Attosecond dynamics through a Fano resonance: Monitoring the birth of a photoelectron
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Watching as helium goes topsy-turvy: Theorists have long pondered the underpinnings of the Fano resonance, a spectral feature that resembles adjacent rightside-up and upside-down peaks. An especially well-studied instance of this feature appears in the electronic spectrum of helium as a transient state undergoes delayed ionization. Two studies have now traced the dynamics of this state in real time. Gruson et al. used photoelectron spectroscopy to extract the amplitude and phase of the electron wave packet after inducing its interference with reference wave packets tuned into resonance at variable delays. Kaldun et al. used extreme ultraviolet absorption spectroscopy to probe the transient state while variably forcing ionization with a strong near-infrared field. Science , this issue pp. 734 and 738
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Pump/probe schemes often use either single attosecond pulses with a rather intense infrared probe pulse or an attosecond pulse train with a weak infrared pulse.
“Pump/probe schemes often use either single attosecond pulses together with a rather intense infrared probe pulse [185,186,191] or an attosecond pulse train together with a weak infrared pulse [187-190, 192, 193].”
From Roadmap of ultrafast x-ray atomic and molecular physics (2018) · cites this paper as [193]
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Isolating Attosecond Electron Dynamics in Molecules where Nuclei Move Fast
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Non-linear processes in the extreme ultraviolet
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Continuous-variable quantum state tomography of photoelectrons
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Self-citationAttosecond metrology in circular polarization
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Spin–orbit-resolved spectral phase measurements around a Fano resonance
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Extracting attosecond delays from spectrally overlapping interferograms
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Probing Molecular Frame Wigner Time Delay and Electron Wavepacket Phase Structure of CO Molecule
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Resonant two-photon ionization of helium atoms studied by attosecond interferometry
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Revealing Molecular Strong Field Autoionization Dynamics
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Self-citationRole of nuclear-electronic coupling in attosecond photoionization of H2
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Self-citationAttosecond spectroscopy reveals alignment dependent core-hole dynamics in the ICl molecule
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- Authors
- Gruson, V., Barreau, L., Jiménez-Galan, Á., Risoud, F., Caillat, J., Maquet, A., Carré, B., Lepetit, F., Hergott, J.-F., Ruchon, T., Argenti, L., Taïeb, R., Martín, F., & Salières, P.
- Affiliations
- Centre National de la Recherche Scientifique (FR)
- Departamento de Química, Módulo 13, Universidad Autónoma de Madrid, 28049 Madrid, Spain.
- Universidad Autónoma de Madrid (ES)
- LIDYL, CEA, CNRS, Université Paris-Saclay, CEA Saclay, 91191 Gif-Sur-Yvette, France.
- Corresponding author
- Gruson, V.
- Barreau, L.
- ORCID
- Venue
- Science
- Published
- 2016-11-11
- Volume
- 354
- Issue
- 6313
- Pages
- 734-738
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2556793726
- Cited by
- 317
- References
- 44
- Citations by year
- 2026: 20 · 2025: 32 · 2024: 30 · 2023: 25 · 2022: 29 · 2021: 37 · 2020: 47 · 2019: 35 · 2018: 30 · 2017: 31 · 2016: 1
- FWCI
- 15.29
- Type
- journal article
- Language
- en
- Open access
- green
- zenodo.org
- Locations
- Science (publishedVersion)
- PubMed (publishedVersion)
- Hispana (publishedVersion)
- Zenodo (CERN European Organization for Nuclear Research) (publishedVersion, other-oa)
- LA Referencia (Red Federada de Repositorios Institucionales de Publicaciones Científicas) (acceptedVersion, other-oa)
- Tesis Doctorals en Xarxa (Consorci de Serveis Universitaris de Catalunya) (acceptedVersion)
- arXiv (Cornell University) (submittedVersion)
- Journal of International Crisis and Risk Communication Research (submittedVersion)
- HAL (submittedVersion)
- Biblos-e Archivo (Universidad Autónoma de Madrid) (submittedVersion, public-domain)
- arXiv (Cornell University)
- Funders
- European Union (H2020-MSCA-ITN-MEDEA-641789)
- Agence Nationale de la Recherche (ANR-15-CE30-0001-01-CIMBAAD, ANR11-EQPX0005-ATTOLAB)
- European Research Council (XCHEM 290853)
- European COST Action (XLIC CM1204)
- MINECO (FIS2013-42002-R)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Atomic and Molecular Physics
- Physical Sciences › Physics and Astronomy › Statistical and Nonlinear Physics › Quantum chaos and dynamical systems
- Keywords
- attosecond dynamics, Fano resonance, autoionizing resonances, electron interferometry, two-photon transitions, helium, electron correlation, coherent control
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