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A Comprehensive Approach toward Stable Lithium–Sulfur Batteries with High Volumetric Energy Density
Abstract
A comprehensive approach is reported to construct stable and high volumetric energy density lithium–sulfur batteries, by coupling a multifunctional and hierarchically structured sulfur composite with an in‐situ cross‐linked binder. Through a combination of first‐principles calculations and experimental studies, it is demonstrated that a hybrid sulfur host composed by alternately stacking graphene and layered graphitic carbon nitride embraces high electronic conductivity as well as high polysulfide adsorptivity. It is further shown that the cross‐linked elastomeric binder empowers the hierarchical sulfur composites—multi‐microns in size—with the ability to form crack‐free and compact high‐loading electrodes using traditional slurry processing. Using this approach, electrodes with up to 14.9 mg cm−2 sulfur loading and an extremely low electrolyte/sulfur ratio as low as 3.5: 1 µL mg−1 are obtained. This study sheds light on the essential role of multifaceted cathode design and further on the challenges facing lithium metal anodes in building high volumetric energy density lithium–sulfur batteries.
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Li-O2 and Li-S batteries with high energy storage
Bruce, P. G., Freunberger, S. A., Hardwick, L. J., & Tarascon, J.-M. (2012) · Nature Materials · doi:10.1038/nmat3191 · Cited by 9,479
Hydrogen evolution by a metal-free electrocatalyst
Zheng, Y., Jiao, Y., Zhu, Y., Li, L. H., Han, Y., Chen, Y., Du, A., Jaroniec, M., & Qiao, S. Z. (2014) · Nature Communications · doi:10.1038/ncomms4783 · Cited by 2,236
Cited by
Review on High‐Loading and High‐Energy Lithium–Sulfur Batteries
Peng, H., Huang, J., Cheng, X., & Zhang, Q. (2017) · Advanced Energy Materials · doi:10.1002/aenm.201700260 · Cited by 1,746
Advances in Lithium–Sulfur Batteries: From Academic Research to Commercial Viability
Chen, Y., Wang, T., Tian, H., Su, D., Zhang, Q., & Wang, G. (2021) · Advanced Materials · doi:10.1002/adma.202003666 · Cited by 870
Current Status and Future Prospects of Metal–Sulfur Batteries
Chung, S., & Manthiram, A. (2019) · Advanced Materials · doi:10.1002/adma.201901125 · Cited by 622
Chen, T., Zhang, Z., Cheng, B., Chen, R., Hu, Y., Ma, L., Zhu, G., Liu, J., & Jin, Z. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.7b06973 · Cited by 502
Progress on the Critical Parameters for Lithium–Sulfur Batteries to be Practically Viable
Chung, S., Chang, C., & Manthiram, A. (2018) · Advanced Functional Materials · doi:10.1002/adfm.201801188 · Cited by 477
Metadata
- Authors
- Pang, Q., Liang, X., Kwok, C. Y., Kulisch, J., & Nazar, L. F.
- Venue
- Advanced Energy Materials
- Publisher
- Wiley
- Published
- 2016-11-18
- Volume
- 7
- Issue
- 6
- ISSN
- 1614-6832 (ISSN-L)
- 1614-6840
- OpenAlex
- W2550906466
- Cited by
- 321
- References
- 2
- FWCI
- 21.04
- Type
- journal article
- Language
- en
- Open access
- closed
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- Pang, Q., Liang, X., Kwok, C. Y., Kulisch, J., & Nazar, L. F. (2017). A Comprehensive Approach toward Stable Lithium–Sulfur Batteries with High Volumetric Energy Density. Advanced Energy Materials. https://doi.org/10.1002/aenm.201601630
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