Sorption characteristics of N-nitrosodimethylamine onto biochar from aqueous solution
Abstract
N-nitrosodimethylamine (NDMA) is an emerging carcinogenic disinfection by-product in water environment. Biochars utilized as sorbents for the removal of NDMA from aqueous solution, and the sorption characteristics and mechanism were investigate. Biochars were prepared from bamboo, rice straw and wood sawdust at 300-700°C. The pseudo-second-order model provided the best fit for the sorption kinetics of NDMA onto biochar and the sorption isotherms were described best with the Slips model. Biochar produced at 500°C removed NDMA from aqueous solution relatively efficiently, and the bamboo char demonstrated the best sorption potential among the three types of biochars. Solution chemistry such as pH and metal ions did not show obvious effect on NDMA removal. Three sorption mechanisms are suggested for NDMA sorption onto biochars, H-bond attraction between -N=O and the O-containing moieties, hydrophobic force between -CH3 and the ordered graphitic structure, and partition process of NDMA into the non-carbonization part of biochar.
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Sorption of organic contaminants on biochar occurs by pore-filling, diffusion and partitioning, surface hydrophobic and hydrophilic interactions, aromatic and cation-π interactions, electrostatic interactions, and hydrogen bonding, or by a simultaneous occurrence of these mechanisms.
“occurs by: (a) pore-filling mechanisms (contributed by the majority of the surface area of biochar); (b) diffusion and partitioning mechanisms (effects of electrostatic interactions on the diffusion and equilibrium partitioning); (c) surface hydrophobic and hydrophilic inter-actions”
From Sustainable hybrid photocatalysts: titania immobilized on carbon materials derived from renewable and biodegradable resources (2016) · cites this paper as [108]
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- Authors
- Chen, C., Zhou, W., & Lin, D.
- Affiliations
- Zhejiang University (CN)
- Corresponding author
- Zhou, Wenjun
- Venue
- Bioresource Technology
- Publisher
- Elsevier BV
- Published
- 2015-03
- Volume
- 179
- Pages
- 359-366
- ISSN
- 0960-8524 (ISSN-L)
- OpenAlex
- W2019164335
- Cited by
- 88
- References
- 36
- Citations by year
- 2026: 2 · 2025: 5 · 2024: 8 · 2023: 3 · 2022: 8 · 2021: 8 · 2020: 7 · 2019: 10 · 2018: 14 · 2017: 7 · 2016: 12 · 2015: 4
- FWCI
- 5.82
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Bioresource Technology (publishedVersion)
- PubMed (publishedVersion)
- Funders
- National Basic Research Program of China (2014CB441103)
- Zhejiang Provincial Natural Science Foundation of China (LZ12B07001)
- National Natural Science Foundation of China (21137003)
- Topics
- Physical Sciences › Environmental Science › Water Science and Technology › Adsorption and biosorption for pollutant removal
- Physical Sciences › Environmental Science › Health, Toxicology and Mutagenesis › Water Treatment and Disinfection
- Physical Sciences › Engineering › Biomedical Engineering › Environmental remediation with nanomaterials
- Keywords
- N-nitrosodimethylamine, biochar, sorption, disinfection by-products, water treatment, rice straw, sawdust, sorption kinetics, pseudo-second-order kinetics, sorption isotherms, sorption mechanism, hydrogen bonding, hydrophobic interactions, partitioning, pH effect, metal ions
- MeSH terms
- Adsorption, Charcoal, Dimethylnitrosamine, Elements, Hydrogen-Ion Concentration, Ions, Kinetics, Metals, Solutions, Temperature, Time Factors, Water Pollutants, Chemical
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