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Recent Advances of Structurally Ordered Intermetallic Nanoparticles for Electrocatalysis

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Xiao, Weiping, Lei, Wen, Gong, Mingxing, Xin, Huolin L., Wang, Deli·2018·ACS Catalysis
DOI 10.1021/acscatal.7b04420
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Abstract

Structurally ordered intermetallic phases have exhibited higher and higher electrocatalytic activity and stability than disordered alloys in many reactions such as the oxygen reduction reaction (ORR) and small-molecule (hydrogen, formic acid, or ethanol) oxidation reactions. The enhanced electrocatalytic activity could be derived from the definite composition and predictable control over structural, geometric, and electronic effects. This review, based on the understanding of the catalytic mechanism of structurally ordered intermetallic nanoparticles, provides a comprehensive acknowledgment of how the particle size and morphology affect the catalytic performance. The strategy for reducing particle size and the impact of particle size on electrocatalysis will be first introduced. Then, recent developments in the synthesis and design of morphology-controlled catalysts are summarized. The structure–activity relationship between the catalytic activity and morphology including core–shell/hollow and porosity will be highlighted. Finally, the current challenges and future developments are provided. On the basis of this review, intermetallic nanoparticles will shed light on the future development of electrocatalysts for fuel cells and metal-air batteries.

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Authors
Xiao, W., Lei, W., Gong, M., Xin, H. L., & Wang, D.
Affiliations
  • Huazhong University of Science and Technology (CN)
  • Brookhaven National Laboratory (US)
Corresponding author
Wang, Deli
ORCID
Venue
ACS Catalysis
Publisher
American Chemical Society (ACS)
Published
2018-03-06
Volume
8
Issue
4
Pages
3237-3256
ISSN
2155-5435 (ISSN-L)
DOI
10.1021/acscatal.7b04420
OpenAlex
W2793644897
Cited by
356
References
182
Citations by year
2026: 25 · 2025: 44 · 2024: 46 · 2023: 44 · 2022: 39 · 2021: 58 · 2020: 57 · 2019: 38 · 2018: 5
FWCI
9.13
Type
journal article
Language
en
Open access
Locations
  • ACS Catalysis (publishedVersion)
  • OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
Funders
  • Basic Energy Sciences (DE-SC0012704)
  • National Natural Science Foundation of China (21573083)
  • Central People's Government of the People's Republic of China
Topics
  • Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
  • Physical Sciences › Materials Science › Materials Chemistry › Catalytic Processes in Materials Science
  • Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
Keywords
intermetallic nanoparticles, electrocatalysis, oxygen reduction reaction, hydrogen oxidation, formic acid oxidation, ethanol oxidation, particle size effects, morphology control, core-shell nanoparticles, hollow nanoparticles, porosity, structure-activity relationship, fuel cells, metal-air batteries

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