Catechol and Humic Acid Sorption onto a Range of Laboratory-Produced Black Carbons (Biochars)
Abstract
Although the major influence of black carbon (BC) on soil and sediment organic contaminant sorption is widely accepted, an understanding of the mechanisms and natural variation in pyrogenic carbon interaction with natural organic matter (NOM) is lacking. The sorption of a phenolic NOM monomer (catechol) and humic acids (HA) onto BC was examined using biochars made from oak, pine, and grass at 250, 400, and 650 degrees C. Catechol sorption equilibrium occurred after 14 d and was described by a diffusion kinetic model, while HA required only 1 d and followed pseudo-second-order kinetics. Catechol sorption capacity increased with increasing biochar combustion temperature, from pine < oak < grass and from coarse < fine particle size. At lower catechol concentrations, sorption affinity (Freundlich constant, K(f)) was directly related to micropore surface area (measured via CO(2) sorptometry) indicating the predominance of specific adsorption. In contrast, HA exhibited an order of magnitude less sorption (0.1% versus 1%, by weight) due to its exclusion from micropores. Greater sorption of both catechol and HA occurred on biochars with nanopores, i.e. biochars made at higher temperatures. These findings suggest that addition of BC to soil, via natural fires or biochar amendments, will sequester abundant native OM through sorption.
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Biochars with higher specific surface area (obtained at temperatures above 600 °C) have greater surface microporosity and increased CEC.
“other studies have found that biochars with higher specific surface area (obtained at temperatures above 600 °C) have greater surface microporosity and increased CEC”
From Biochar physicochemical properties: pyrolysis temperature and feedstock kind effects (2020) · cites this paper as Kasozi et al. 2010
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- Authors
- Kasozi, G. N., Zimmerman, A. R., Nkedi-Kizza, P., & Gao, B.
- Affiliations
- University of Florida (US)
- Department of Geological Sciences, University of Florida, 241 Williamson Hall, Gainesville, Florida 32611-2120, Department of Soil and Water Science, University of Florida, Gainesville, Florida, and Department of Agricultural and Biological Engineering, University of Florida, Gainesville, Florida
- Corresponding author
- Zimmerman, Andrew R.
- Venue
- Environmental Science & Technology
- Publisher
- American Chemical Society (ACS)
- Published
- 2010-07-29
- Volume
- 44
- Issue
- 16
- Pages
- 6189-6195
- ISSN
- 0013-936X (ISSN-L)
- 1520-5851
- OpenAlex
- W2081147875
- Cited by
- 509
- References
- 51
- Citations by year
- 2026: 21 · 2025: 25 · 2024: 29 · 2023: 49 · 2022: 40 · 2021: 52 · 2020: 48 · 2019: 26 · 2018: 30 · 2017: 43 · 2016: 31 · 2015: 38 · 2014: 32 · 2013: 23 · 2012: 11
- FWCI
- 14.61
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Environmental Science & Technology (publishedVersion)
- PubMed (publishedVersion)
- Topics
- Physical Sciences › Environmental Science › Water Science and Technology › Adsorption and biosorption for pollutant removal
- Physical Sciences › Environmental Science › Health, Toxicology and Mutagenesis › Toxic Organic Pollutants Impact
- Life Sciences › Agricultural and Biological Sciences › Soil Science › Soil Carbon and Nitrogen Dynamics
- Keywords
- black carbon, biochar, catechol, humic acid, organic matter adsorption, pyrogenic carbon, natural organic matter, combustion temperature, micropore surface area, nanopores, diffusion kinetics, pseudo-second-order kinetics, Freundlich isotherm, biochar amendment
- MeSH terms
- Adsorption, Catechols, Charcoal, Environment, Poaceae, Humic Substances, Kinetics, Laboratories, Models, Chemical, Temperature, Pinus, Quercus, Soot
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
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