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Cited by 616Polymer Surface Interaction StudiesAdvanced Polymer Synthesis and CharacterizationEpoxy Resin Curing Processes

Catechols as versatile platforms in polymer chemistry

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Faure, Emilie, Falentin-Daudré, Céline, Jérôme, Christine, Lyskawa, Joël, Fournier, David, Woisel, Patrice, Detrembleur, Christophe·2013·Progress in Polymer Science
DOI 10.1016/j.progpolymsci.2012.06.004
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  • Using classic organic reactions, the catechol group has been successfully incorporated into a series of natural polymers, such as PL, HA, chitosan, SA, and gelatin, and synthetic polymers, such as PEG-based polymers.

    “Using these classic organic reactions, the catechol group has been successfully incorporated into a series of natural polymers, such as PL, HA, chitosan, SA, and gelatin (GT), and synthetic polymers, such as polyethylene glycol (PEG)-based polymers [45,47,51,52,53,54,55].”

    From Mussel-Inspired Injectable Adhesive Hydrogels for Biomedical Applications (2024) · cites this paper as [47]

    Section 3.3.3 describes catechol grafting onto hyaluronic acid, poly(L-lysine), and chitosan; section 3.3.4 describes modification of gelatin and PEG-based polymers. I found no passage supporting the listed SA example (searched for alginate), so the full list is not supported by this source. (LLM, conf=0.83)

    Experimental — accuracy not yet measured

  • Many methods have been developed to incorporate the catechol group into polymers, including incorporation by classic organic reactions, polymerization of catechol-based monomers, and biosynthesis of catechol-containing proteins.

    “During recent decades, many methods have been developed to incorporate the catechol group into polymers [4,47], including the incorporation of the catechol group by classic organic reactions, polymerization of catechol-based monomers, and biosynthesis of catechol-containing proteins (Figure 3).”

    From Mussel-Inspired Injectable Adhesive Hydrogels for Biomedical Applications (2024) · cites this paper as [47]

    Sections 3.3 and 3.1 describe chemical incorporation of catechols into preformed polymers and polymerization of catechol-bearing monomers. The Introduction describes naturally occurring DOPA-containing mussel proteins, but the passages do not describe biosynthesis of catechol-containing proteins as a developed method for incorporating catechols into polymers. (LLM, conf=0.84)

    Experimental — accuracy not yet measured

  • The catechol group's radical-scavenging capacity makes mussel-inspired hydrogels suitable for eliminating ROS in wound healing.

    “On the one hand, this makes the mussel-inspired hydrogel suitable for eliminating ROS in the wound healing process.”

    From Mussel-Inspired Injectable Adhesive Hydrogels for Biomedical Applications (2024) · cites this paper as [47]

    Section 2.2 reports radical-scavenging activity for poly(catechin), and section 3.3.4 describes mussel-inspired catechol hydrogels used as tissue sealants. Neither passage establishes that those hydrogels eliminate ROS or are suitable for wound healing on that basis. (LLM, conf=0.83)

    Experimental — accuracy not yet measured

  • Commonly, catechol is protected before polymerization.

    “Therefore, commonly, catechol is protected before polymerization [47].”

    From Mussel-Inspired Injectable Adhesive Hydrogels for Biomedical Applications (2024) · cites this paper as [47]

  • The catechol group is a polymerization inhibitor that can react with free radicals.

    “Second, the catechol group is a polymerization inhibitor with the capacity to react with free radicals [47].”

    From Mussel-Inspired Injectable Adhesive Hydrogels for Biomedical Applications (2024) · cites this paper as [47]

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Authors
Faure, E., Falentin-Daudré, C., Jérôme, C., Lyskawa, J., Fournier, D., Woisel, P., & Detrembleur, C.
Affiliations
  • University of Liège (BE)
  • Unité Matériaux et Transformations (FR)
  • École Nationale Supérieure de Chimie de Lille (FR)
Corresponding author
  • Woisel, Patrice
  • Detrembleur, Christophe
ORCID
Venue
Progress in Polymer Science
Publisher
Elsevier BV
Published
2013-01
Volume
38
Issue
1
Pages
236-270
ISSN
0079-6700 (ISSN-L)
DOI
10.1016/j.progpolymsci.2012.06.004
OpenAlex
W2134995275
Cited by
616
References
0
Citations by year
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FWCI
14.98
Type
journal article
Language
en
Open access
Licence
www.elsevier.com/tdm/userlicense/1.0/ (tdm)
Locations
  • Progress in Polymer Science (publishedVersion)
  • ORBi (University of Liège) (submittedVersion, other-oa)
Funders
  • Waalse Gewest
  • Fonds De La Recherche Scientifique - FNRS
  • Belgian Federal Science Policy Office
Topics
  • Physical Sciences › Materials Science › Surfaces, Coatings and Films › Polymer Surface Interaction Studies
  • Physical Sciences › Chemistry › Organic Chemistry › Advanced Polymer Synthesis and Characterization
  • Physical Sciences › Engineering › Mechanical Engineering › Epoxy Resin Curing Processes
Keywords
catechol, mussel-inspired adhesives, synthetic adhesives, surface coating, surface modification, anchoring groups, pendant groups, end-functionalized polymers, polymer synthesis

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