The DOI matches its Crossref record; 31 of the 31 references it cites were found in a registry or an index.
A process for combination of recycling lithium and regenerating graphite from spent lithium-ion battery
Abstract
Recycling lithium and graphite from spent lithium-ion battery plays a significant role in mitigation of lithium resources shortage, comprehensive utilization of spent anode graphite and environmental protection. In this study, spent graphite was firstly collected by a two-stage calcination. Secondly, under the optimal conditions of 1.5 M HCI, 60 min and solid-liquid ratio (S/L) of 100 g·L-1, the collected graphite suffers simple acid leaching to make almost 100% lithium, copper and aluminum in it into leach liquor. Thirdly, 99.9% aluminum and 99.9% copper were removed from leach liquor by adjusting pH first to 7 and then to 9, and thenthe lithium was recovered by adding sodium carbonate in leach liquor to form lithium carbonate with high purity (>99%). The regenerated graphite is found to have high initial specific capacity at the rate of 37.2 mA·g-1 (591 mAh·g-1), 74.4 mA·g-1 (510 mAh·g-1) and 186 mA·g-1 (335 mAh·g-1), and with the high retention ratio of 97.9% after 100 cycles, it also displays excellent cycle performance at high rate of 372 mA·g-1. By this process, copper and lithium can be recovered and graphite can be regenerated, serving as a sustainable approach for the comprehensive utilization of anode material from spent lithium-ion battery.
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Cited by
Neumann, J., Petranikova, M., Meeus, M., Gamarra, J. D., Younesi, R., Winter, M., & Nowak, S. (2022) · Advanced Energy Materials · doi:10.1002/aenm.202102917 · Cited by 805
Nižetić, S., Djilali, N., Papadopoulos, A., & Rodrigues, J. J. P. C. (2019) · Journal of Cleaner Production · doi:10.1016/j.jclepro.2019.04.397 · Cited by 538
Technologies of lithium recycling from waste lithium ion batteries: a review
Bae, H., & Kim, Y. (2021) · Materials Advances · doi:10.1039/d1ma00216c · Cited by 428
Recent progress on the recycling technology of Li-ion batteries
Wang, Y., An, N., Wen, L., Wang, L., Jiang, X., Hou, F., Yin, Y., & Liang, J. (2021) · Journal of Energy Chemistry · doi:10.1016/j.jechem.2020.05.008 · Cited by 404
A review on the recycling of spent lithium-ion batteries (LIBs) by the bioleaching approach
Roy, J. J., Cao, B., & Madhavi, S. (2021) · Chemosphere · doi:10.1016/j.chemosphere.2021.130944 · Cited by 346
Metadata
- Authors
- Yang, Y., Song, S., Lei, S., Sun, W., Hou, H., Jiang, F., Ji, X., Zhao, W., & Hu, Y.
- Venue
- Waste Management
- Publisher
- Elsevier BV
- Published
- 2019-02
- Volume
- 85
- Pages
- 529-537
- ISSN
- 0956-053X (ISSN-L)
- OpenAlex
- W2913698145
- Cited by
- 309
- References
- 31
- FWCI
- 16.75
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yang, Y., Song, S., Lei, S., Sun, W., Hou, H., Jiang, F., Ji, X., Zhao, W., & Hu, Y. (2019). A process for combination of recycling lithium and regenerating graphite from spent lithium-ion battery. Waste Management. https://doi.org/10.1016/j.wasman.2019.01.008
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