Graphene paper supported MoS2 nanocrystals monolayer with Cu submicron-buds: High-performance flexible platform for sensing in sweat
Abstract
Flexible sweat biosensors are of considerable current interest for the development of wearable smart miniature devices. In this work, we report a novel type of flexible and electrochemical sweat platform fabricated by depositing Cu submicron buds on freestanding graphene paper (GP) carrying MoS 2 nanocrystals monolayer for bio-functional detection of glucose and lactate. Quantitative analysis of glucose and lactate was carried out by using amperometric i-t method. Linear ranges were obtained between 5 and 1775 μM for glucose and 0.01-18.4 mM for lactate, and their corresponding limits of detection were 500 nM and 0.1 μM, respectively. The platform demonstrates fast response, good selectivity, superb reproducibility and outstanding flexibility, which enable its use for monitoring glucose and lactate in human perspiration. The strategy of structurally integrating 3D transition metal, 0D transition metal sulfide and 2D graphene will provide new insight into the design of flexible electrodes for sweat glucose and lactate monitoring and a wider range of applications in biosensing, bioelectronics, and lab-on-a-chip devices.
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Various materials have been used as working electrodes, such as noble metals (Au and Ag), metallic oxides, graphene, and carbon black.
“Various materials have been used as working electrodes, such as noble metal (Au and Ag) (20–22), metallic oxides (23, 24), graphene (25, 26), and carbon black (27).”
From Integrated textile sensor patch for real-time and multiplex sweat analysis (2019) · cites this paper as [26]
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Shingange, K., Sharma, S., Makgwane, P. R., & Kumar, N. (2024) · Elsevier eBooks · doi:10.1016/b978-0-443-13464-7.00006-2 · Cited by 1 · see citing works
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Engineered Two-Dimensional Materials-Based Smart Biosensors for Point-of-Care Diagnosis
Surehkumar, K., Manjunath, K., Ramasami, A. K., & Ramakrishnappa, T. (2023) · Springer eBooks · doi:10.1007/978-981-19-9437-1_23 · Cited by 1 · see citing works
Applications of Nanomaterials in Biomedicine
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MoS2 for Nanoelectronic Device Applications (Transistor, Sensor, Photodetector)
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2D Materials’ Sensing Mechanisms
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A Low-Cost Nonenzymatic Sensor for Lactic Acid Detection Based on Graphene/CuO Nanocomposites
Holdefer, M. M. M., Bosenbecker, M., & Bertemes-Filho, P. (2026) · IEEE Sensors Letters · doi:10.1109/lsens.2026.3706720
- Authors
- Wang, Z., Dong, S., Gui, M., Asif, M., Wang, W., Wang, F., & Liu, H.
- Affiliations
- Huazhong University of Science and Technology (CN)
- Corresponding author
- Liu, Hongfang
- Venue
- Analytical Biochemistry
- Publisher
- Elsevier BV
- Published
- 2018-02
- Volume
- 543
- Pages
- 82-89
- ISSN
- 0003-2697 (ISSN-L)
- OpenAlex
- W2773230078
- Cited by
- 59
- References
- 50
- Citations by year
- 2026: 2 · 2025: 4 · 2024: 8 · 2023: 8 · 2022: 8 · 2021: 10 · 2020: 8 · 2019: 6 · 2018: 5
- FWCI
- 2.16
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Analytical Biochemistry (publishedVersion)
- PubMed (publishedVersion)
- Funders
- Huazhong University of Science and Technology (2015ZZGH010, 2015TS150)
- Topics
- Physical Sciences › Engineering › Electrical and Electronic Engineering › Electrochemical sensors and biosensors
- Physical Sciences › Engineering › Biomedical Engineering › Advanced Sensor and Energy Harvesting Materials
- Life Sciences › Biochemistry, Genetics and Molecular Biology › Molecular Biology › Advanced biosensing and bioanalysis techniques
- Keywords
- graphene paper, glucose detection, lactate detection, electrochemical biosensing, wearable devices, amperometric detection, sweat monitoring
- MeSH terms
- Copper, Disulfides, Glucose, Graphite, Molybdenum, Paper, Particle Size, Surface Properties, Sweat, Biosensing Techniques, Lactic Acid, Nanoparticles, Electrochemical Techniques
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