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A High-Rate Two-Dimensional Polyarylimide Covalent Organic Framework Anode for Aqueous Zn-Ion Energy Storage Devices
Open accessAbstract
Rechargeable aqueous Zn-ion energy storage devices are promising candidates for next-generation energy storage technologies. However, the lack of highly reversible Zn 2+ -storage anode materials with low potential windows remains a primary concern. Here, we report a two-dimensional polyarylimide covalent organic framework (PI-COF) anode with high-kinetics Zn 2+ -storage capability. The well-organized pore channels of PI-COF allow the high accessibility of the build-in redox-active carbonyl groups and efficient ion diffusion with a low energy barrier. The constructed PI-COF anode exhibits a specific capacity (332 C g –1 or 92 mAh g –1 at 0.7 A g –1 ), a high rate capability (79.8% at 7 A g –1 ), and a long cycle life (85% over 4000 cycles). In situ Raman investigation and first-principle calculations clarify the two-step Zn 2+ -storage mechanism, in which imide carbonyl groups reversibly form negatively charged enolates. Dendrite-free full Zn-ion devices are fabricated by coupling PI-COF anodes with MnO 2 cathodes, delivering excellent energy densities (23.9 ∼ 66.5 Wh kg –1 ) and supercapacitor-level power densities (133 ∼ 4782 W kg –1 ). This study demonstrates the feasibility of covalent organic framework as Zn 2+ -storage anodes and shows a promising prospect for constructing reliable aqueous energy storage devices.
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Metadata
- Authors
- Yu, M., Chandrasekhar, N., Raghupathy, R. K. M., Ly, K. H., Zhang, H., Dmitrieva, E., Liang, C., Lu, X., Kühne, T. D., Mirhosseini, H., Weidinger, I. M., & Feng, X.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2020-11-09
- Volume
- 142
- Issue
- 46
- Pages
- 19570-19578
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W3104594706
- Cited by
- 406
- References
- 39
- FWCI
- 17.98
- Type
- journal article
- Language
- en
- Open access
- green
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