Cited by 122High Entropy Alloys StudiesPhysics of Superconductivity and MagnetismSuperconducting Materials and Applications

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Sc–Zr–Nb–Rh–Pd and Sc–Zr–Nb–Ta–Rh–Pd High-Entropy Alloy Superconductors on a CsCl-Type Lattice

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Stolze, Karoline, Tao, Jing, von Rohr, Fabian O., Kong, Tai, Cava, Robert J.·2018·Chemistry of Materials

DOI 10.1021/acs.chemmater.7b04578

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Abstract

We have synthesized previously unreported high-entropy alloys (HEAs) in the pentanary (ScZrNb) 1– x [RhPd] x and hexanary (ScZrNbTa) 1– x [RhPd] x systems. The materials have CsCl-type structures and mixed site occupancies. Both HEAs are type-II superconductors with strongly varying critical temperatures ( T c ’s) depending on the valence electron count (VEC); the T c ’s increase monotonically with decreasing VEC within each series, and do not follow the trends seen for either crystalline or amorphous transition metal superconductors. The (ScZrNb) 0.65 [RhPd] 0.35 HEA with the highest T c, ∼9.3 K, also exhibits the largest μ 0 H c2 (0) = 10.7 T. The pentanary and hexanary HEAs have higher superconducting transition temperatures than their simple binary intermetallic relatives with the CsCl-type structure and a surprisingly ductile mechanical behavior. The presence of niobium, even at the 20% level, has a positive impact on the T c . Nevertheless, niobium-free (ScZr) 0.50 [RhPd] 0.50, as mother-compound of both superconducting HEAs found here, is itself superconducting, proving that superconductivity is an intrinsic feature of the bulk material.

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Authors: Stolze, K., Tao, J., von Rohr, F. O., Kong, T., & Cava, R. J.
Affiliations: Princeton University (US)
Brookhaven National Laboratory (US)
Department of Chemistry, University of Zürich, CH-8057 Zürich, Switzerland
Corresponding author: Stolze, Karoline
Cava, Robert J.
ORCID: Stolze, Karoline
Tao, Jing
Kong, Tai
Cava, Robert J.
Venue: Chemistry of Materials
Publisher: American Chemical Society (ACS)
Published: 2018-02-02
Volume: 30
Issue: 3
Pages: 906-914
ISSN: 0897-4756 (ISSN-L)
1520-5002
DOI: 10.1021/acs.chemmater.7b04578
OpenAlex: W2783348740
Cited by: 122
References: 37
Citations by year: 2026: 4 · 2025: 20 · 2024: 18 · 2023: 17 · 2022: 26 · 2021: 15 · 2020: 13 · 2019: 6 · 2018: 3
FWCI: 5.91
Type: journal article
Language: en
Open access: green
www.osti.gov
Locations: Chemistry of Materials (publishedVersion)
Archive ouverte UNIGE (University of Geneva) (publishedVersion)
OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
Archive ouverte UNIGE (University of Geneva) (submittedVersion, cc-by)
Zurich Open Repository and Archive (University of Zurich) (submittedVersion)
Funders: Gordon and Betty Moore Foundation (GBMF-4412)
Basic Energy Sciences (DE-SC0012704)
Topics: Physical Sciences › Engineering › Mechanical Engineering › High Entropy Alloys Studies
Physical Sciences › Physics and Astronomy › Condensed Matter Physics › Physics of Superconductivity and Magnetism
Physical Sciences › Engineering › Electrical and Electronic Engineering › Superconducting Materials and Applications
Keywords: high-entropy alloys, superconductors, B2 phase, critical temperature, valence electron count, type-II superconductivity, upper critical field, ductility, niobium effect, intermetallic compounds, transition metal superconductors

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Sc–Zr–Nb–Rh–Pd and Sc–Zr–Nb–Ta–Rh–Pd High-Entropy Alloy Superconductors on a CsCl-Type Lattice

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