The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
A low-toxicity and high-efficiency deep eutectic solvent for the separation of aluminum foil and cathode materials from spent lithium-ion batteries
Abstract
The separation of cathode materials from aluminum (Al) foil is a key issue worthy of attention in the process of resource utilization of spent lithium-ion batteries (LIBs). Traditional technologies for the Al foil and cathode materials separation have the disadvantages of the use of corrosive acid/alkali, release of HF hazards, and environment and healthy risks of the toxicity reagent. In this study, a low-toxicity, high-efficiency, and low-cost deep eutectic solvent (DES), choline chloride-glycerol, was synthesized and applied to solving the separation dilemma of Al foil and cathode materials in spent LIBs. The experimental results show that separation of the Al foil and cathode materials can be achieved under optimal conditions designed by the response surface method: heating temperature 190 ℃, choline chloride: glycerol molar ratio 2.3:1, and heating time 15.0 min; the peeling percentage of cathode material can reach 99.86 wt%. Mechanism analysis results confirm that the separation of Al foil and cathode materials was the result of the deactivation of the organic binder polyvinylidene fluoride (PVDF), which can be attributed to an alkali degradation process caused by the attack of the hydroxide of choline chloride on the acidic hydrogen atom in PVDF.
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Cites
Deep Eutectic Solvents (DESs) and Their Applications
Smith, E. L., Abbott, A. P., & Ryder, K. S. (2014) · Chemical Reviews · doi:10.1021/cr300162p · Cited by 7,378
Deep eutectic solvents: syntheses, properties and applications
Zhang, Q., De Oliveira Vigier, K., Royer, S., & Jérôme, F. (2012) · Chemical Society Reviews · doi:10.1039/c2cs35178a · Cited by 4,899
Toward sustainable and systematic recycling of spent rechargeable batteries
Zhang, X., Li, L., Fan, E., Xue, Q., Bian, Y., Wu, F., & Chen, R. (2018) · Chemical Society Reviews · doi:10.1039/c8cs00297e · Cited by 1,038
Evaluation of toxicity and biodegradability of choline chloride based deep eutectic solvents
Radošević, K., Cvjetko Bubalo, M., Gaurina Srček, V., Grgas, D., Landeka Dragičević, T., & Radojčić Redovniković, I. (2015) · Ecotoxicology and Environmental Safety · doi:10.1016/j.ecoenv.2014.09.034 · Cited by 770
Lithium market research – global supply, future demand and price development
Martin, G., Rentsch, L., Höck, M., & Bertau, M. (2017) · Energy Storage Materials · doi:10.1016/j.ensm.2016.11.004 · Cited by 740
Cited by
Neumann, J., Petranikova, M., Meeus, M., Gamarra, J. D., Younesi, R., Winter, M., & Nowak, S. (2022) · Advanced Energy Materials · doi:10.1002/aenm.202102917 · Cited by 805
Progresses in Sustainable Recycling Technology of Spent Lithium‐Ion Batteries
Du, K., Ang, E. H., Wu, X., & Liu, Y. (2022) · ENERGY & ENVIRONMENTAL MATERIALS · doi:10.1002/eem2.12271 · Cited by 458
Wu, J., Liang, Q., Yu, X., Lü, Q., Ma, L., Qin, X., Chen, G., & Li, B. (2021) · Advanced Functional Materials · doi:10.1002/adfm.202011102 · Cited by 447
The 2021 battery technology roadmap
Ma, J., Li, Y., Grundish, N. S., Goodenough, J. B., Chen, Y., Guo, L., Peng, Z., Qi, X., Yang, F., Qie, L., et al. (2021) · Journal of Physics D: Applied Physics · doi:10.1088/1361-6463/abd353 · Cited by 269
Rensmo, A., Savvidou, E. K., Cousins, I. T., Hu, X., Schellenberger, S., & Benskin, J. P. (2023) · Environmental Science: Processes & Impacts · doi:10.1039/d2em00511e · Cited by 123
Metadata
- Authors
- Wang, M., Tan, Q., Liu, L., & Li, J.
- Venue
- Journal of Hazardous Materials
- Publisher
- Elsevier BV
- Published
- 2019-12
- Volume
- 380
- Pages
- 120846
- ISSN
- 0304-3894 (ISSN-L)
- OpenAlex
- W2954923082
- Cited by
- 230
- References
- 5
- FWCI
- 10.75
- Type
- journal article
- Language
- en
- Open access
- closed
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- Wang, M., Tan, Q., Liu, L., & Li, J. (2019). A low-toxicity and high-efficiency deep eutectic solvent for the separation of aluminum foil and cathode materials from spent lithium-ion batteries. Journal of Hazardous Materials. https://doi.org/10.1016/j.jhazmat.2019.120846
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