Photoelectron spectrometer for attosecond spectroscopy of liquids and gases
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A new apparatus for attosecond time-resolved photoelectron spectroscopy of liquids and gases is described. It combines a liquid microjet source with a magnetic-bottle photoelectron spectrometer and an actively stabilized attosecond beamline. The photoelectron spectrometer permits venting and pumping of the interaction chamber without affecting the low pressure in the flight tube. This pressure separation has been realized through a sliding skimmer plate, which effectively seals the flight tube in its closed position and functions as a differential pumping stage in its open position. A high-harmonic photon spectrometer, attached to the photoelectron spectrometer, exit port is used to acquire photon spectra for calibration purposes. Attosecond pulse trains have been used to record photoelectron spectra of noble gases, water in the gas and liquid states as well as solvated species. RABBIT scans demonstrate the attosecond resolution of this setup.
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The extension of attosecond science to the liquid phase has been successfully addressed in the XUV spectral region.
“The second challenge, the extension of attosecond science to the liquid phase, has also been successfully addressed in the XUV spectral region [205].”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [205]
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- Authors
- Jordan, I., Huppert, M., Brown, M. A., van Bokhoven, J. A., & Wörner, H. J.
- Affiliations
- ETH Zurich (CH)
- Institute for Chemical and Bioengineering 3 , ETH Zurich, Vladimir-Prelog-Weg 1, 8093 Zurich, Switzerland
- Venue
- Review of Scientific Instruments
- Publisher
- AIP Publishing
- Published
- 2015-12-01
- Volume
- 86
- Issue
- 12
- Pages
- 123905-123905
- ISSN
- 0034-6748 (ISSN-L)
- 1089-7623
- OpenAlex
- W2209335714
- Cited by
- 49
- References
- 42
- Citations by year
- 2026: 2 · 2025: 3 · 2024: 1 · 2023: 3 · 2022: 4 · 2021: 3 · 2020: 11 · 2019: 5 · 2018: 5 · 2017: 9 · 2016: 2 · 2015: 1
- FWCI
- 2.88
- Type
- journal article
- Language
- en
- Open access
- green
- www.dora.lib4ri.ch
- Licence
- other-oa
- Locations
- Review of Scientific Instruments (publishedVersion)
- PubMed (publishedVersion)
- DORA PSI (Paul Scherrer Institute) (submittedVersion, other-oa)
- Repository for Publications and Research Data (ETH Zurich) (submittedVersion, other-oa)
- ETH Zürich Research Collection
- Funders
- ERC Starting Grant (307270)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Materials Science › Surfaces, Coatings and Films › Electron and X-Ray Spectroscopy Techniques
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Atomic and Molecular Physics
- Keywords
- attosecond spectroscopy, photoelectron spectroscopy, liquid microjet, differential pumping, noble gases, water, time-resolved spectroscopy
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Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
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