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Template-Directed Materials for Rechargeable Lithium-Ion Batteries
Abstract
Extensive research activities have been directed to develop flexible rechargeable lithium-ion batteries with large capacity, high power, and long cycling life. Template technology offers the benefits in terms of either designing new-type electrode materials or modifying traditional battery configurations. With the aid of “hard” or “soft” templates, a variety of functional materials with diverse structures and morphologies such as one-dimensional (1D) nanostructures, 2D films, and 3D porous frameworks have been synthesized. This review highlights the recent progress in the template-prepared electrode materials for lithium storage, mainly focusing on the Li + intercalation reactions and the Li conversion properties with the nanostructures of LiCoO 2, C, SnO 2, Fe 2 O 3, Co 3 O 4, VO x, and MnO 2 . In some specifically demonstrated examples, the templated cathode materials (e.g., lithium metal oxides) show significantly improved reversibility and high rate capability over a voltage of 3 V after 100 cycles, whereas the templated anode materials (e.g., metal oxides) can deliver high capacity exceeding 1000 mA h g −1 . The structural and morphological merits of the template-directed materials have been especially addressed in comparison with their traditional bulk forms.
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Metadata
- Authors
- Cheng, F., Tao, Z., Liang, J., & Chen, J.
- Venue
- Chemistry of Materials
- Publisher
- American Chemical Society (ACS)
- Published
- 2007-12-28
- Volume
- 20
- Issue
- 3
- Pages
- 667-681
- ISSN
- 0897-4756 (ISSN-L)
- 1520-5002
- OpenAlex
- W2077511701
- Cited by
- 537
- References
- 73
- FWCI
- 23.63
- Type
- journal article
- Language
- en
- Open access
- closed
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