The DOI matches its Crossref record; 27 of the 27 references it cites were found in a registry or an index.
Fast and Slow Rates of Naphthalene Sorption to Biochars Produced at Different Temperatures
Abstract
This study investigated the sorption kinetics of a model solute (naphthalene) with a series of biochars prepared from a pine wood at 150-700 °C (referred as PW100-PW700) to probe the effect of the degree of carbonization of a biochar. The samples were characterized by the elemental compositions, thermal gravimetric analyses, Fourier transform IR spectroscopy, scanning electron microscopy, Brunauer-Emmett-Teller-N(2) surface areas (SA), and pore size distributions. Naphthalene exhibited a fast rate of sorption to PW150 owning a high oxygen content and a small SA, due supposedly to the solute partition into a swollen well-hydrated uncarbonized organic matter of PW150. The partial removal of polar-group contents in PW250/PW350, which increased the compactness of the partition medium, decreased the diffusion of the solute into the partition phase to result in a slow sorption rate. With PW500 and PW700 displaying low oxygen contents and high SA, the solute sorption rates were fast, attributed to the near exhaustion of a partition phase in the sample and to the fast solute adsorption on the carbonized biochar component. The results illustrate that the sorption rate of a solute with biochars is controlled largely by the solute's diffusivity in the biochar's partition phase, in which the medium compactness affects directly the solute diffusivity.
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Metadata
- Authors
- Chen, Z., Chen, B., & Chiou, C. T.
- Venue
- Environmental Science & Technology
- Publisher
- American Chemical Society (ACS)
- Published
- 2012-09-26
- Volume
- 46
- Issue
- 20
- Pages
- 11104-11111
- ISSN
- 0013-936X (ISSN-L)
- 1520-5851
- OpenAlex
- W2013118853
- Cited by
- 329
- References
- 27
- FWCI
- 13.08
- Type
- journal article
- Language
- en
- Open access
- closed
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