The DOI matches its Crossref record; 7 of the 7 references it cites were found in a registry or an index.
A Highly Selective Copper–Indium Bimetallic Electrocatalyst for the Electrochemical Reduction of Aqueous CO2 to CO
Abstract
The challenge in the electrochemical reduction of aqueous carbon dioxide is in designing a highly selective, energy‐efficient, and non‐precious‐metal electrocatalyst that minimizes the competitive reduction of proton to form hydrogen during aqueous CO 2 conversion. A non‐noble metal electrocatalyst based on a copper‐indium (Cu‐In) alloy that selectively converts CO 2 to CO with a low overpotential is reported. The electrochemical deposition of In on rough Cu surfaces led to Cu‐In alloy surfaces. DFT calculations showed that the In preferentially located on the edge sites rather than on the corner or flat sites and that the d‐electron nature of Cu remained almost intact, but adsorption properties of neighboring Cu was perturbed by the presence of In. This preparation of non‐noble metal alloy electrodes for the reduction of CO 2 provides guidelines for further improving electrocatalysis.
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Cites
New insights into the electrochemical reduction of carbon dioxide on metallic copper surfaces
Kuhl, K. P., Cave, E. R., Abram, D. N., & Jaramillo, T. F. (2012) · Energy & Environmental Science · doi:10.1039/c2ee21234j · Cited by 3,160
Hori, Y., Wakebe, H., Tsukamoto, T., & Koga, O. (1994) · Electrochimica Acta · doi:10.1016/0013-4686(94)85172-7 · Cited by 2,140
Li, C. W., & Kanan, M. W. (2012) · Journal of the American Chemical Society · doi:10.1021/ja3010978 · Cited by 2,000
Electroreduction of carbon monoxide to liquid fuel on oxide-derived nanocrystalline copper
Li, C. W., Ciston, J., & Kanan, M. W. (2014) · Nature · doi:10.1038/nature13249 · Cited by 1,728
Activity Descriptors for CO 2 Electroreduction to Methane on Transition-Metal Catalysts
Peterson, A. A., & Nørskov, J. K. (2012) · The Journal of Physical Chemistry Letters · doi:10.1021/jz201461p · Cited by 1,667
Kim, D., Resasco, J., Yu, Y., Asiri, A. M., & Yang, P. (2014) · Nature Communications · doi:10.1038/ncomms5948 · Cited by 1,374
Embedding Covalency into Metal Catalysts for Efficient Electrochemical Conversion of CO2
Lim, H.-K., Shin, H., Goddard, W. A., Hwang, Y. J., Min, B. K., & Kim, H. (2014) · Journal of the American Chemical Society · doi:10.1021/ja503782w · Cited by 222
Cited by
Progress and perspectives of electrochemical CO2 reduction on copper in aqueous electrolyte
Nitopi, S., Bertheussen, E., Scott, S. B., Liu, X., Engstfeld, A. K., Horch, S., Seger, B., Stephens, I. E. L., Chan, K., Hahn, C., et al. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00705 · Cited by 5,223
General Techno-Economic Analysis of CO 2 Electrolysis Systems
Jouny, M., Luc, W., & Jiao, F. (2018) · Industrial & Engineering Chemistry Research · doi:10.1021/acs.iecr.7b03514 · Cited by 1,628
Recent Advances in Inorganic Heterogeneous Electrocatalysts for Reduction of Carbon Dioxide
Zhu, D. D., Liu, J. L., & Qiao, S. Z. (2016) · Advanced Materials · doi:10.1002/adma.201504766 · Cited by 1,594
Zhang, L., Zhao, Z., & Gong, J. (2017) · Angewandte Chemie International Edition · doi:10.1002/anie.201612214 · Cited by 1,048
Understanding trends in electrochemical carbon dioxide reduction rates
Liu, X., Xiao, J., Peng, H., Hong, X., Chan, K., & Nørskov, J. K. (2017) · Nature Communications · doi:10.1038/ncomms15438 · Cited by 804
Metadata
- Authors
- Rasul, S., Anjum, D. H., Jedidi, A., Minenkov, Y., Cavallo, L., & Takanabe, K.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2014-12-23
- Volume
- 54
- Issue
- 7
- Pages
- 2146-2150
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2128158452
- Cited by
- 510
- References
- 7
- FWCI
- 12.55
- Type
- journal article
- Language
- en
- Open access
- closed
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- Rasul, S., Anjum, D. H., Jedidi, A., Minenkov, Y., Cavallo, L., & Takanabe, K. (2015). A Highly Selective Copper–Indium Bimetallic Electrocatalyst for the Electrochemical Reduction of Aqueous CO2 to CO. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201410233
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