The DOI matches its Crossref record; 29 of the 29 references it cites were found in a registry or an index.
Imparting Functionality to Biocatalysts via Embedding Enzymes into Nanoporous Materials by a de Novo Approach: Size-Selective Sheltering of Catalase in Metal–Organic Framework Microcrystals
Abstract
We develop a new concept to impart new functions to biocatalysts by combining enzymes and metal-organic frameworks (MOFs). The proof-of-concept design is demonstrated by embedding catalase molecules into uniformly sized ZIF-90 crystals via a de novo approach. We have carried out electron microscopy, X-ray diffraction, nitrogen sorption, electrophoresis, thermogravimetric analysis, and confocal microscopy to confirm that the ~10 nm catalase molecules are embedded in 2 μm single-crystalline ZIF-90 crystals with ~5 wt % loading. Because catalase is immobilized and sheltered by the ZIF-90 crystals, the composites show activity in hydrogen peroxide degradation even in the presence of protease proteinase K.
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Cites
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Cited by
Alsaiari, S. K., Patil, S., Alyami, M., Alamoudi, K. O., Aleisa, F. A., Merzaban, J. S., Li, M., & Khashab, N. M. (2018) · Journal of the American Chemical Society · doi:10.1021/jacs.7b11754 · Cited by 517
Multifunctional metal–organic framework heterostructures for enhanced cancer therapy
Liu, J., Huang, J., Zhang, L., & Lei, J. (2021) · Chemical Society Reviews · doi:10.1039/d0cs00178c · Cited by 285
Liao, Y.-T., Nguyen, V. C., Ishiguro, N., Young, A. P., Tsung, C.-K., & Wu, K. C.-W. (2020) · Applied Catalysis B: Environmental · doi:10.1016/j.apcatb.2020.118805 · Cited by 281
Self-citationControllable Syntheses of MOF‐Derived Materials
Zou, K., & Li, Z. (2018) · Chemistry – A European Journal · doi:10.1002/chem.201705415 · Cited by 172
Chen, J., Zhang, X., Huang, C., Cai, H., Hu, S., Wan, Q., Pei, X., & Wang, J. (2017) · Journal of Biomedical Materials Research Part A · doi:10.1002/jbm.a.35960 · Cited by 150
Metadata
- Authors
- Shieh, F.-K., Wang, S.-C., Yen, C.-I., Wu, C.-C., Dutta, S., Chou, L.-Y., Morabito, J. V., Hu, P., Hsu, M.-H., Wu, K. C.-W., & Tsung, C.-K.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-03-27
- Volume
- 137
- Issue
- 13
- Pages
- 4276-4279
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W2331326812
- Cited by
- 774
- References
- 29
- FWCI
- 28.56
- Type
- journal article
- Language
- en
- Open access
- closed
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- Shieh, F.-K., Wang, S.-C., Yen, C.-I., Wu, C.-C., Dutta, S., Chou, L.-Y., Morabito, J. V., Hu, P., Hsu, M.-H., Wu, K. C.-W., & Tsung, C.-K. (2015). Imparting Functionality to Biocatalysts via Embedding Enzymes into Nanoporous Materials by a de Novo Approach: Size-Selective Sheltering of Catalase in Metal–Organic Framework Microcrystals. Journal of the American Chemical Society. https://doi.org/10.1021/ja513058h
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