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Platinum/Nickel Bicarbonate Heterostructures towards Accelerated Hydrogen Evolution under Alkaline Conditions
Abstract
Heterostructured nanomaterials, generally have physicochemical properties that differ from those of the individual components, and thus have potential in a wide range of applications. New platinum (Pt)/nickel bicarbonate (Ni(HCO 3)2) heterostructures are designed for an efficient alkaline hydrogen evolution reaction (HER). Notably, the specific and mass activity of Pt in Pt/Ni(HCO 3)2 are substantially improved compared to the bare Pt nanoparticles (NPs). The Ni(HCO 3)2 provides abundant water adsorption/dissociation sites and modulate the electronic structure of Pt, which determine the elementary reaction kinetics of alkaline HER. The Ni(HCO 3)2 nanoplates offer a platform for the uniform dispersion of Pt NPs, ensuring the maximum exposure of active sites. The results demonstrate that, Ni(HCO 3)2 is an effective catalyst promoter for alkaline HER.
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Heterojunction catalyst in electrocatalytic water splitting
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Metadata
- Authors
- Lao, M., Rui, K., Zhao, G., Cui, P., Zheng, X., Dou, S. X., & Sun, W.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2019-03-13
- Volume
- 58
- Issue
- 16
- Pages
- 5432-5437
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2914781440
- Cited by
- 244
- References
- 6
- FWCI
- 8.50
- Type
- journal article
- Language
- en
- Open access
- closed
- Licence
- Funders
- Australian Research Council (DE160100596)
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- Lao, M., Rui, K., Zhao, G., Cui, P., Zheng, X., Dou, S. X., & Sun, W. (2019). Platinum/Nickel Bicarbonate Heterostructures towards Accelerated Hydrogen Evolution under Alkaline Conditions. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201901010
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