Photochemical and acoustic interactions of biochar with CO 2 and H 2 O: Applications in power generation and CO 2 capture
Abstract
A critical literature review suggests that carbonaceous compounds react with (CO 2 +H 2 O) mixture through thermal, photochemical, and sonochemical/sonophysical routes. A biochar was selected for studying these effects at 60°C and 1 atm for its potential benefits on power generation and CO 2 capture. All treatments remove sizable minerals (K, Na, and Si) detrimental in power generation, and introduce carbon (up to 16% of original carbon in biochar) into the biochar matrix. Most treatments show increased hydrogen (up to 24%). Treatments lead to notable increased heating value of biochar (up to 50%). Treated biochars show increase (up to 19 fold) in internal surface area. The ultrasound energy output is a fraction of the increased heating value. Thus, pretreatment is potentially attractive for increasing the energy efficiency in combustion and gasification. Moreover, better understandings of the salient reactions of these processes will be advantageous for the development of advanced adsorbents for CO 2 capture. © 2014 American Institute of Chemical Engineers AIChE J , 60: 1054–1065, 2014
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Ultrasound cavitation results in exfoliation of graphitic clusters, removal of mineral matter, and opening of pores, thereby increasing microporous surface area.
“Ultrasound cavitation results in the exfoliation of the graphitic clusters of the biochar structure, removal of mineral matter, and opening of the pores, thereby increasing microporous surface area.”
From Effect of Pyrolysis Temperature on PhysicoChemical Properties and Acoustic-Based Amination of Biochar for Efficient CO2 Adsorption (2020) · cites this paper as Chen et al., 2014
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Sajjadi, B., Chen, W.-Y., & Mattern, D. L. (2022) · Biomass and Bioenergy · doi:10.1016/j.biombioe.2022.106420 · Cited by 7 · see citing works
Date palm waste biochar for the adsorptive removal of pharmaceuticals: a review
Abdelaal, A. H., Ahmed, A. K., Wang, H., Dalahmeh, S. S., Chehimi, M. M., Abdullah, A. M., & Jlassi, K. (2026) · Environmental Sciences Europe · doi:10.1186/s12302-026-01333-8 · Cited by 4 · see citing works
Mulabagal, V., Baah, D. A., Egiebor, N. O., Sajjadi, B., Chen, W.-Y., Viticoski, R. L., & Hayworth, J. S. (2025) · Springer eBooks · doi:10.1007/978-3-031-84483-6_80 · Cited by 3 · see citing works
Ming, T., Liu, W., Wu, Y., Gui, J., Peng, K., & Pan, T. (2016) · Elsevier eBooks · doi:10.1016/b978-0-12-805370-6.00001-6 · Cited by 3 · see citing works
Modeling radical edge-site reactions of biochar in CO2/water solution under ultrasonic treatment
Zubatiuk, T. A., Sajjadi, B., Hill, G., Leszczyńska, D., Chen, W.-Y., & Leszczyński, J. (2017) · Chemical Physics Letters · doi:10.1016/j.cplett.2017.09.058 · Cited by 2 · see citing works
Acoustic Treatment of a Coal Gasification Residue for Extraction of Selenium
Sajjadi, B., Chen, W.-Y., & Chatterjee, R. (2019) · Energy & Fuels · doi:10.1021/acs.energyfuels.9b00683 · Cited by 2 · see citing works
Bhadha, J. H., Jennewein, S. P., & Khatiwada, R. (2017) · Sustainable Agriculture Research · doi:10.5539/sar.v6n4p1 · Cited by 1 · see citing works
Mulabagal, V., Baah, D. A., Egiebor, N. O., Sajjadi, B., Chen, W.-Y., Viticoski, R. L., & Hayworth, J. S. (2024) · Springer eBooks · doi:10.1007/978-1-4614-6431-0_80-3 · Cited by 2 · see citing works
Current and Emerging Materials for Zero Energy Buildings
Durakovic, B. (2026) · Green energy and technology · doi:10.1007/978-3-032-16027-0_6
Joshi, R. C., & Shrivastava, S. K. (2026) · Discover Agriculture · doi:10.1007/s44279-026-00734-w
Fu, S., Yang, H., de Jong, W., & Kortlever, R. (2026) · Carbon Energy · doi:10.1002/cey2.70299
- Authors
- Chen, W., Mattern, D. L., Okinedo, E., Senter, J. C., Mattei, A. A., & Redwine, C. W.
- Affiliations
- University of Mississippi (US)
- Corresponding author
- Chen, Wei‐Yin
- Venue
- AIChE Journal
- Publisher
- Wiley
- Published
- 2014-01-16
- Volume
- 60
- Issue
- 3
- Pages
- 1054-1065
- ISSN
- 0001-1541 (ISSN-L)
- 1547-5905
- OpenAlex
- W2133672197
- Cited by
- 56
- References
- 61
- Citations by year
- 2026: 5 · 2025: 2 · 2024: 2 · 2023: 4 · 2022: 4 · 2021: 5 · 2020: 7 · 2019: 6 · 2018: 8 · 2017: 4 · 2016: 5 · 2015: 3 · 2014: 1
- FWCI
- 2.25
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- AIChE Journal (publishedVersion)
- Topics
- Physical Sciences › Engineering › Biomedical Engineering › Thermochemical Biomass Conversion Processes
- Physical Sciences › Engineering › Mechanical Engineering › Carbon Dioxide Capture Technologies
- Physical Sciences › Engineering › Mechanical Engineering › Mining and Gasification Technologies
- Keywords
- biochar, photochemical reactions, sonochemical reactions, mineral removal, hydrogen production, calorific value, surface area, electricity generation, gasification, combustion
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