The DOI matches its Crossref record; 6 of the 6 references it cites were found in a registry or an index.
Accessing Organonitrogen Compounds via C–N Coupling in Electrocatalytic CO2 Reduction
Abstract
Given the limited product variety of electrocatalytic CO 2 reduction reactions solely from CO 2 and H 2 O as the reactants, it is desirable to expand the product scope by introducing additional reactants that provide elemental diversity. The integration of inorganic heteroatom-containing reactants into electrocatalytic CO 2 reduction could, in principle, enable the sustainable synthesis of valuable products, such as organonitrogen compounds, which have widespread applications but typically rely on NH 3 derived from the energy-intensive and fossil-fuel-dependent Haber–Bosch process for their industrial-scale production. In this Perspective, research progress toward building C–N bonds in N-integrated electrocatalytic CO 2 reduction is highlighted, and the electrosyntheses of urea, acetamides, and amines are examined from the standpoints of reactivity, catalyst structure, and, most fundamentally, mechanism. Mechanistic discussions of C–N coupling in these advances are emphasized and critically evaluated, with the aim of directing future investigations on improving the product yield and broadening the product scope of N-integrated electrocatalytic CO 2 reduction.
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Cites
CO 2 electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface
Dinh, C.-T., Burdyny, T., Kibria, M. G., Seifitokaldani, A., Gabardo, C. M., García de Arquer, F. P., Kiani, A., Edwards, J. P., De Luna, P., Bushuyev, O. S., et al. (2018) · Science · doi:10.1126/science.aas9100 · Cited by 2,515
Electrocatalytic Conversion of Carbon Dioxide to Methane and Methanol on Transition Metal Surfaces
Kuhl, K. P., Hatsukade, T., Cave, E. R., Abram, D. N., Kibsgaard, J., & Jaramillo, T. F. (2014) · Journal of the American Chemical Society · doi:10.1021/ja505791r · Cited by 1,649
Industrial carbon dioxide capture and utilization: state of the art and future challenges
Gao, W., Liang, S., Wang, R., Jiang, Q., Zhang, Y., Zheng, Q., Xie, B., Toe, C. Y., Zhu, X., Wang, J., et al. (2020) · Chemical Society Reviews · doi:10.1039/d0cs00025f · Cited by 1,388
Domino electroreduction of CO2 to methanol on a molecular catalyst
Wu, Y., Jiang, Z., Lu, X., Liang, Y., & Wang, H. (2019) · Nature · doi:10.1038/s41586-019-1760-8 · Cited by 1,194
Verma, S., Hamasaki, Y., Kim, C., Huang, W., Lu, S., Jhong, H.-R. M., Gewirth, A. A., Fujigaya, T., Nakashima, N., & Kenis, P. J. A. (2018) · ACS Energy Letters · doi:10.1021/acsenergylett.7b01096 · Cited by 521
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Cited by
Luo, Y., Xie, K., Ou, P., Lavallais, C., Peng, T., Chen, Z., Zhang, Z., Wang, N., Li, X.-Y., Grigioni, I., et al. (2023) · Nature Catalysis · doi:10.1038/s41929-023-01020-4 · Cited by 380
Meng, N., Ma, X., Wang, C., Wang, Y., Yang, R., Shao, J., Huang, Y., Xu, Y., Zhang, B., & Yu, Y. (2022) · ACS Nano · doi:10.1021/acsnano.2c01177 · Cited by 322
Jiang, M., Wang, H., Zhu, M., Luo, X., He, Y., Wang, M., Wu, C., Zhang, L., Li, X., Liao, X., et al. (2024) · Chemical Society Reviews · doi:10.1039/d3cs00857f · Cited by 299
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Metadata
- Authors
- Tao, Z., Rooney, C. L., Liang, Y., & Wang, H.
- Venue
- Journal of the American Chemical Society
- Publisher
- American Chemical Society (ACS)
- Published
- 2021-11-17
- Volume
- 143
- Issue
- 47
- Pages
- 19630-19642
- ISSN
- 0002-7863 (ISSN-L)
- 1520-5126
- OpenAlex
- W3211664316
- Cited by
- 356
- References
- 6
- FWCI
- 9.69
- Type
- journal article
- Language
- en
- Open access
- closed
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