Resonance Effects in Photoemission Time Delays
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We present measurements of single-photon ionization time delays between the outermost valence electrons of argon and neon using a coincidence detection technique that allows for the simultaneous measurement of both species under identical conditions. The analysis of the measured traces reveals energy-dependent time delays of a few tens of attoseconds with high energy resolution. In contrast to photoelectrons ejected through tunneling, single-photon ionization can be well described in the framework of Wigner time delays. Accordingly, the overall trend of our data is reproduced by recent Wigner time delay calculations. However, besides the general trend we observe resonance features occurring at specific photon energies. These features have been qualitatively reproduced and identified by a calculation using the multiconfigurational Hartree-Fock method, including the influence of doubly excited states and ionization thresholds.
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Pump/probe schemes often use either single attosecond pulses with a rather intense infrared probe pulse or an attosecond pulse train with a weak infrared pulse.
“Pump/probe schemes often use either single attosecond pulses together with a rather intense infrared probe pulse [185,186,191] or an attosecond pulse train together with a weak infrared pulse [187-190, 192, 193].”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [191]
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- Authors
- Sabbar, M., Heuser, S., Boge, R., Lucchini, M., Carette, T., Lindroth, E., Gallmann, L., Cirelli, C., & Keller, U.
- Affiliations
- ETH Zurich (CH)
- Université Libre de Bruxelles (BE)
- Stockholm University (SE)
- University of Bern (CH)
- Venue
- Physical Review Letters
- Publisher
- American Physical Society (APS)
- Published
- 2015-09-23
- Volume
- 115
- Issue
- 13
- Pages
- 133001-133001
- ISSN
- 0031-9007 (ISSN-L)
- 1079-7114
- OpenAlex
- W2150063188
- Cited by
- 106
- References
- 36
- Citations by year
- 2026: 4 · 2025: 1 · 2024: 4 · 2023: 5 · 2022: 9 · 2021: 10 · 2020: 14 · 2019: 13 · 2018: 19 · 2017: 13 · 2016: 11 · 2015: 3
- FWCI
- 7.79
- Type
- journal article
- Language
- en
- Open access
- green
- arxiv.org
- Locations
- Physical Review Letters (publishedVersion)
- PubMed (publishedVersion)
- arXiv (Cornell University) (submittedVersion)
- Virtual Community of Pathological Anatomy (University of Castilla La Mancha) (submittedVersion, other-oa)
- Dépôt institutionnel de l'Université libre de Bruxelles (Université Libre de Bruxelles) (submittedVersion)
- arXiv (Cornell University)
- Funders
- European Research Council (ERC-2012-ADG_20120216)
- Schweizerische Nationalfonds zur Förderung der Wissenschaftlichen Forschung
- Eidgenössische Technische Hochschule Zürich
- Swedish Research Council
- Wenner-Gren Foundation (2012-3668)
- IUAP
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Atomic and Molecular Physics
- Physical Sciences › Physics and Astronomy › Statistical and Nonlinear Physics › Quantum chaos and dynamical systems
- Keywords
- single-photon ionization, Wigner time delay, resonance effects, argon, NEON, valence electrons, attosecond time resolution, doubly excited states, ionization threshold
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