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Ruthenium-Based Electrocatalysts Supported on Reduced Graphene Oxide for Lithium-Air Batteries
Abstract
Ruthenium-based nanomaterials supported on reduced graphene oxide (rGO) have been investigated as air cathodes in non-aqueous electrolyte Li-air cells using a TEGDME-LiCF3SO3 electrolyte. Homogeneously distributed metallic ruthenium and hydrated ruthenium oxide (RuO2·0.64H2O), deposited exclusively on rGO, have been synthesized with average size below 2.5 nm. The synthesized hybrid materials of Ru-based nanoparticles supported on rGO efficiently functioned as electrocatalysts for Li2O2 oxidation reactions, maintaining cycling stability for 30 cycles without sign of TEGDME-LiCF3SO3 electrolyte decomposition. Specifically, RuO2·0.64H2O-rGO hybrids were superior to Ru-rGO hybrids in catalyzing the OER reaction, significantly reducing the average charge potential to ∼3.7 V at the high current density of 500 mA g(-1) and high specific capacity of 5000 mAh g(-1).
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Metadata
- Authors
- Jung, H.-G., Jeong, Y. S., Park, J.-B., Sun, Y.-K., Scrosati, B., & Lee, Y. J.
- Venue
- ACS Nano
- Publisher
- American Chemical Society (ACS)
- Published
- 2013-04-05
- Volume
- 7
- Issue
- 4
- Pages
- 3532-3539
- ISSN
- 1936-0851 (ISSN-L)
- 1936-086X
- OpenAlex
- W2330909815
- Cited by
- 382
- References
- 41
- FWCI
- 37.15
- Type
- journal article
- Language
- en
- Open access
- closed
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