Cited by 594Electrocatalysts for Energy ConversionCatalytic Processes in Materials ScienceHydrogen Storage and Materials

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Engineering the Coordination Environment of Single‐Atom Platinum Anchored on Graphdiyne for Optimizing Electrocatalytic Hydrogen Evolution

Yin, Xue‐Peng, Wang, Hong‐Juan, Tang, Shang‐Feng, Lu, Xiu‐Li, Shu, Miao, Si, Rui, Lu, Tong‐Bu·2018·Angewandte Chemie International Edition

DOI 10.1002/anie.201804817

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Abstract

Abstract Two Pt single‐atom catalysts (SACs) of Pt‐GDY1 and Pt‐GDY2 were prepared on graphdiyne (GDY)supports. The isolated Pt atoms are dispersed on GDY through the coordination interactions between Pt atoms and alkynyl C atoms in GDY, with the formation of five‐coordinated C 1 ‐Pt‐Cl 4 species in Pt‐GDY1 and four‐coordinated C 2 ‐Pt‐Cl 2 species in Pt‐GDY2. Pt‐GDY2 shows exceptionally high catalytic activity for the hydrogen evolution reaction (HER), with a mass activity up to 3.3 and 26.9 times more active than Pt‐GDY1 and the state‐of‐the‐art commercial Pt/C catalysts, respectively. Pt‐GDY2 possesses higher total unoccupied density of states of Pt 5d orbital and close to zero value of Gibbs free energy of the hydrogen adsorption (|Δ |) at the Pt active sites, which are responsible for its excellent catalytic performance. This work can help better understand the structure–catalytic activity relationship in Pt SACs.

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411Chapter 9 Electrocatalyticelectrocatalytic hydrogenhydrogen productionproduction
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Authors: Yin, X., Wang, H., Tang, S., Lu, X., Shu, M., Si, R., & Lu, T.
Affiliations: Institute for New Energy Materials & Low Carbon Technologies School of Materials Science and Engineering Tianjin University of Technology Tianjin 300384 China
Chinese Academy of Sciences (CN)
Tianjin University of Technology (CN)
Corresponding author: Si, Rui
Lu, Tong‐Bu
ORCID: Si, Rui
Lu, Tong‐Bu
Venue: Angewandte Chemie International Edition
Publisher: Wiley
Published: 2018-06-28
Volume: 57
Issue: 30
Pages: 9382-9386
ISSN: 1433-7851 (ISSN-L)
1521-3773
DOI: 10.1002/anie.201804817
OpenAlex: W2805542846
Cited by: 594
References: 49
Citations by year: 2026: 36 · 2025: 48 · 2024: 65 · 2023: 78 · 2022: 91 · 2021: 114 · 2020: 103 · 2019: 47 · 2018: 12
FWCI: 15.94
Type: journal article
Language: en
Open access: closed
Licence: onlinelibrary.wiley.com/termsAndConditions#vor (vor)
Locations: Angewandte Chemie International Edition (publishedVersion)
PubMed (publishedVersion)
Funders: National Natural Science Foundation of China (21790052 , 21331007 and 21773288)
Topics: Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
Physical Sciences › Materials Science › Materials Chemistry › Catalytic Processes in Materials Science
Physical Sciences › Materials Science › Materials Chemistry › Hydrogen Storage and Materials
Keywords: single-atom catalysts, platinum, graphdiyne, hydrogen evolution reaction, electrocatalysis, coordination environment, structure-activity relationship, hydrogen adsorption Gibbs free energy, mass activity

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Engineering the Coordination Environment of Single‐Atom Platinum Anchored on Graphdiyne for Optimizing Electrocatalytic Hydrogen Evolution

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