The DOI matches its Crossref record; 8 of the 8 references it cites were found in a registry or an index.
Single Atom Bi Decorated Copper Alloy Enables C−C Coupling for Electrocatalytic Reduction of CO2 into C2+ Products**
Abstract
Single atom alloy (SAA) catalysts have been recently explored for promotion of various heterogeneous catalysis, but it remains unexplored for selective electrocatalytic reduction of carbon dioxide (CO 2) into multi‐carbon (C 2+) products involving C−C coupling. Herein we report a single‐atomic Bi decorated Cu alloy (denoted as BiCu‐SAA) electrocatalyst that could effectively modulate selectivity of CO 2 reduction into C 2+ products instead of previous C 1 ones. The BiCu‐SAA catalyst exhibits remarkably superior selectivity of C 2+ products with optimal Faradaic efficiency (FE) of 73.4 % compared to the pure copper nanoparticle or Bi nanoparticles‐decorated Cu nanocomposites, and its structure and performance can be well maintained at current density of 400 mA cm−2 under the flow cell system. Based on our in situ characterizations and density functional theory calculations, the BiCu‐SAA is found to favor the activation of CO 2 and subsequent C−C coupling during the electrocatalytic reaction, as should be responsible for its extraordinary C 2+ selectivity.
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Cites
Progress and perspectives of electrochemical CO2 reduction on copper in aqueous electrolyte
Nitopi, S., Bertheussen, E., Scott, S. B., Liu, X., Engstfeld, A. K., Horch, S., Seger, B., Stephens, I. E. L., Chan, K., Hahn, C., et al. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00705 · Cited by 5,223
Advances and challenges in understanding the electrocatalytic conversion of carbon dioxide to fuels
Birdja, Y. Y., Pérez-Gallent, E., Figueiredo, M. C., Göttle, A. J., Calle-Vallejo, F., & Koper, M. T. M. (2019) · Nature Energy · doi:10.1038/s41560-019-0450-y · Cited by 2,747
CO 2 electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface
Dinh, C.-T., Burdyny, T., Kibria, M. G., Seifitokaldani, A., Gabardo, C. M., García de Arquer, F. P., Kiani, A., Edwards, J. P., De Luna, P., Bushuyev, O. S., et al. (2018) · Science · doi:10.1126/science.aas9100 · Cited by 2,515
Electrocatalytic Conversion of Carbon Dioxide to Methane and Methanol on Transition Metal Surfaces
Kuhl, K. P., Hatsukade, T., Cave, E. R., Abram, D. N., Kibsgaard, J., & Jaramillo, T. F. (2014) · Journal of the American Chemical Society · doi:10.1021/ja505791r · Cited by 1,649
What Should We Make with CO2 and How Can We Make It?
Bushuyev, O. S., De Luna, P., Dinh, C. T., Tao, L., Saur, G., van de Lagemaat, J., Kelley, S. O., & Sargent, E. H. (2018) · Joule · doi:10.1016/j.joule.2017.09.003 · Cited by 1,593
CO 2 electrolysis to multicarbon products in strong acid
Huang, J. E., Li, F., Ozden, A., Sedighian Rasouli, A., García de Arquer, F. P., Liu, S., Zhang, S., Luo, M., Wang, X., Lum, Y., et al. (2021) · Science · doi:10.1126/science.abg6582 · Cited by 1,359
Long, R., Li, Y., Liu, Y., Chen, S., Zheng, X., Gao, C., He, C., Chen, N., Qi, Z., Song, L., et al. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.7b00452 · Cited by 571
Self-citationGao, L., Li, X., Yao, Z., Bai, H., Lu, Y., Ma, C., Lu, S., Peng, Z., Yang, J., Pan, A., et al. (2019) · Journal of the American Chemical Society · doi:10.1021/jacs.9b07238 · Cited by 376
Cited by
Jiang, M., Wang, H., Zhu, M., Luo, X., He, Y., Wang, M., Wu, C., Zhang, L., Li, X., Liao, X., et al. (2024) · Chemical Society Reviews · doi:10.1039/d3cs00857f · Cited by 299
Fan, X., Chen, W., Xie, L., Liu, X., Ding, Y., Zhang, L., Tang, M., Liao, Y., Yang, Q., Fu, X., et al. (2024) · Advanced Materials · doi:10.1002/adma.202313179 · Cited by 89
Metadata
- Authors
- Cao, Y., Chen, S., Bo, S., Fan, W., Li, J., Jia, C., Zhou, Z., Liu, Q., Zheng, L., & Zhang, F.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2023-06-16
- Volume
- 62
- Issue
- 30
- Pages
- e202303048-e202303048
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W4378746109
- Cited by
- 194
- References
- 8
- FWCI
- 9.08
- Type
- journal article
- Language
- en
- Open access
- closed
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- The paper
- Cao, Y., Chen, S., Bo, S., Fan, W., Li, J., Jia, C., Zhou, Z., Liu, Q., Zheng, L., & Zhang, F. (2023). Single Atom Bi Decorated Copper Alloy Enables C−C Coupling for Electrocatalytic Reduction of CO2 into C2+ Products**. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.202303048
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