Trace element content of sedimentary pyrite as a new proxy for deep-time ocean–atmosphere evolution
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Archean marine sediments have low concentrations of elements that enter rivers during oxidative continental weathering.
“Furthermore, Archean marine sediments have low concentrations of elements that enter rivers during oxidative continental weathering (68–70).”
From The Archean atmosphere (2020) · cites this paper as [69]
Under more oxic conditions first observed in the Cryogenian and continuing into the Cambrian-Ordovician, models indicated Fe and Mn concentrations in seawater would have been drawn down to modern levels by oxide mineral precipitation.
“Under more oxic conditions first observed in the Cryogenian and continuing to develop into the Cambrian-Ordovician (Large et al., 2014;Sperling et al., 2015;Sahoo et al., 2016), the models of Saito et al. (2003) indicated that Fe and Mn concentrations in seawater would have been drawn down to modern levels as the result of oxide mineral precipitation.”
From Trace elements at the intersection of marine biological and geochemical evolution (2016) · cites this paper as Large et al., 2014
Assessments of pyrite versus matrix incorporation, sulfide recrystallization, and formation site, plus further studies, indicate that the pyrite record can preserve seawater signatures.
“Large et al. (2014) also provided an assessment of the importance of pyrite versus matrix trace element incorporation, sulfide recrystallization, and the location in the water column or sediment where pyrite forms, which suggest the record is favorable to recording seawater signatures; a result further supported by several additional studies (Gregory et al., 2014;Large et al., 2015;Mukherjee and”
From Trace elements at the intersection of marine biological and geochemical evolution (2016) · cites this paper as Large et al., 2014
Pyrite may form at deposition or during early diagenesis and can take up trace element signatures typical of seawater.
“Pyrite (FeS2) can form in sediments contemporaneous with deposition or during early diagenesis, and it may therefore incorporate trace element signatures characteristic of seawater (see Large et al., 2014).”
From Trace elements at the intersection of marine biological and geochemical evolution (2016) · cites this paper as Large et al., 2014
Large et al. presented Ni analyses in sedimentary to early diagenetic pyrite that mirrored the temporal trend in Ni/Fe ratios observed in iron formations.
“Large et al. (2014) presented a suite of Ni analyses in sedimentary to early diagenetic pyrite that mirrored the observed temporal trend in Ni/Fe ratios observed in IF.”
From Trace elements at the intersection of marine biological and geochemical evolution (2016) · cites this paper as Large et al., 2014
First-order trends in Ni abundances in the iron formation record are also recorded in sedimentary pyrite.
“Interestingly, the first-order trends in Ni abundances observed in the IF record (Fig. 6) are also recorded in sedimentary pyrite.”
From Trace elements at the intersection of marine biological and geochemical evolution (2016) · cites this paper as Large et al., 2014
High Ni and Co values in Late Permian pyrites support the assertion that Ni and Co may be associated with Siberian traps volcanism and the Permian mass extinction.
“An observation that supports this assertion is the high Ni and Co values observed in pyrites in the Late Permian (Large et al., 2014), in which case the Ni and Co may be associated with the Siberian traps volcanism and Permian mass extinction”
From Trace elements at the intersection of marine biological and geochemical evolution (2016) · cites this paper as Large et al., 2014
Large et al. noted a correlation between Ni and Co in the pyrite record and suggested it may be tied to the emplacement and subsequent erosion of large igneous provinces.
“Large et al. (2014) further noted a correlation between Ni and Co in the pyrite record, and suggested that this may be tied to the emplacement and subsequent erosion of large igneous provinces.”
From Trace elements at the intersection of marine biological and geochemical evolution (2016) · cites this paper as Large et al., 2014
The syngenetic and early diagenetic pyrite record for Co indicates a steadier decline in Co levels from 3 Ga to present.
“However, the syngenetic and early diagenetic pyrite record for Co presented by Large et al. (2014) indicates a steadier decline in Co levels from 3 Ga to present.”
From Trace elements at the intersection of marine biological and geochemical evolution (2016) · cites this paper as Large et al., 2014
They argued that Cr should be sourced from ultramafic rocks similar to Ni and Co, and that the decrease may reflect a decrease in the abundance of the source.
“They argued that Cr should be sourced from ultramafic rocks similar to Ni and Co, and that this decrease may reflect a decrease in the abundance of the source”
From Trace elements at the intersection of marine biological and geochemical evolution (2016) · cites this paper as Large et al., 2014
Large et al. attributed the decrease in Cr concentrations from the Archean to the Proterozoic to a change in source availability.
“Large et al. (2014) attributed a decrease in Cr concentrations, from the Archean to the Proterozoic (Fig. 9), as reflective of a change in source availability.”
From Trace elements at the intersection of marine biological and geochemical evolution (2016) · cites this paper as Large et al., 2014
Large et al. found patterns in Cr and Mo concentrations in sedimentary pyrite consistent with dominance of anoxic settings in the Proterozoic from 2.15 to 0.7 Ga, with euxinic settings more prevalent between 1.2 and 0.8 Ga.
“Large et al. (2014) also investigated Cr and Mo concentrations in sedimentary pyrite and found patterns consistent with the dominance of anoxic settings in the Proterozoic from 2.15 to 0.7 Ga, with euxinic settings more prevalent between 1.2 and 0.8 Ga.”
From Trace elements at the intersection of marine biological and geochemical evolution (2016) · cites this paper as Large et al., 2014
Large et al. attribute this Mesoproterozoic U rise to enhanced oxidative weathering of U-rich granites.
“They attribute this rise to enhanced oxidative weathering of U-rich granites.”
From Trace elements at the intersection of marine biological and geochemical evolution (2016) · cites this paper as Large et al., 2014
Large et al. showed a temporal trend in Se with small peaks at 3.0 and 2.4 Ga, a Paleoproterozoic to Mesoproterozoic perturbation between 1800-1300 Ma, and a rise in the Neoproterozoic to Phanerozoic.
“In their analyses of syngenetic and early diagenetic pyrite, Large et al. (2014) showed a temporal trend in Se with several small peaks at 3.0 and 2.4 Ga, along with a Paleoproterozoic to Mesoproterozoic perturbation between 1800-1300 Ma, and finally a rise in the Neoproterozoic to Phanerozoic.”
From Trace elements at the intersection of marine biological and geochemical evolution (2016) · cites this paper as Large et al., 2014
Large et al. suggested this Se trend may be used as a paleoproxy for tracking oxygenation.
“Large et al. (2014) further suggested that this trend in Se may be used as a paleoproxy for tracking oxygenation.”
From Trace elements at the intersection of marine biological and geochemical evolution (2016) · cites this paper as Large et al., 2014
Laser ablation analyses of black shale matrices show an increase in U during the Mesoproterozoic, with a peak between 1.4 and 1.7 Ga.
“laser ablation analyses of black shale matrices by Large et al. (2014) seem to show an increase in U during the Mesoproterozoic, with a peak between 1.4 to 1.7 Ga”
From Trace elements at the intersection of marine biological and geochemical evolution (2016) · cites this paper as Large et al., 2014
The black shale record for V mirrors that of Mo and is relatively consistent with Neoproterozoic enrichments in the pyrite record.
“Overall, it appears that the black shale record for V mirrors that of Mo, and is relatively consistent with Neoproterozoic enrichments seen in the pyrite record (Large et al., 2014).”
From Trace elements at the intersection of marine biological and geochemical evolution (2016) · cites this paper as Large et al., 2014
A similar trend is observed in the pyrite record, but some Phanerozoic variability in the pyrite record is not present in the IF record.
“A similar trend is observed in the pyrtie record as presented by Large et al. (2014), however, some variability in the Phanerozoic is observed in the pyrite record that is not present in the IF record.”
From Trace elements at the intersection of marine biological and geochemical evolution (2016) · cites this paper as Large et al. (2014)
The chromium decline resembles the shale matrix record reported by Large et al. (2014).
“similar to the shale matrix record of Large et al. (2014)”
From Trace elements at the intersection of marine biological and geochemical evolution (2016) · cites this paper as Large et al. (2014)
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Mukherjee, I., Large, R. R., Bull, S. W., Gregory, D., Stepanov, A. S., Ávila, J. N., Ireland, T. R., & Corkrey, R. (2019) · American Mineralogist · doi:10.2138/am-2019-6873 · Cited by 41 · see citing works
Self-citationMachine learning coupled with mineral geochemistry reveals the origin of ore deposits
Sun, G., Zeng, Q., & Zhou, J. (2022) · Ore Geology Reviews · doi:10.1016/j.oregeorev.2022.104753 · Cited by 40 · see citing works
- Authors
- Large, R. R., Halpin, J. A., Danyushevsky, L. V., Maslennikov, V. V., Bull, S. W., Long, J. A., Gregory, D. D., Lounejeva, E., Lyons, T. W., Sack, P. J., McGoldrick, P. J., & Calver, C. R.
- Affiliations
- University of Tasmania (AU)
- Flinders University (AU)
- University of California, Riverside (US)
- Yukon Geological Survey (CA)
- Corresponding author
- Large, Ross R.
- ORCID
- Venue
- Earth and Planetary Science Letters
- Publisher
- Elsevier BV
- Published
- 2014-03
- Volume
- 389
- Pages
- 209-220
- ISSN
- 0012-821X (ISSN-L)
- OpenAlex
- W1969023317
- Cited by
- 545
- References
- 71
- Citations by year
- 2026: 46 · 2025: 59 · 2024: 45 · 2023: 56 · 2022: 54 · 2021: 47 · 2020: 66 · 2019: 45 · 2018: 39 · 2017: 36 · 2016: 18 · 2015: 26 · 2014: 8
- FWCI
- 19.65
- Type
- journal article
- Language
- en
- Open access
- green
- figshare.com
- Licence
- Locations
- Earth and Planetary Science Letters (publishedVersion)
- eCite Digital Repository (University of Tasmania) (submittedVersion)
- Figshare (submittedVersion, cc-by)
- Funders
- ARC Centre of Excellence (CE0561595)
- AMIRA (P923)
- Topics
- Physical Sciences › Earth and Planetary Sciences › Paleontology › Paleontology and Stratigraphy of Fossils
- Physical Sciences › Earth and Planetary Sciences › Geochemistry and Petrology › Geochemistry and Elemental Analysis
- Physical Sciences › Earth and Planetary Sciences › Geophysics › Geological and Geochemical Analysis
- Keywords
- sedimentary pyrite, trace elements, black shales, seawater chemistry, Great Oxidation Event, ocean anoxia, large igneous provinces, continental erosion, Precambrian, Proterozoic, Archean, seawater nutrients, selenium, molybdenum, uranium, nickel, cobalt, Cryogenian, paleo-oxygenation
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