Rare-earth nickelates R NiO 3 : thin films and heterostructures
Open accessAbstract
This review stands in the larger framework of functional materials by focussing on heterostructures of rare-earth nickelates, described by the chemical formula R NiO 3 where R is a trivalent rare-earth R = La, Pr, Nd, Sm, …, Lu. Nickelates are characterized by a rich phase diagram of structural and physical properties and serve as a benchmark for the physics of phase transitions in correlated oxides where electron–lattice coupling plays a key role. Much of the recent interest in nickelates concerns heterostructures, that is single layers of thin film, multilayers or superlattices, with the general objective of modulating their physical properties through strain control, confinement or interface effects. We will discuss the extensive studies on nickelate heterostructures as well as outline different approaches to tuning and controlling their physical properties and, finally, review application concepts for future devices.
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The electrical properties of LNO are sensitive to mechanical stress, grain boundaries, and pores.
“The electrical properties of LNO are sensitive to mechanical stress, grain boundaries, and pores [1,22].”
From Control of Columnar Grain Microstructure in CSD LaNiO3 Films (2023) · cites this paper as [1]
The indexed record’s Abstract (no page given) says that strain control can modulate the physical properties of rare-earth nickelate heterostructures, which provides some support for sensitivity to mechanical stress. The available passages do not address grain boundaries or pores, or specifically link either to LNO’s electrical properties. (LLM, conf=0.78)
Experimental — accuracy not yet measuredThe increase in annealing time from 5 to 10 min slightly decreases resistivity, and this can be caused by improving film crystalline performance.
“However, the increase in annealing time from 5 to 10 min slightly decreases the resistivity value, and this can be caused by improving of the film crystalline performance [1,22].”
From Control of Columnar Grain Microstructure in CSD LaNiO3 Films (2023) · cites this paper as [1]
The indexed entry for Catalano et al. (2018; no page given) describes a review of rare-earth nickelate thin films and ways to tune their properties. The available passages do not address a change in annealing time from 5 to 10 minutes, a resulting resistivity decrease, or improved crystallinity. Searches for those terms found no passage that verifies the claim. (LLM, conf=0.72)
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“This manifests as a geometric change in local bond angles, which may be trackable since correlation effects tend to increase with decreasing bond angle (relative to 180°) [23,33,34].”
BackgroundDynamics of the electrically induced insulator-to-metal transition in rare-earth nickelates
del Valle, J., Rocco, R., Domínguez, C., Fowlie, J., Gariglio, S., Rozenberg, M., & Triscone, J. (2021) · Physical review B · doi:10.1103/physrevb.104.165141 · Cited by 20
Self-citationHigh-density electron doping of SmNiO3 from first principles
Kotiuga, M., & Rabe, K. (2017) · PHYSICAL REVIEW MATERIALS · doi:10.1103/physrevmaterials.3.115002 · Cited by 20
Rare-earth control of phase transitions in infinite-layer nickelates
Zhang, Y.-J., Zhang, J., He, X., Wang, J., & Ghosez, P. (2023) · PNAS Nexus · doi:10.1093/pnasnexus/pgad108 · Cited by 19
“…in perovskites and related compounds is well known as an efficient parameter for tuning phase transitions and has become an essential factor to differentiate the behaviors of different compounds within the same family like in R NiO 3 (44, 45) and the investigated R NiO 2 systems (1, 39).”
BackgroundSudden Collapse of Magnetic Order in Oxygen-Deficient Nickelate Films.
Li, J.-R., Green, R., Zhang, Z., Sutarto, R., Sadowski, J., Zhu, Z.-H., Zhang, G. H., Zhou, D., Sun, Y., He, F., et al. (2020) · Physical Review Letters · doi:10.1103/physrevlett.126.187602 · Cited by 19
Spatial Interactions in Hydrogenated Perovskite Nickelate Synaptic Networks.
Bisht, R. S., Park, J., Yu, H., Wu, C., Tilak, N., Rangan, S., Park, T. J., Yuan, Y., Das, S., Goteti, U. S., et al. (2023) · Nano letters (Print) · doi:10.1021/acs.nanolett.3c02076 · Cited by 18 · see citing works
Phase formation in hole- and electron-doped rare-earth nickelate single crystals
Puphal, P., Sundaramurthy, V., Zimmermann, V., Küster, K., Starke, U., Isobe, M., Keimer, B., & Hepting, M. (2023) · APL Materials · doi:10.1063/5.0160912 · Cited by 18
Carrier Doping Physics of Rare Earth Perovskite Nickelates RENiO3
Li, J., Ramanathan, S., & Comin, R. (2022) · Frontiers of Physics · doi:10.3389/fphy.2022.834882 · Cited by 18
Origin of functionality for functional materials at atomic scale
Xiao, D., & Gu, L. (2020) · Nano Select · doi:10.1002/nano.202000020 · Cited by 22 · see citing works
Beyond Coherent Oxide Heterostructures: Atomic‐Scale Structure of Misfit Dislocations
Dholabhai, P., & Uberuaga, B. (2019) · Advanced Theory and Simulations · doi:10.1002/adts.201900078 · Cited by 18
Dynamics of the photoinduced insulator-to-metal transition in a nickelate film
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Proton-Doped Strongly Correlated Perovskite Nickelate Memory Devices
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“photovoltaics and resistance switching [3], [4].”
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Characteristic length scales of the electrically induced insulator-to-metal transition
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“These compounds are two wellknown members of the rare earth nickelate family [2,6].”
BackgroundInfluentialSelf-citationGoodge, B., Baggari, I. E., Hong, S., Wang, Z., Schlom, D., Hwang, H., & Kourkoutis, L. (2022) · Microscopy and Microanalysis · doi:10.1017/s1431927622000125 · Cited by 17
“…complex oxides, for instance, the perovskite lattice may undergo distortions that underlie the diversity of electronic properties, including oxygen octahedral rotations (Catalano et al., 2018), cation antipolar distortions, and ferroelectric displacements (Ahn et al., 2004; Spaldin & Fiebig, 2005).”
BackgroundVibrational properties of LaNiO3 films in the ultrathin regime
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Self-citationPrajapati, G. L., Das, S., & Rana, D. S. (2019) · ACS Applied Materials and Interfaces · doi:10.1021/acsami.9b09362 · Cited by 17
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Identifying a perovskite phase in rare-earth nickelates using X-ray photoelectron spectroscopy
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Structural and electronic properties of rare-earth chromites: A computational and experimental study
Shi, J., Fernando, G., Dang, Y., Suib, S., & Jain, M. (2022) · Physical review B · doi:10.1103/physrevb.106.165117 · Cited by 16 · see citing works
Bian, Y., Li, H.-Y., Yan, F.-B., Li, H.-F., Wang, J.-O., Zhang, H., Jiang, Y., Chen, N., & Chen, J. (2021) · Applied Physics Letters · doi:10.1063/5.0082917 · Cited by 16
- Authors
- Catalano, S., Gibert, M., Fowlie, J., Íñiguez, J., Triscone, J.-M., & Kreisel, J.
- Affiliations
- University of Geneva (CH)
- Luxembourg Institute of Science and Technology (LU)
- University of Luxembourg (LU)
- Corresponding author
- Kreisel, J
- Venue
- Reports on Progress in Physics
- Publisher
- IOP Publishing
- Published
- 2018-02-14
- Volume
- 81
- Issue
- 4
- Pages
- 046501
- ISSN
- 0034-4885 (ISSN-L)
- 1361-6633
- OpenAlex
- W2778004626
- Cited by
- 453
- References
- 250
- Citations by year
- 2026: 23 · 2025: 69 · 2024: 55 · 2023: 69 · 2022: 68 · 2021: 61 · 2020: 52 · 2019: 49 · 2018: 7
- FWCI
- 12.47
- Type
- journal article
- Language
- en
- Open access
- green
- orbilu.uni.lu
- Licence
- Locations
- Reports on Progress in Physics (publishedVersion)
- PubMed (publishedVersion)
- Open Repository and Bibliography (University of Luxembourg) (submittedVersion, cc-by-nc-sa)
- Funders
- Fonds National de la Recherche Luxembourg (FNR/P12/4853155)
- FP7 Ideas: European Research Council (319286 (Q-MAC))
- Topics
- Physical Sciences › Materials Science › Materials Chemistry › Electronic and Structural Properties of Oxides
- Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Magnetic and transport properties of perovskites and related materials
- Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Multiferroics and related materials
- Keywords
- rare-earth nickelates, thin films, heterostructures, superlattices, multilayer structures, strain engineering, confinement effects, interface effects, phase transitions, correlated oxides, electron-lattice coupling, functional materials, device applications
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