece.2025.116151 · Cited by 7
Prospects for the development of materials based on high-entropy oxides, carbides, and oxycarbides stable at high temperatures
Stolyarova, V., Vasileva, I., Vorozhtcov, V. A., & Sokolova, T. (2025) · Russian Chemical Reviews · doi:10.59761/rcr5156 · Cited by 7
Recent advancements of high entropy ceramic/carbon composites toward rechargeable batteries
Li, H., Cheng, X.-Q., Zhao, J.-Y., Gao, M., Xu, H., & Wang, X.-M. (2025) · Journal of Alloys and Compounds · doi:10.1016/j.jallcom.2024.178237 · Cited by 7
Exploring the inhibitory effect of WTaVCr high-entropy alloys on hydrogen retention: From dissolution, diffusion to desorption
Yang, T.-R., Wang, Y., Li, Y., Zhao, S., Zhou, H.-B., Tian, F., & Lu, G. (2024) · Journal of Nuclear Materials · doi:10.1016/j.jnucmat.2024.155346 · Cited by 6
Recent developments strategies in high entropy modified lithium-rich layered oxides cathode for lithium-ion batteries
Ajayi, S., Dolla, T., Bello, I. T., Liu, X.-Y., Makgwane, P., Mathe, M., & Ehi-Eromosele, C. O. (2024) · Inorganic Chemistry Communications · doi:10.1016/j.inoche.2024.113721 · Cited by 7
Binder-Dependent Electrochemical Properties of High Entropy Oxide Anodes for Lithium-Ion Batteries
Patra, J., Nguyen, T., Panda, A., Majumder, S. B., Yang, C.-C., Wu, T.-Y., Su, Y.-S., Hsieh, C.-T., Ting, J., & Chang, J.-K. (2024) · Electrochimica Acta · doi:10.1016/j.electacta.2024.144653 · Cited by 7
Synthesis and Catalytic Performance of High-Entropy Rare-Earth Perovskite Nanofibers: (Y0.2La0.2Nd0.2Gd0.2Sm0.2)CoO3 in Low-Temperature Carbon Monoxide Oxidation
Krawczyk, P. A., Wyrwa, J., & Kubiak, W. (2024) · Materials · doi:10.3390/ma17081883 · Cited by 7
“Known for their versatility in both bulk [9,10] and thin-film configurations [11], perovskite-type high-entropy oxides exhibit distinctive properties that make them highly attractive in a variety of applications covering technological domains from photovoltaics [12–15] to electronics [16–19], to a…”
Background
High-entropy and compositionally complex battery materials
Strauss, F., Botros, M., Breitung, B., & Brezesinski, T. (2024) · Journal of Applied Physics · doi:10.1063/5.0200031 · Cited by 7
Self-citation
Thermally stable high-entropy oxide glasses with high refractive index
Zhang, X.-Y., Zhang, J.-R., Li, L., & Qi, X. (2023) · Journal of Materials Science · doi:10.1007/s10853-023-08819-3 · Cited by 7
Design and preparation of high-entropy fluorite oxides based on R¯-S diagram
Lan, Q., Ma, J.-X., Li, S.-Y., Chen, K.-P., Li, C.-W., & An, L. (2023) · Ceramics International · doi:10.1016/j.ceramint.2023.03.128 · Cited by 7
Synthesis of porous Mn-based spinel microspheres with enhanced lithium storage properties
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Evolution of a self-assembled chessboard nanostructure spinel in a CoFeGaMnZn multicomponent oxide
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“MCOs are potential candidate materials for high-density memory devices, nanoscale batteries and thermoelectric devices [9,10].”
Background
Recent advances in high-entropy oxides electrocatalysts for oxygen evolution reaction
Huang, J.-J., Zhang, C., Geng, Y., Li, S., Zhao, Z., & Bai, J.-R. (2026) · Journal of Alloys and Compounds · doi:10.1016/j.jallcom.2026.189310 · Cited by 7
High and stable energy-storage performance in BiFeO3 ceramics via high-entropy design
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High-performance, high-entropy perovskite cathodes for low-temperature solid-oxide fuel cells
Dąbrowa, J., Zielińska, K., Nowakowska, M. Z. M., Szymczak, M. M., Moździerz, M., Mikuła, A., Li, K.-Y., Czaja, P., Schwab, C., Falkenstein, A., et al. (2026) · Applied Catalysis B: Environment and Energy · doi:10.1016/j.apcatb.2026.126571 · Cited by 6
Extreme compositional complexity in crystalline perovskite oxide: a new paradigm in quantum materials research
Middey, S., Bhattacharya, N., Nevgi, R., Joshi, S. C., & Dey, S. (2026) · Advances in Physics X · doi:10.1080/23746149.2026.2646243 · Cited by 5
Properties and performances of high-entropy materials in batteries
Wang, J., Jiang, J. Z., Liaw, P. K., & Zhang, Y. (2025) · International Journal of Minerals Metallurgy and Materials · doi:10.1007/s12613-025-3275-7 · Cited by 7
Fluorine-engineered high-entropy layered oxyfluorides enable ultrafast and stable sodium storage: Synergistic stabilization and kinetics enhancement
Li, J., Zhang, D., Zhao, L.-N., Wen, Y., Zhang, H.-J., Bi, S., Lu, S., Yin, P., Liu, L., Shi, F., et al. (2025) · Journal of Power Sources · doi:10.1016/j.jpowsour.2025.237487 · Cited by 6
Defect engineering in high‐entropy ceramics glaze enable infrared emissivity and antibacterial properties
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“17,18 Among them, high-entropy ceramics (HECs), a new class of materials composed of multiple metal elements in nearly equal proportions, offer distinct advantages in IR emission control.”
Recent advances in high entropy alloys for electrochemical water splitting: Materials, synthesis, and applications
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Authors: Ma, Y., Ma, Y., Wang, Q., Schweidler, S., Botros, M., Fu, T., Hahn, H., Brezesinski, T., & Breitung, B.
Affiliations: Karlsruhe Institute of Technology (DE)
University of Waterloo (CA)
Corresponding author: Ma, Yanjiao
Brezesinski, Torsten
Breitung, Ben
ORCID: Ma, Yanjiao
Ma, Yuan
Wang, Qingsong
Schweidler, Simon
Botros, Miriam
Fu, Tongtong
Hahn, Horst
Brezesinski, Torsten
Breitung, Ben
Venue: Energy & Environmental Science
Publisher: Royal Society of Chemistry (RSC)
Published: 2021
Volume: 14
Issue: 5
Pages: 2883-2905
ISSN: 1754-5692 (ISSN-L)
1754-5706
DOI: 10.1039/d1ee00505g
OpenAlex: W3148416643
Cited by: 963
References: 186
Citations by year: 2026: 187 · 2025: 262 · 2024: 263 · 2023: 137 · 2022: 87 · 2021: 27
FWCI: 54.92
Type: journal article
Language: en
Open access: hybrid
doi.org
Licence: cc-by-nc
creativecommons.org/licenses/by-nc/3.0/ (vor, 91 d)
Locations: Energy & Environmental Science (publishedVersion, cc-by-nc)
Repository KITopen (Karlsruhe Institute of Technology) (publishedVersion, cc-by-nc-nd)
ERef Bayreuth (University of Bayreuth) (submittedVersion)
Zenodo (CERN European Organization for Nuclear Research) (submittedVersion, cc-by)
KITopen
Funders: Deutsche Forschungsgemeinschaft (BR 3499/5-1, HA 1344/43-1, SE 1407/4-2)
Carl-Zeiss-Stiftung
Helmholtz Association
Horizon 2020 (730957, 101017709)
Topics: Physical Sciences › Engineering › Mechanical Engineering › High Entropy Alloys Studies
Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
Physical Sciences › Materials Science › Materials Chemistry › Machine Learning in Materials Science
Keywords: high-entropy materials, hydrogen catalysis, hydrogen storage, CO2 conversion, oxygen catalysis, electrochemical energy storage, energy materials

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High-entropy energy materials: challenges and new opportunities

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