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Dopamine-Triggered Hydrogels with High Transparency, Self-Adhesion, and Thermoresponse as Skinlike Sensors
Abstract
Mussel-inspired conductive hydrogels are attractive for the development of next-generation self-adhesive, flexible skinlike sensors. However, despite extensive progress, there are still some daunting challenges that hinder their applications, such as inferior optical transparency, low catechol content ( e.g., poor adhesion), as well as limited sensation performances. Here, we report a dopamine-triggered gelation (DTG) strategy for fabricating mussel-inspired, transparent, and conductive hydrogels. The DTG design leverages on the dual functions of dopamine, which serves as both polymerization initiator and dynamic mediator to elaborate and orchestrate the cross-linking networks of hydrogels, allowing for pronounced adhesion, robust elasticity, self-healing ability, excellent injectability and three-dimensional printability, reversible and tunable transparent-opaque transition, and thermoresponsive feature. These preferable performances enable DTG hydrogels as self-adhesive, flexible skinlike sensors for achieving multiple sensations toward pressure, strain, and temperature, even an extraordinary visual perception effect, making it a step closer in the exploration of future biomimetic skin.
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Metadata
- Authors
- Zhang, C., Zhou, Y., Han, H., Zheng, H., Xu, W., & Wang, Z.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2021-01-06
- Volume
- 15
- Issue
- 1
- Pages
- 1785-1794
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W3118899852
- Cited by
- 316
- References
- 40
- FWCI
- 16.15
- Type
- journal article
- Language
- en
- Open access
- closed
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