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Metal–Organic Framework Based upon the Synergy of a Brønsted Acid Framework and Lewis Acid Centers as a Highly Efficient Heterogeneous Catalyst for Fixed-Bed Reactions

Li, Baiyan, Leng, Kunyue, Zhang, Yiming, Dynes, James J., Wang, Jian, Hu, Yongfeng, Ma, Dingxuan, Shi, Zhan, Zhu, Liangkui, Zhang, Daliang, Sun, Yinyong, Chrzanowski, Matthew, Ma, Shengqian·2015·Journal of the American Chemical Society

DOI 10.1021/jacs.5b01352

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Abstract

We report a strategy of combining a Brønsted acid metal-organic framework (MOF) with Lewis acid centers to afford a Lewis acid@Brønsted acid MOF with high catalytic activity, as exemplified in the context of MIL-101-Cr-SO3H·Al(III). Because of the synergy between the Brønsted acid framework and the Al(III) Lewis acid centers, MIL-101-Cr-SO3H·Al(III) demonstrates excellent catalytic performance in a series of fixed-bed reactions, outperforming two benchmark zeolite catalysts (H-Beta and HMOR). Our work therefore not only provides a new approach to achieve high catalytic activity in MOFs but also paves a way to develop MOFs as a new type of highly efficient heterogeneous catalysts for fixed-bed reactions.

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See all 264

Authors: Li, B., Leng, K., Zhang, Y., Dynes, J. J., Wang, J., Hu, Y., Ma, D., Shi, Z., Zhu, L., Zhang, D., Sun, Y., Chrzanowski, M., & Ma, S.
Venue: Journal of the American Chemical Society
Publisher: American Chemical Society (ACS)
Published: 2015-03-23
Volume: 137
Issue: 12
Pages: 4243-4248
ISSN: 0002-7863 (ISSN-L)
1520-5126
DOI: 10.1021/jacs.5b01352
OpenAlex: W2112225100
Cited by: 264
References: 71
FWCI: 16.63
Type: journal article
Language: en
Open access: closed

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Metal–Organic Framework Based upon the Synergy of a Brønsted Acid Framework and Lewis Acid Centers as a Highly Efficient Heterogeneous Catalyst for Fixed-Bed Reactions

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