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Carbon-Based CsPbBr3 Perovskite Solar Cells: All-Ambient Processes and High Thermal Stability
Abstract
The device instability has been an important issue for hybrid organic–inorganic halide perovskite solar cells (PSCs). This work intends to address this issue by exploiting inorganic perovskite (CsPbBr 3 ) as light absorber, accompanied by replacing organic hole transport materials (HTM) and the metal electrode with a carbon electrode. All the fabrication processes (including those for CsPbBr 3 and the carbon electrode) in the PSCs are conducted in ambient atmosphere. Through a systematical optimization on the fabrication processes of CsPbBr 3 film, carbon-based PSCs (C-PSCs) obtained the highest power conversion efficiency (PCE) of about 5.0%, a relatively high value for inorganic perovskite-based PSCs. More importantly, after storage for 250 h at 80 °C, only 11.7% loss in PCE is observed for CsPbBr 3 C-PSCs, significantly lower than that for popular CH 3 NH 3 PbI 3 C-PSCs (59.0%) and other reported PSCs, which indicated a promising thermal stability of CsPbBr 3 C-PSCs.
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Metadata
- Authors
- Chang, X., Li, W., Zhu, L., Liu, H., Geng, H., Xiang, S., Liu, J., & Chen, H.
- Venue
- ACS Applied Materials & Interfaces
- Publisher
- American Chemical Society (ACS)
- Published
- 2016-12-01
- Volume
- 8
- Issue
- 49
- Pages
- 33649-33655
- ISSN
- 1944-8244 (ISSN-L)
- 1944-8252
- OpenAlex
- W2554212518
- Cited by
- 285
- References
- 42
- FWCI
- 16.77
- Type
- journal article
- Language
- en
- Open access
- closed
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