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Tuning the Morphology of g-C3N4 for Improvement of Z-Scheme Photocatalytic Water Oxidation
Abstract
Solar-driven water oxidation is the key step for overall water splitting that efficiently harvests and converts solar energy into fuels; the development of a highly efficient photocatalyst that can mediate water oxidation has become an appealing challenge. Herein, we report a facile two-step process to decorate silver phosphate (Ag3PO4) particles on different types of graphitic carbon nitrides (g-C3N4) as composite photocatalysts for water oxidation. For all the Ag3PO4/g-C3N4 materials, an in situ Z-scheme is created by the generation of Ag nanoparticles which act as a cross-linking bridge between Ag3PO4 and g-C3N4 in the composite, resulting in better charge separation and higher catalytic performance. A detailed analysis emphasizes the importance of the g-C3N4 on the chemical, photophysical, and catalytic properties of the composite materials. Our results show that the alteration of the morphology dominates the performance of the composite materials.
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Metadata
- Authors
- Yang, X., Chen, Z., Xu, J., Tang, H., Chen, K., & Jiang, Y.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2015-07-09
- Volume
- 7
- Issue
- 28
- Pages
- 15285-15293
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W1166945226
- Cited by
- 283
- References
- 44
- FWCI
- 11.54
- Type
- journal article
- Language
- en
- Open access
- closed
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