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An Engineered Superhydrophilic/Superaerophobic Electrocatalyst Composed of the Supported CoMoSx Chalcogel for Overall Water Splitting
Abstract
The development of high‐efficiency electrocatalysts for large‐scale water splitting is critical but also challenging. In this study, a hierarchical CoMoSx chalcogel was synthesized on a nickel foam (NF) through an in situ metathesis reaction and demonstrated excellent activity and stability in the electrocatalytic hydrogen evolution reaction and oxygen evolution reaction in alkaline media. The high catalytic activity could be ascribed to the abundant active sites/defects in the amorphous framework and promotion of activity through cobalt doping. Furthermore, the superhydrophilicity and superaerophobicity of micro‐/nanostructured CoMoSx/NF promoted mass transfer by facilitating access of electrolytes and ensuring fast release of gas bubbles. By employing CoMoSx/NF as bifunctional electrocatalysts, the overall water splitting device delivered a current density of 500 mA cm−2 at a low voltage of 1.89 V and maintained its activity without decay for 100 h.
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Cited by
Bifunctional Electrocatalysts for Overall and Hybrid Water Splitting
Quan, L., Jiang, H., Mei, G., Sun, Y., & You, B. (2024) · Chemical Reviews · doi:10.1021/acs.chemrev.3c00332 · Cited by 874
Water Splitting: From Electrode to Green Energy System
Li, X., Zhao, L., Yu, J., Liu, X., Zhang, X., Liu, H., & Zhou, W. (2020) · Nano-Micro Letters · doi:10.1007/s40820-020-00469-3 · Cited by 619
Self-supported electrocatalysts for practical water electrolysis
Yang, H., Driess, M., & Menezes, P. W. (2021) · Advanced Energy Materials · doi:10.1002/aenm.202102074 · Cited by 489
Gas Evolution in Water Electrolysis
Kempler, P. A., Coridan, R. H., & Luo, L. (2024) · Chemical Reviews · doi:10.1021/acs.chemrev.4c00211 · Cited by 289
Progress and Perspectives for Solar‐Driven Water Electrolysis to Produce Green Hydrogen
Zhao, H., & Yuan, Z. (2023) · Advanced Energy Materials · doi:10.1002/aenm.202300254 · Cited by 240
Metadata
- Authors
- Shan, X., Liu, J., Mu, H., Xiao, Y., Mei, B., Liu, W., Lin, G., Jiang, Z., Wen, L., & Jiang, L.
- Venue
- Angewandte Chemie International Edition
- Publisher
- Wiley
- Published
- 2019-12-02
- Volume
- 59
- Issue
- 4
- Pages
- 1659-1665
- ISSN
- 1433-7851 (ISSN-L)
- 1521-3773
- OpenAlex
- W2981908337
- Cited by
- 437
- References
- 7
- FWCI
- 8.14
- Type
- journal article
- Language
- en
- Open access
- closed
- Funders
- National Natural Science Foundation of China (21802080, 21625303)
- Natural Science Foundation of Shandong Province (ZR2019JQ05)
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- Shan, X., Liu, J., Mu, H., Xiao, Y., Mei, B., Liu, W., Lin, G., Jiang, Z., Wen, L., & Jiang, L. (2020). An Engineered Superhydrophilic/Superaerophobic Electrocatalyst Composed of the Supported CoMoSx Chalcogel for Overall Water Splitting. Angewandte Chemie International Edition. https://doi.org/10.1002/anie.201911617
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