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Facile Surface Functionalization of Hydrophobic Magnetic Nanoparticles
Open accessAbstract
Nonpolar phase synthesized hydrophobic nanocrystals show attractive properties and have demonstrated prominent potential in biomedical applications. However, the preparation of biocompatible nanocrystals is made difficult by the presence of hydrophobic surfactant stabilizer on their surfaces. To address this limitation, we have developed a facile, high efficiency, single-phase and low-cost method to convert hydrophobic magnetic nanoparticles (MNPs) to an aqueous phase using tetrahydrofuran, NaOH and 3,4-dihydroxyhydrocinnamic acid without any complicated organic synthesis. The as-transferred hydrophilic MNPs are water-soluble over a wide pH range (pH = 3-12), and the solubility is pH-controllable. Furthermore, the as-transferred MNPs with carboxylate can be readily adapted with further surface functionalization, varying from small molecule dyes to oligonucleotides and enzymes. Finally, the strategy developed here can easily be extended to other types of hydrophobic nanoparticles to facilitate biomedical applications of nanomaterials.
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Ultra-large-scale syntheses of monodisperse nanocrystals
Park, J., An, K., Hwang, Y., Park, J.-G., Noh, H.-J., Kim, J.-Y., Park, J.-H., Hwang, N.-M., & Hyeon, T. (2004) · Nature Materials · doi:10.1038/nmat1251 · Cited by 4,076
Guardia, P., Di Corato, R., Lartigue, L., Wilhelm, C., Espinosa, A., Garcia-Hernandez, M., Gazeau, F., Manna, L., & Pellegrino, T. (2012) · ACS Nano · doi:10.1021/nn2048137 · Cited by 752
Cited by
Organic Phase Syntheses of Magnetic Nanoparticles and Their Applications
Wu, L., Mendoza-Garcia, A., Li, Q., & Sun, S. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.5b00687 · Cited by 601
Kandasamy, G., & Maity, D. (2015) · International Journal of Pharmaceutics · doi:10.1016/j.ijpharm.2015.10.058 · Cited by 422
Recent Developments in Magnetic Diagnostic Systems
Lee, H., Shin, T.-H., Cheon, J., & Weissleder, R. (2015) · Chemical Reviews · doi:10.1021/cr500698d · Cited by 292
Yang, H. Y., Li, Y., & Lee, D. S. (2018) · Advanced Therapeutics · doi:10.1002/adtp.201800011 · Cited by 107
Zhang, W., Taheri-Ledari, R., Ganjali, F., Afruzi, F. H., Hajizadeh, Z., Saeidirad, M., Qazi, F. S., Kashtiaray, A., Sehat, S. S., Hamblin, M. R., et al. (2022) · Heliyon · doi:10.1016/j.heliyon.2022.e09577 · Cited by 79
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Metadata
- Authors
- Liu, Y., Chen, T., Wu, C., Qiu, L., Hu, R., Li, J., Cansiz, S., Zhang, L., Cui, C., Zhu, G., You, M., Zhang, T., & Tan, W.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2014-08-28
- Volume
- 136
- Issue
- 36
- Pages
- 12552-12555
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2321197535
- Cited by
- 187
- References
- 2
- FWCI
- 8.77
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Liu, Y., Chen, T., Wu, C., Qiu, L., Hu, R., Li, J., Cansiz, S., Zhang, L., Cui, C., Zhu, G., You, M., Zhang, T., & Tan, W. (2014). Facile Surface Functionalization of Hydrophobic Magnetic Nanoparticles. Journal of the American Chemical Society. https://doi.org/10.1021/ja5060324
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