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p-type Mesoscopic Nickel Oxide/Organometallic Perovskite Heterojunction Solar Cells

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Wang, Kuo-Chin, Jeng, Jun-Yuan, Shen, Po-Shen, Chang, Yu-Cheng, Diau, Eric Wei-Guang, Tsai, Cheng-Hung, Chao, Tzu-Yang, Hsu, Hsu-Cheng, Lin, Pei-Ying, Chen, Peter, Guo, Tzung-Fang, Wen, Ten-Chin·2014·Scientific Reports

DOI 10.1038/srep04756

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Abstract

In this article, we present a new paradigm for organometallic hybrid perovskite solar cell using NiO inorganic metal oxide nanocrystalline as p-type electrode material and realized the first mesoscopic NiO/perovskite/[6,6]-phenyl C61-butyric acid methyl ester (PC61BM) heterojunction photovoltaic device. The photo-induced transient absorption spectroscopy results verified that the architecture is an effective p-type sensitized junction, which is the first inorganic p-type, metal oxide contact material for perovskite-based solar cell. Power conversion efficiency of 9.51% was achieved under AM 1.5 G illumination, which significantly surpassed the reported conventional p-type dye-sensitized solar cells. The replacement of the organic hole transport materials by a p-type metal oxide has the advantages to provide robust device architecture for further development of all-inorganic perovskite-based thin-film solar cells and tandem photovoltaics.

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See all 444

Authors: Wang, K.-C., Jeng, J.-Y., Shen, P.-S., Chang, Y.-C., Diau, E. W.-G., Tsai, C.-H., Chao, T.-Y., Hsu, H.-C., Lin, P.-Y., Chen, P., Guo, T.-F., & Wen, T.-C.
Venue: Scientific Reports
Publisher: Springer Science and Business Media LLC
Published: 2014-04-23
Volume: 4
Issue: 1
Pages: 4756-4756
ISSN: 2045-2322 (ISSN-L)
DOI: 10.1038/srep04756
OpenAlex: W1967782095
Cited by: 444
References: 47
FWCI: 35.55
Type: journal article
Language: en
Open access: gold

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p-type Mesoscopic Nickel Oxide/Organometallic Perovskite Heterojunction Solar Cells

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