Green Processing of Lignocellulosic Biomass and Its Derivatives in Deep Eutectic Solvents
Abstract
The scientific community has been seeking cost-competitive and green solvents with good dissolving capacity for the valorization of lignocellulosic biomass. At this point, deep eutectic solvents (DESs) are currently emerging as a new class of promising solvents that are generally liquid eutectic mixtures formed by self-association (or hydrogen-bonding interaction) of two or three components. DESs are attractive solvents for the fractionation (or pretreatment) of lignocellulose and the valorization of lignin, owing to the high solubility of lignin in DESs. DESs are also employed as effective media for the modification of cellulose to afford functionalized cellulosic materials, such as cellulose nanocrystals. More interestingly, biomassderived carbohydrates, such as fructose, can be used as one of the constituents of DESs and then dehydrated to 5-hydroxymethylfurfural in high yield. In this review, a comprehensive summary of recent contribution of DESs to the processing of lignocellulosic biomass and its derivatives is provided. Moreover, further discussion about the challenges of the application of DESs in biomass processing is presented.
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NADES have been suggested as alternatives to traditional volatile organic solvents in chemical processes such as carbon dioxide capture, biodiesel production, lignocellulose processing, electrolytes, biocatalysis, electrochemical detection, biodegradable reaction media, super absorbents, and soil washing.
“Therefore, in recent years they have been suggested as an alternative to traditional volatile organic solvents in chemical processes and applications such as: solvents for carbon dioxide capture (García et al. 2015;Mulia et al. 2016b), solvents for biodiesel production and processing lignocellulose (Tang et al. 2017;Taslim et al. 2016), as electrolytes (Gomez, Spisso, and Silva 2017), in biocataly”
From The perspectives of natural deep eutectic solvents in agri-food sector (2020) · cites this paper as Tang et al. 2017
DESs have been used as delignification agents owing to their ability to dissolve phenolic compounds.
“owing to the already well-known ability of DESs to dissolve phenolic compounds [29], DESs have been used as delignification agents [30].”
From Deep eutectic solvents: overcoming 21st century challenges (2019) · cites this paper as [30]
DESs with hydrophobic nature, low viscosity, and bearing kosmotropic anions or chaotropic cations enhance the activities and stabilities of enzymes.
“Commonly, DESs with hydrophobic nature, with low viscosity, and bearing kosmotropic anions or chaotropic cations enhance the activities and stabilities of enzymes [29,30].”
From Deep eutectic solvents: overcoming 21st century challenges (2019) · cites this paper as [30]
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Self-citation
- Authors
- Tang, X., Zuo, M., Li, Z., Liu, H., Xiong, C., Zeng, X., Sun, Y., Hu, L., Liu, S., Lei, T., & Lin, L.
- Affiliations
- Xiamen University (CN)
- Huaiyin Normal University (CN)
- State University of New York (US)
- Henan Key Lab of Biomass Energy Zhengzhou Henan 450008 P. R. China
- Corresponding author
- Zeng, Xianhai
- Lin, Lu
- Venue
- ChemSusChem
- Publisher
- Wiley
- Published
- 2017-05-23
- Volume
- 10
- Issue
- 13
- Pages
- 2696-2706
- ISSN
- 1864-5631 (ISSN-L)
- 1864-564X
- OpenAlex
- W2606717551
- Cited by
- 380
- References
- 105
- Citations by year
- 2026: 21 · 2025: 37 · 2024: 41 · 2023: 47 · 2022: 54 · 2021: 56 · 2020: 49 · 2019: 40 · 2018: 27 · 2017: 6 · 2016: 1
- FWCI
- 1.16
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- ChemSusChem (publishedVersion)
- PubMed (publishedVersion)
- Funders
- National Natural Science Foundation of China (21676223, 21506177)
- Topics
- Physical Sciences › Chemical Engineering › Catalysis › Ionic liquids properties and applications
- Physical Sciences › Engineering › Biomedical Engineering › Catalysis for Biomass Conversion
- Physical Sciences › Engineering › Biomedical Engineering › Biofuel production and bioconversion
- Keywords
- deep eutectic solvents, lignocellulosic biomass, lignin valorization, lignocellulosic biomass pretreatment, cellulose modification, cellulose nanocrystals, 5-hydroxymethylfurfural, fructose dehydration, biomass-derived carbohydrates, green solvents, hydrogen bonding
- MeSH terms
- Catalysis, Lignin, Solvents, Biomass, Green Chemistry Technology
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
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