Development of high harmonic generation spectroscopy of organic molecules and biomolecules
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In this review we will discuss the topic of high order harmonic generation (HHG) from samples of organic and bio-molecules. The possibility to extract useful dynamical and structural information from the measurement of the HHG emission, a technique termed high harmonic generation spectroscopy (HHGS), will be the special focus of our discussions. We will begin by introducing the salient facts of HHG from atoms and simple molecules and explaining the principles behind HHGS. Next the technical difficulties associated with HHG from samples of organic molecules and biomolecules, principally the low sample density and the low ionization potential, will be examined. Then we will present some recent experiments where HHG spectra from samples of these molecules have been measured and discuss what has been learned from these measurements. Finally we will look at the future prospects for HHG spectroscopy of organic molecules, discussing some of the technical and in principle limits of the technique and methods that may ameliorate these limits.
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Important breakthroughs have been achieved in both branches of attosecond spectroscopy, as summarized in recent reviews.
“In both branches, important breakthroughs have been achieved, as summarized in recent reviews [198,199].”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [198]
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- Niikura H, Worner H J, Villeneuve D M and Corkum P B 2011 Probing the spatial structure of a molecular attosecond electron wave-packet using shaped recollision trajectories Phys. Rev. Lett. 107 093004 · DOI
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- Authors
- Marangos, J. P.
- Affiliations
- Imperial College London (GB)
- Corresponding author
- Marangos, J P
- ORCID
- Marangos, J P
- Venue
- Journal of Physics B: Atomic, Molecular and Optical Physics
- Publisher
- IOP Publishing
- Published
- 2016-05-31
- Volume
- 49
- Issue
- 13
- Pages
- 132001
- ISSN
- 0953-4075 (ISSN-L)
- 1361-6455
- OpenAlex
- W2529289822
- Cited by
- 111
- References
- 147
- Citations by year
- 2026: 7 · 2025: 13 · 2024: 9 · 2023: 3 · 2022: 12 · 2021: 16 · 2020: 9 · 2019: 16 · 2018: 12 · 2017: 8 · 2016: 6
- FWCI
- 6.62
- Type
- journal article
- Language
- en
- Open access
- hybrid
- doi.org
- Licence
- Locations
- Journal of Physics B Atomic Molecular and Optical Physics (publishedVersion, cc-by)
- Funders
- European Research Council (ASTEX 290467)
- Engineering and Physical Sciences Research Council (EP/I032517/1)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Spectroscopy and Quantum Chemical Studies
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Terahertz technology and applications
- Keywords
- high harmonic generation, organic compounds, biomolecules, molecular dynamics, molecular structure, attosecond spectroscopy
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