The DOI matches its Crossref record; 10 of the 10 references it cites were found in a registry or an index.
Femtosecond Mid-IR Pump-Probe Spectroscopy of Liquid Water: Evidence for a Two-Component Structure
Abstract
A femtosecond mid-infrared pump-probe study of the vibrational and orientational dynamics of the OH-stretching mode of HDO dissolved in D 2 O is presented. The orientational relaxation of the HDO molecules was observed to occur on either a very slow or a very fast time scale, with associated time constants of τ R = 13 picoseconds and τ R = 0.7 picosecond. It was observed that strongly hydrogen-bonded water molecules only relax through the slow orientational relaxation process, whereas the fast process dominates for weakly hydrogen-bonded molecules. This suggests that, with respect to orientional dynamics, two distinct molecular species exist in liquid water.
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Citations
Cites
Hydrogen-bond kinetics in liquid water
Luzar, A., & Chandler, D. (1996) · Nature · doi:10.1038/379055a0 · Cited by 2,048
Effect of Environment on Hydrogen Bond Dynamics in Liquid Water
Luzar, A., & Chandler, D. (1996) · Physical Review Letters · doi:10.1103/physrevlett.76.928 · Cited by 1,180
Kindt, J. T., & Schmuttenmaer, C. A. (1996) · The Journal of Physical Chemistry · doi:10.1021/jp960141g · Cited by 687
Hansen, C., Stickel, F., Berger, T., Richert, R., & Fischer, E. W. (1997) · The Journal of Chemical Physics · doi:10.1063/1.474456 · Cited by 430
Theory of fluorescence depolarization in macromolecules and membranes
Szabo, A. (1984) · The Journal of Chemical Physics · doi:10.1063/1.447378 · Cited by 409
THz reflection spectroscopy of liquid water
Thrane, L., Jacobsen, R. H., Uhd Jepsen, P., & Keiding, S. R. (1995) · Chemical Physics Letters · doi:10.1016/0009-2614(95)00543-d · Cited by 339
Chang, Y. J., & Castner, E. W. (1993) · The Journal of Chemical Physics · doi:10.1063/1.465710 · Cited by 225
New spectroscopy of water using tunable picosecond pulses in the infrared
Graener, H., Seifert, G., & Laubereau, A. (1991) · Physical Review Letters · doi:10.1103/physrevlett.66.2092 · Cited by 217
Far-infrared absorption in liquid water
Hasted, J. B., Husain, S., Frescura, F. A. M., et al. (1985) · Chemical Physics Letters · doi:10.1016/0009-2614(85)85366-5 · Cited by 181
Tokmakoff, A., Urdahl, R. S., Zimdars, D. A., Francis, R. S., Kwok, A. S., & Fayer, M. D. (1995) · The Journal of Chemical Physics · doi:10.1063/1.468568 · Cited by 85
Cited by
Hydrogen bonding definitions and dynamics in liquid water
Kumar, R., Schmidt, J. R., & Skinner, J. L. (2007) · The Journal of Chemical Physics · doi:10.1063/1.2742385 · Cited by 772
Resonant intermolecular transfer of vibrational energy in liquid water
Woutersen, S., & Bakker, H. J. (1999) · Nature · doi:10.1038/990058 · Cited by 553
Self-citationHydrogen bonds in liquid water are broken only fleetingly
Eaves, J. D., Loparo, J. J., Fecko, C. J., Roberts, S. T., Tokmakoff, A., & Geissler, P. L. (2005) · Proceedings of the National Academy of Sciences · doi:10.1073/pnas.0505125102 · Cited by 507
Dynamics of Water Molecules in Aqueous Solvation Shells
Kropman, M. F., & Bakker, H. J. (2001) · Science · doi:10.1126/science.1058190 · Cited by 465
Self-citationTHz Spectroscopy of LiquidH2OandD2O
Rønne, C., Åstrand, P.-O., & Keiding, S. R. (1999) · Physical Review Letters · doi:10.1103/physrevlett.82.2888 · Cited by 366
Metadata
- Authors
- Woutersen, S., Emmerichs, U., & Bakker, H. J.
- Venue
- Science
- Published
- 1997-10-24
- Volume
- 278
- Issue
- 5338
- Pages
- 658-660
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2051698784
- Cited by
- 579
- References
- 10
- FWCI
- 8.02
- Type
- journal article
- Language
- en
- Open access
- closed
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- Woutersen, S., Emmerichs, U., & Bakker, H. J. (1997). Femtosecond Mid-IR Pump-Probe Spectroscopy of Liquid Water: Evidence for a Two-Component Structure. Science. https://doi.org/10.1126/science.278.5338.658
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Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.