The DOI matches its Crossref record; 8 of the 8 references it cites were found in a registry or an index.
Interaction of colloidal nanoparticles with their local environment: the (ionic) nanoenvironment around nanoparticles is different from bulk and determines the physico-chemical properties of the nanoparticles
Open accessAbstract
The physico-chemical properties of colloidal nanoparticles (NPs) are influenced by their local environment, as, in turn, the local environment influences the physico-chemical properties of the NPs. In other words, the local environment around NPs has a profound impact on the NPs, and it is different from bulk due to interaction with the NP surface. So far, this important effect has not been addressed in a comprehensive way in the literature. The vicinity of NPs can be sensitively influenced by local ions and ligands, with effects already occurring at extremely low concentrations. NPs in the Hückel regime are more sensitive to fluctuations in the ionic environment, because of a larger Debye length. The local ion concentration hereby affects the colloidal stability of the NPs, as it is different from bulk owing to Debye Hückel screening caused by the charge of the NPs. This can have subtle effects, now caused by the environment to the performance of the NP, such as for example a buffering effect caused by surface reaction on ultrapure ligand-free nanogold, a size quenching effect in the presence of specific ions and a significant impact on fluorophore-labelled NPs acting as ion sensors. Thus, the aim of this review is to clarify and give an unifying view of the complex interplay between the NP's surface with their nanoenvironment.
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Metadata
- Authors
- Pfeiffer, C., Rehbock, C., Hühn, D., Carrillo-Carrion, C., de Aberasturi, D. J., Merk, V., Barcikowski, S., & Parak, W. J.
- Venue
- Journal of The Royal Society Interface
- Publisher
- The Royal Society
- Published
- 2014-07-06
- Volume
- 11
- Issue
- 96
- Pages
- 20130931
- ISSN
- 1742-5662 (ISSN-L)
- 1742-5689
- OpenAlex
- W2160154617
- Cited by
- 378
- References
- 8
- FWCI
- 21.21
- Type
- journal article
- Language
- en
- Open access
- green
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- Pfeiffer, C., Rehbock, C., Hühn, D., Carrillo-Carrion, C., de Aberasturi, D. J., Merk, V., Barcikowski, S., & Parak, W. J. (2014). Interaction of colloidal nanoparticles with their local environment: the (ionic) nanoenvironment around nanoparticles is different from bulk and determines the physico-chemical properties of the nanoparticles. Journal of The Royal Society Interface. https://doi.org/10.1098/rsif.2013.0931
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