The DOI matches its Crossref record; 44 of the 44 references it cites were found in a registry or an index.
Three-dimensional porous hollow fibre copper electrodes for efficient and high-rate electrochemical carbon dioxide reduction
Open accessAbstract
Aqueous-phase electrochemical reduction of carbon dioxide requires an active, earth-abundant electrocatalyst, as well as highly efficient mass transport. Here we report the design of a porous hollow fibre copper electrode with a compact three-dimensional geometry, which provides a large area, three-phase boundary for gas–liquid reactions. The performance of the copper electrode is significantly enhanced; at overpotentials between 200 and 400 mV, faradaic efficiencies for carbon dioxide reduction up to 85% are obtained. Moreover, the carbon monoxide formation rate is at least one order of magnitude larger when compared with state-of-the-art nanocrystalline copper electrodes. Copper hollow fibre electrodes can be prepared via a facile method that is compatible with existing large-scale production processes. The results of this study may inspire the development of new types of microtubular electrodes for electrochemical processes in which at least one gas-phase reactant is involved, such as in fuel cell technology.
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Self-citationAqueous CO2 Reduction at Very Low Overpotential on Oxide-Derived Au Nanoparticles
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Self-citationCO 2 electroreduction to ethylene via hydroxide-mediated copper catalysis at an abrupt interface
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Large-Scale and Highly Selective CO2 Electrocatalytic Reduction on Nickel Single-Atom Catalyst
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Metadata
- Authors
- Kas, R., Hummadi, K. K., Kortlever, R., de Wit, P., Milbrat, A., Luiten-Olieman, M. W. J., Benes, N. E., Koper, M. T. M., & Mul, G.
- Venue
- Nature Communications
- Published
- 2016-02-18
- Volume
- 7
- Issue
- 1
- Pages
- 10748-10748
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2339617683
- Cited by
- 365
- References
- 44
- FWCI
- 12.96
- Type
- journal article
- Language
- en
- Open access
- gold
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