S-doped AuPd aerogels as high efficiency catalysts for the oxygen reduction reaction by balancing the ratio between bridging S 2 2− and apical S 2− ligands
Abstract
S-doped AuPd aerogels with a breathtaking performance towards the ORR are achieved by balancing the ratio of S 2 2− and S 2− ligands.
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The AuPb3, PbS and PbS2 in the S-doped AuPb networks are involved in the formation of AuPdPt, PtS, Pd2.8S and Pd(II)-Pt(II)S2 during conversion to the aerogels, and Pb diffuses into the reaction media.
“This is because the AuPb3,”
From Realization of Au81Pd2Pt9-S8B4.6A3.4 aerogels as superior catalysts toward HER and ORR by synergism of coarse and fine tuning d-band center of Pt (2023) · cites this paper as [26]
The superior ORR activity of AuPd-SB67A33 aerogels is because of the introduction of an optimal ratio of bridging S2^2- and apical S2- ligands, whose synergistic effect may adjust the d-band center of Pd to an optimal level.
“because of the introduction of an optimal ratio”
From Realization of Au81Pd2Pt9-S8B4.6A3.4 aerogels as superior catalysts toward HER and ORR by synergism of coarse and fine tuning d-band center of Pt (2023) · cites this paper as [26]
The diffraction peaks of the aerogels in the pink, orange, and brown rectangles agree with Pd2.8S, PdS2, and Pd, respectively.
“are in good agreement with those of the Pd2.8S”
From Realization of Au81Pd2Pt9-S8B4.6A3.4 aerogels as superior catalysts toward HER and ORR by synergism of coarse and fine tuning d-band center of Pt (2023) · cites this paper as [26]
AuPd-SB67A33 aerogels show superior ORR activity in alkaline media (E1/2 = 0.970 V, ΔE1/2 = 85 mV) compared with commercial Pt/C catalysts (E1/2 = 0.885 V).
“AuPd-SB67A33 aerogels show the supe”
From Realization of Au81Pd2Pt9-S8B4.6A3.4 aerogels as superior catalysts toward HER and ORR by synergism of coarse and fine tuning d-band center of Pt (2023) · cites this paper as [26]
Pt(II) ions cannot be bonded with bridging S2^2- ligands to form Pt(II)S2, unlike the formation of PdS2 reported in previous work.
“Note that Pt(II) ions cannot be bonded with bridging S2 2- ligands to form Pt(II)S2, unlike the formation of PdS2 reported in in our previous work [26].”
From Realization of Au81Pd2Pt9-S8B4.6A3.4 aerogels as superior catalysts toward HER and ORR by synergism of coarse and fine tuning d-band center of Pt (2023) · cites this paper as [26]
The excellent stability of the as-prepared CS Pt3Fe@Pt NP-O-A-Fe SA/C catalyst is likely attributed to O-bridging structures (N4-Fe-O-Pt units) on the surface of Pt3Fe@Pt NPs, which suppress the formation of Pt-O species at high potentials and inhibit the agglomeration and dissolution of Pt3Fe NPs.
“This is likely attributed to the presence of O-bridging structures (N4–Fe–O–Pt units) on the surface of Pt3Fe@Pt NPs, which not only can suppress the formation of Pt–O species at high potentials, but also can inhibit the agglomeration and dissolution of Pt3Fe NPs.”
From Tuning the local environment of atomic Pt shells of Pt <sub>3</sub> Fe@Pt nanoparticles enables energy-saving hydrogen production (2026) · cites this paper as [83]
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Self-citation
- Authors
- Zhang, X., Wang, J., Zhang, M., Yue, X., Du, W., Fan, W., & Xia, H.
- Affiliations
- Shandong University (CN)
- Yantai University (CN)
- Corresponding author
- Fan, Weiliu
- Xia, Haibing
- Venue
- Journal of Materials Chemistry A
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2022
- Volume
- 10
- Issue
- 14
- Pages
- 7800-7810
- ISSN
- 2050-7488 (ISSN-L)
- 2050-7496
- OpenAlex
- W4213129369
- Cited by
- 17
- References
- 74
- Citations by year
- 2026: 2 · 2025: 6 · 2024: 4 · 2023: 4 · 2022: 1
- FWCI
- 0.72
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Journal of Materials Chemistry A (publishedVersion)
- Funders
- National Natural Science Foundation of China (22072076, 21773142)
- Shandong University
- Taishan Scholar Foundation of Shandong Province (tsqn20161001)
- Topics
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
- Physical Sciences › Materials Science › Materials Chemistry › Catalytic Processes in Materials Science
- Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
- Keywords
- oxygen reduction reaction, electrocatalysts
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
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