Cited by 143Membrane Separation TechnologiesArsenic contamination and mitigationMembrane-based Ion Separation Techniques

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Experimental study of arsenic removal by direct contact membrane distillation

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Qu, Dan, Wang, Jun, Hou, Deyin, Luan, Zhaokun, Fan, Bin, Zhao, Changwei·2009·Journal of Hazardous Materials

DOI 10.1016/j.jhazmat.2008.07.042

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Abstract

Arsenite (As(III)) and arsenate (As(V)) removal by direct contact membrane distillation (DCMD) were investigated with self-made polyvinylidene fluoride (PVDF) membranes in the present work. Permeability and ion rejection efficiency of the membrane were tested before the arsenic removal experiments. A maximum permeate flux 20.90 kg/m(2)h was obtained, and due to the hydrophobic property, the PVDF membrane had high rejection of inorganic anions and cations which was independent of the solution pH and the temperature. The experimental results indicated that DCMD process had higher removal efficiency of arsenic than pressure-driven membrane processes, especially for high-concentration arsenic and arsenite removal. The experimental results indicated that the permeate As(III) and As(V) were under the maximum contaminant limit (10 microg/L) until the feed As(III) and As(V) achieved 40 and 2000 mg/L, respectively. The 250 h simultaneous DCMD performance of 0.5mg/L As(III) and As(V) solution was carried out, respectively. The permeate arsenic was not detected during the process which showed the PVDF membrane had stable arsenic removal efficiency. Membrane morphology changed slightly after the experiments, however, the permeability and the ion rejection of the membrane did not change.

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Authors: Qu, D., Wang, J., Hou, D., Luan, Z., Fan, B., & Zhao, C.
Affiliations: Chinese Academy of Sciences (CN)
Corresponding author: Luan, Zhaokun
ORCID: Qu, Dan
Wang, Jun
Hou, Deyin
Zhao, Changwei
Venue: Journal of Hazardous Materials
Publisher: Elsevier BV
Published: 2009-04
Volume: 163
Issue: 2-3
Pages: 874-879
ISSN: 0304-3894 (ISSN-L)
DOI: 10.1016/j.jhazmat.2008.07.042
OpenAlex: W2018723048
Cited by: 143
References: 27
Citations by year: 2026: 3 · 2025: 6 · 2024: 18 · 2023: 2 · 2022: 6 · 2021: 9 · 2020: 12 · 2019: 7 · 2018: 14 · 2017: 9 · 2016: 9 · 2015: 10 · 2014: 8 · 2013: 9 · 2012: 4
FWCI: 6.22
Type: journal article
Language: en
Open access: green
ir.rcees.ac.cn
Licence: cc-by-nc-nd
www.elsevier.com/tdm/userlicense/1.0/ (tdm)
Locations: Journal of Hazardous Materials (publishedVersion)
PubMed (publishedVersion)
Research Center for Eco-Environmental Sciences OpenIR (Chinese Academy of Sciences) (submittedVersion, cc-by-nc-nd)
Topics: Physical Sciences › Environmental Science › Water Science and Technology › Membrane Separation Technologies
Physical Sciences › Environmental Science › Environmental Chemistry › Arsenic contamination and mitigation
Physical Sciences › Chemical Engineering › Filtration and Separation › Membrane-based Ion Separation Techniques
Keywords: arsenic removal, direct contact membrane distillation, arsenite, arsenate, PVDF membranes, ion rejection, permeate flux, hydrophobic membranes, arsenic removal efficiency, membrane stability
MeSH terms: Arsenic, Filtration, Fluorocarbon Polymers, Ions, Membranes, Artificial, Permeability, Polyvinyls, Water Pollutants, Chemical, Arsenites

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Experimental study of arsenic removal by direct contact membrane distillation

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