The DOI matches its Crossref record; 43 of the 43 references it cites were found in a registry or an index.
Selective light absorber-assisted single nickel atom catalysts for ambient sunlight-driven CO2 methanation
Open accessAbstract
Ambient sunlight-driven CO 2 methanation cannot be realized due to the temperature being less than 80 °C upon irradiation with dispersed solar energy. In this work, a selective light absorber was used to construct a photothermal system to generate a high temperature (up to 288 °C) under weak solar irradiation (1 kW m−2), and this temperature is three times higher than that in traditional photothermal catalysis systems. Moreover, ultrathin amorphous Y 2 O 3 nanosheets with confined single nickel atoms (SA Ni/Y 2 O 3) were synthesized, and they exhibited superior CO 2 methanation activity. As a result, 80% CO 2 conversion efficiency and a CH 4 production rate of 7.5 L m−2 h−1 were achieved through SA Ni/Y 2 O 3 under solar irradiation (from 0.52 to 0.7 kW m−2) when assisted by a selective light absorber, demonstrating that this system can serve as a platform for directly harnessing dispersed solar energy to convert CO 2 to valuable chemicals.
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Metadata
- Authors
- Li, Y., Hao, J., Song, H., Zhang, F., Bai, X., Meng, X., Zhang, H., Wang, S., Hu, Y., & Ye, J.
- Venue
- Nature Communications
- Published
- 2019-05-29
- Volume
- 10
- Issue
- 1
- Pages
- 2359-2359
- ISSN
- 2041-1723 (ISSN-L)
- OpenAlex
- W2947298237
- Cited by
- 305
- References
- 43
- FWCI
- 6.82
- Type
- journal article
- Language
- en
- Open access
- gold
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- Li, Y., Hao, J., Song, H., Zhang, F., Bai, X., Meng, X., Zhang, H., Wang, S., Hu, Y., & Ye, J. (2019). Selective light absorber-assisted single nickel atom catalysts for ambient sunlight-driven CO2 methanation. Nature Communications. https://doi.org/10.1038/s41467-019-10304-y
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