Cited by 217CO2 Sequestration and Geologic InteractionsGeological and Geochemical AnalysisCarbon Dioxide Capture Technologies

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CARBONATED SERPENTINITE (LISTWANITE) AT ATLIN, BRITISH COLUMBIA: A GEOLOGICAL ANALOGUE TO CARBON DIOXIDE SEQUESTRATION

Hansen, L. D., Dipple, G. M., Gordon, T. M., Kellett, D. A.·2005·The Canadian Mineralogist

DOI 10.2113/gscanmin.43.1.225

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Abstract

Listwanite, a carbonate-altered serpentinite commonly associated with gold and mercury mineralization, also represents a natural analogue to CO2 sequestration via in situ carbonation of minerals. The reaction pathways and permeability structure controlling listwanite formation are preserved and exposed at Atlin, British Columbia, where listwanite extends tens of meters into surrounding wallrock. The overall mineralogical transformation is the same as that being considered for industrial sequestration of CO2. In nature, this reaction proceeds via subreactions that are fossilized as spatially distinct zones. Serpentine + olivine + brucite reacted with CO2 to form serpentine + magnesite, then magnesite + talc, and finally magnesite + quartz. These mineralogical transformations are achieved isochemically, except for the volatile species H2O and CO2. Although the first stage of the reaction only accounts for about 5‐15% of the carbonation potential of serpentinite, it is very widespread, and therefore may have sequestered a significant portion of the total bound CO2. Moreover, within intact bedrock, the progress of the magnesite + talc reaction generates fracture permeability, which appears to have locally enhanced reaction. The first two reactions combined account for about half of the carbonation potential for serpentinite and have a small associated increase in the volume of solids, which limits porosity loss. They thus hold the greatest promise for in situ mineral carbonation. The carbonation reactions are controlled by the activity of CO2 in the fluid phase. Proponents of industrial mineral-carbonation processes therefore may seek to control the composition of the input gas to preferentially drive carbonation reactions that minimize porosity loss and maximize permeability generation. Magnetite was progressively destroyed during carbonation, which allowed magnetic susceptibility to be used as a proxy for carbonation-reaction progress. It facilitated the mapping of the permeability structure of these systems and delineated subtle variations in reaction progress that might otherwise have gone unnoticed in the field.

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Authors: Hansen, L. D., Dipple, G. M., Gordon, T. M., & Kellett, D. A.
Affiliations: University of British Columbia (CA)
University of Calgary (CA)
ORCID: Hansen, L. D.
Dipple, G. M.
Kellett, D. A.
Venue: The Canadian Mineralogist
Publisher: Mineralogical Association of Canada
Published: 2005-02-01
Volume: 43
Issue: 1
Pages: 225-239
ISSN: 0008-4476 (ISSN-L)
1499-1261
DOI: 10.2113/gscanmin.43.1.225
OpenAlex: W2057774402
Cited by: 216
References: 27
Citations by year: 2026: 14 · 2025: 11 · 2024: 11 · 2023: 13 · 2022: 21 · 2021: 23 · 2020: 12 · 2019: 13 · 2018: 11 · 2017: 14 · 2016: 9 · 2015: 9 · 2014: 4 · 2013: 12 · 2012: 16
FWCI: 3.00
Type: journal article
Language: en
Open access: closed
Locations: The Canadian Mineralogist (publishedVersion)
Funders: Canadian Natural Resources Limited
Natural Resources Canada
Topics: Physical Sciences › Environmental Science › Environmental Engineering › CO2 Sequestration and Geologic Interactions
Physical Sciences › Earth and Planetary Sciences › Geochemistry and Petrology › Geological and Geochemical Analysis
Physical Sciences › Chemical Engineering › Filtration and Separation › Carbon Dioxide Capture Technologies
Keywords: serpentinite, CO2 mineralization, CO2 sequestration, magnesite, talc, brucite, olivine, serpentine, fracture permeability, porosity reduction, magnetite, magnetic susceptibility, reaction progress

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CARBONATED SERPENTINITE (LISTWANITE) AT ATLIN, BRITISH COLUMBIA: A GEOLOGICAL ANALOGUE TO CARBON DIOXIDE SEQUESTRATION

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