The DOI matches its Crossref record; 16 of the 16 references it cites were found in a registry or an index.
Defining a Materials Database for the Design of Copper Binary Alloy Catalysts for Electrochemical CO2 Conversion
Abstract
While Cu electrodes are a versatile material in the electrochemical production of desired hydrocarbon fuels, Cu binary alloy electrodes are recently proposed to further tune reaction directionality and, more importantly, overcome the intrinsic limitation of scaling relations. Despite encouraging empirical demonstrations of various Cu‐based metal alloy systems, the underlying principles of their outstanding performance are not fully addressed. In particular, possible phase segregation with concurrent composition changes, which is widely observed in the field of metallurgy, is not at all considered. Moreover, surface‐exposed metals can easily form oxide species, which is another pivotal factor that determines overall catalytic properties. Here, the understanding of Cu binary alloy catalysts for CO 2 reduction and recent progress in this field are discussed. From the viewpoint of the thermodynamic stability of the alloy system and elemental mixing, possible microstructures and naturally generated surface oxide species are proposed. These basic principles of material science can help to predict and understand metal alloy structure and, moreover, act as an inspiration for the development of new binary alloy catalysts to further improve CO 2 conversion and, ultimately, achieve a carbon‐neutral cycle.
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Progress and perspectives of electrochemical CO2 reduction on copper in aqueous electrolyte
Nitopi, S., Bertheussen, E., Scott, S. B., Liu, X., Engstfeld, A. K., Horch, S., Seger, B., Stephens, I. E. L., Chan, K., Hahn, C., et al. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00705 · Cited by 5,223
Multifunctional Transition Metal‐Based Phosphides in Energy‐Related Electrocatalysis
Li, Y., Dong, Z., & Jiao, L. (2020) · Advanced Energy Materials · doi:10.1002/aenm.201902104 · Cited by 603
Electrochemical CO2 reduction (CO2RR) to multi-carbon products over copper-based catalysts
Woldu, A. R., Huang, Z., Zhao, P., Hu, L., & Astruc, D. (2022) · Coordination Chemistry Reviews · doi:10.1016/j.ccr.2021.214340 · Cited by 578
Alloying of Cu with Ru Enabling the Relay Catalysis for Reduction of Nitrate to Ammonia
Gao, W., Xie, K., Xie, J., Wang, X., Zhang, H., Chen, S., Wang, H., Li, Z., & Li, C. (2023) · Advanced Materials · doi:10.1002/adma.202202952 · Cited by 532
Cu-Ag Tandem Catalysts for High-Rate CO2 Electrolysis toward Multicarbons
Chen, C., Li, Y., Yu, S., Louisia, S., Jin, J., Li, M., Ross, M. B., & Yang, P. (2020) · Joule · doi:10.1016/j.joule.2020.07.009 · Cited by 502
Metadata
- Authors
- Lee, C. W., Yang, K. D., Nam, D., Jang, J. H., Cho, N. H., Im, S. W., & Nam, K. T.
- Venue
- Advanced Materials
- Publisher
- Wiley
- Published
- 2018-01-24
- Volume
- 30
- Issue
- 42
- Pages
- e1704717-e1704717
- ISSN
- 0935-9648 (ISSN-L)
- 1521-4095
- OpenAlex
- W2791012639
- Cited by
- 206
- References
- 16
- FWCI
- 6.16
- Type
- journal article
- Language
- en
- Open access
- closed
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- Lee, C. W., Yang, K. D., Nam, D., Jang, J. H., Cho, N. H., Im, S. W., & Nam, K. T. (2018). Defining a Materials Database for the Design of Copper Binary Alloy Catalysts for Electrochemical CO2 Conversion. Advanced Materials. https://doi.org/10.1002/adma.201704717
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