Giant effective magnetic fields from optically driven chiral phonons in 4 f paramagnets
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We present a mechanism by which optically driven chiral phonon modes in rare-earth trihalides generate giant effective magnetic fields acting on the paramagnetic $4f$ spins. With cerium trichloride (${\mathrm{CeCl}}_{3}$) as our example system, we calculate the coherent phonon dynamics in response to the excitation by an ultrashort terahertz pulse using a combination of phenomenological modeling and first-principles calculations. We find that effective magnetic fields of over 100 T can possibly be generated that polarize the spins for experimentally accessible pulse energies. The direction of induced magnetization can be reversed by changing the handedness of circular polarization of the laser pulse. The underlying process is a phonon analog of the inverse Faraday effect in optics that has been described recently, and which enables novel ways of achieving control over and switching of magnetic order at terahertz frequencies.
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A recent theoretical work found that in semimetals and small-gap (tens of millielectronvolts) insulators, a four orders of magnitude enhancement of the phonon magnetic moment can be expected.
“A recent theoretical work29 found that in semimetals and small-gap (tens of millielectronvolts) insulators, a four orders of magnitude enhancement of the phonon magnetic moment can be expected30–32.”
From Terahertz electric-field-driven dynamical multiferroicity in SrTiO3 (2024) · cites this paper as [32]
Section V says that phonon magnetic moments arising from topological band features in semimetals do not play a role in this work. The Discussion instead predicts much larger effective magnetic fields and induced moments from optically driven phonons in a 4f paramagnet (CeCl₃); it does not predict a four-orders-of-magnitude enhancement of the phonon magnetic moment in semimetals or small-gap insulators. Page numbers were not available in our copy. (LLM, conf=0.82)
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Disorder-Induced Slow Relaxation of Phonon Polarization
Suzuki, Y., & Murakami, S. (2025) · Physical Review Letters · doi:10.1103/z8wj-f384 · Cited by 2 · see citing works
All-Optical Switching in Ferromagnets and Its Application to Magnetic Weyl Semimetals
Yoshikawa, N., Ogawa, K., & Shimano, R. (2025) · Journal of the Physical Society of Japan · doi:10.7566/jpsj.94.111005 · Cited by 2 · see citing works
The rise of chiral phononics: From fundamental concepts to emergent quasiparticle interactions
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Crystal growth, magnetic and magnetocaloric properties of J eff = 1/2 quantum antiferromagnet CeCl 3
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Ultrafast Faraday rotation probe of chiral phonon-polaritons in LiNbO 3
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SU ( N ) spin-phonon simulations of Floquet dynamics in spin S > 1 2 Mott insulators
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Giant Barnett effect from moving dislocations
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Pseudochiral Phonons from Octupolar Magnetic Order
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- Authors
- Juraschek, D. M., Neuman, T., & Narang, P.
- Affiliations
- Harvard University (US)
- Venue
- Physical Review Research
- Publisher
- American Physical Society (APS)
- Published
- 2022-02-17
- Volume
- 4
- Issue
- 1
- ISSN
- 2643-1564 (ISSN-L)
- OpenAlex
- W4213036136
- Cited by
- 113
- References
- 114
- Citations by year
- 2026: 24 · 2025: 34 · 2024: 31 · 2023: 22 · 2022: 2
- FWCI
- 8.31
- Type
- journal article
- Language
- en
- Open access
- gold
- doi.org
- Licence
- Locations
- Physical Review Research (publishedVersion, cc-by)
- arXiv (Cornell University) (submittedVersion)
- DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion)
- OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
- arXiv (Cornell University)
- Funders
- Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung (184259)
- Defense Advanced Research Projects Agency (D18AC00014)
- Gordon and Betty Moore Foundation (GBMF8048)
- Office of Science
- U.S. Department of Energy (DE-AC02-05CH11231)
- National Energy Research Scientific Computing Center (GBMF8048)
- Topics
- Physical Sciences › Physics and Astronomy › Condensed Matter Physics › Advanced Condensed Matter Physics
- Physical Sciences › Physics and Astronomy › Condensed Matter Physics › Rare-earth and actinide compounds
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Magnetic properties of thin films
- Keywords
- chiral phonons, effective magnetic field, cerium trichloride, coherent phonon dynamics, terahertz pulses, inverse Faraday effect, spin polarization
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Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
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