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Pure PEDOT:PSS hydrogels

Open access
Lu, Baoyang, Yuk, Hyunwoo, Lin, Shaoting, Jian, Nannan, Qu, Kai, Xu, Jingkun, Zhao, Xuanhe·2019·Nature Communications

Abstract

Hydrogels of conducting polymers, particularly poly(3,4-ethylenedioxythiophene):poly(styrene sulfonate) (PEDOT:PSS), provide a promising electrical interface with biological tissues for sensing and stimulation, owing to their favorable electrical and mechanical properties. While existing methods mostly blend PEDOT:PSS with other compositions such as non-conductive polymers, the blending can compromise resultant hydrogels’ mechanical and/or electrical properties. Here, we show that designing interconnected networks of PEDOT:PSS nanofibrils via a simple method can yield high-performance pure PEDOT:PSS hydrogels. The method involves mixing volatile additive dimethyl sulfoxide (DMSO) into aqueous PEDOT:PSS solutions followed by controlled dry-annealing and rehydration. The resultant hydrogels exhibit a set of properties highly desirable for bioelectronic applications, including high electrical conductivity (~20 S cm−1 in PBS, ~40 S cm−1 in deionized water), high stretchability (> 35% strain), low Young’s modulus (~2 MPa), superior mechanical, electrical and electrochemical stability, and tunable isotropic/anisotropic swelling in wet physiological environments.

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Metadata

Authors
Lu, B., Yuk, H., Lin, S., Jian, N., Qu, K., Xu, J., & Zhao, X.
Venue
Nature Communications
Published
2019-03-05
Volume
10
Issue
1
Pages
1043-1043
ISSN
2041-1723 (ISSN-L)
OpenAlex
W2918284348
Cited by
1,035
References
10
FWCI
37.55
Type
journal article
Language
en
Open access
gold

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CoChat. (2026). Citation check: Pure PEDOT:PSS hydrogels. https://app.cochat.ai/papers/10.1038/s41467-019-09003-5
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Lu, B., Yuk, H., Lin, S., Jian, N., Qu, K., Xu, J., & Zhao, X. (2019). Pure PEDOT:PSS hydrogels. Nature Communications. https://doi.org/10.1038/s41467-019-09003-5

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