Cited by 138Carbon Dioxide Capture TechnologiesThermochemical Biomass Conversion ProcessesIndustrial Gas Emission Control

The Application of Biochar for CO 2 Capture: Influence of Biochar Preparation and CO 2 Capture Reactors

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Zhang, Chen, Ji, Ying, Li, Chunchun, Zhang, Yingrui, Sun, Shuzhuang, Xu, Yikai, Jiang, Long, Wu, Chunfei·2023·Industrial & Engineering Chemistry Research

Abstract

High Resolution Image Download MS PowerPoint Slide This work investigates three types of biochar (bamboo charcoal, wood pellet, and coconut shell) for postcombustion carbon capture. Each biochar is structurally modified through physical (H 2 O, CO 2 ) and chemical (ZnCl 2, KOH, H 3 PO 4 ) activation to improve carbon capture performance. Three methods (CO 2 adsorption isotherms, CO 2 fixed-bed adsorption, and thermogravimetric analysis) are used to determine the CO 2 adsorption capacity. The results show that a more than 2.35 mmol·g –1 (1 bar, 298 K) CO 2 capture capacity was achieved using the activated biochar samples. It is also demonstrated that the CO 2 capture performance by biochar depends on multiple surface and textural properties. A high surface area and pore volume of biochar resulted in an enhanced CO 2 capture capacity. Furthermore, the O*/C ratio and pore width show a negative correlation with the CO 2 capture capacity of biochars.

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Crossref · 10.1021/acs.iecr.3c00445

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Research works printed but not linked: 2

  1. Lehmann J.; Joseph S. Biochar for environmental management: an introduction. Biochar for environmental management; Routledge: 2015; pp 1– 13.
  2. XIAO A.-Y.; ZHANG R.-C. Adsorption equilibrium and diffusion of CH4, N2 and CO2 in coconut shell activated carbon. Journal of China Coal Society 2010, 35 (8), 1341– 1346.

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Authors
Zhang, C., Ji, Y., Li, C., Zhang, Y., Sun, S., Xu, Y., Jiang, L., & Wu, C.
Affiliations
  • Queen's University Belfast (GB)
  • Zhejiang University (CN)
Corresponding author
  • Jiang, Long
  • Wu, Chunfei
Venue
Industrial & Engineering Chemistry Research
Published
2023-06-29
Volume
62
Issue
42
Pages
17168-17181
ISSN
  • 0888-5885 (ISSN-L)
  • 1520-5045
OpenAlex
W4382600535
Cited by
138
References
51
Citations by year
2026: 64 · 2025: 46 · 2024: 25 · 2023: 3
FWCI
13.56
Type
journal article
Language
en
Open access
Locations
  • Industrial & Engineering Chemistry Research (publishedVersion, cc-by)
  • PubMed Central (publishedVersion, cc-by)
  • PubMed (publishedVersion)
  • Research Portal (Queen's University Belfast) (publishedVersion, cc-by)
Funders
H2020 Marie Sklodowska-Curie Actions (823745, 872102)
Topics
  • Physical Sciences › Engineering › Mechanical Engineering › Carbon Dioxide Capture Technologies
  • Physical Sciences › Engineering › Biomedical Engineering › Thermochemical Biomass Conversion Processes
  • Physical Sciences › Engineering › Mechanical Engineering › Industrial Gas Emission Control
Keywords
biochar, CO2 capture, post-combustion carbon capture, bamboo charcoal, coconut shell, chemical activation, CO2 adsorption isotherms, fixed-bed adsorption, surface area, pore volume, O/C ratio, pore width, adsorption capacity

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