The DOI matches its Crossref record; 10 of the 10 references it cites were found in a registry or an index.
Selective Electrochemical Reduction of Carbon Dioxide to Ethanol on a Boron‐ and Nitrogen‐Co‐doped Nanodiamond
Abstract
Electrochemical reduction of CO 2 to ethanol, a clean and renewable liquid fuel with high heating value, is an attractive strategy for global warming mitigation and resource utilization. However, converting CO 2 to ethanol remains great challenge due to the low activity, poor product selectivity and stability of electrocatalysts. Here, the B‐ and N‐co‐doped nanodiamond (BND) was reported as an efficient and stable electrode for selective reduction of CO 2 to ethanol. Good ethanol selectivity was achieved on the BND with high Faradaic efficiency of 93.2 % (−1.0 V vs. RHE), which overcame the limitation of low selectivity for multicarbon or high heating value fuels. Its superior performance was mainly originated from the synergistic effect of B and N co‐doping, high N content and overpotential for hydrogen evolution. The possible pathway for CO 2 reduction revealed by DFT computation was CO 2→*COOH→*CO→*COCO→*COCH 2 OH→*CH 2 OCH 2 OH→CH 3 CH 2 OH.
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Electrocatalysis for CO 2 conversion: from fundamentals to value-added products
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Metadata
- Authors
- Liu, Y., Zhang, Y., Cheng, K., Quan, X., Fan, X., Su, Y., Chen, S., Zhao, H., Zhang, Y., Yu, H., & Hoffmann, M. R.
- Venue
- Angewandte Chemie
- Publisher
- Wiley
- Published
- 2017-10-24
- Volume
- 129
- Issue
- 49
- Pages
- 15813-15817
- ISSN
- 0044-8249 (ISSN-L)
- 1521-3757
- OpenAlex
- W4250038493
- Cited by
- 196
- References
- 10
- FWCI
- 7.90
- Type
- journal article
- Language
- en
- Open access
- closed
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- Liu, Y., Zhang, Y., Cheng, K., Quan, X., Fan, X., Su, Y., Chen, S., Zhao, H., Zhang, Y., Yu, H., & Hoffmann, M. R. (2017). Selective Electrochemical Reduction of Carbon Dioxide to Ethanol on a Boron‐ and Nitrogen‐Co‐doped Nanodiamond. Angewandte Chemie. https://doi.org/10.1002/ange.201706311
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