Electronically programmable photonic molecule
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Written from the paper’s full text.
TL;DR
The paper demonstrates an electronically programmable photonic molecule made from two coupled lithium niobate microring resonators, with microwave control of two optical energy levels. It observes atomic-like two-level dynamics and uses bright-dark mode reconfiguration for on-demand photon storage and retrieval.
Key findings
- A pair of 80 µm radius coupled lithium niobate microrings forms a photonic molecule with two modes separated by \(2\mu = 2\pi \times 7\) GHz and linewidths \(\gamma = 2\pi \times 96\) MHz, corresponding to a loaded optical quality factor of \(1.9 \times 10^6\).
- Microwave and DC electric fields coherently control the system: DC Stark tuning gives \(g = 2\pi \times 0.5\) GHz/V, and microwave driving produces Autler-Townes splitting, AC Stark shift, Rabi oscillation, and Ramsey interference.
- For a peak drive voltage \(V_p = 1.1\) V, coherent Rabi oscillation is observed at 1.1 GHz, which is 16% of the initial mode splitting; the optical coherence time is \(\sim 1.6\) ns for both Rabi and Ramsey oscillations, in agreement with cavity decay.
- Reconfiguring the molecule into bright and dark modes enables deterministic photon storage and retrieval, with a measured dark-mode lifetime of 2 ns, about twice the lifetime of the critically coupled bright mode.
Methods
- Devices are fabricated on thin-film lithium niobate: coupled microring resonators with gold microwave electrodes placed 2.5 µm from the ring edge for differential driving; 60 programmable photonic molecules are patterned on a 10 mm by 8 mm chip.
- Measurements use a tunable telecom laser, an arbitrary waveform generator and amplifiers for microwave control, DC bias up to ±15 V, and fast photodetection for Rabi, Ramsey, and storage/retrieval experiments.
- The dynamics are analyzed with a Hamiltonian and input-output theory, including rotating-wave approximation, Autler-Townes splitting, AC Stark shift, and Bloch-sphere descriptions of Rabi and Ramsey oscillations.
Limitations
- The paper states that the phase coherence time of the two energy levels is dominated by cavity dissipation (\(\sim 1.6\) ns), since the optical lifetime is much shorter than the laser coherence time (\(\sim \mu\)s); longer storage would require over-coupled bright modes and improved resonator quality factors toward the material limit (\(>10^9\)).
- Evident from the text: the demonstration uses continuous-wave laser fields and classical optical readout, while quantum single-photon operation is discussed only as a future application, not demonstrated.
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Claims the paper makes
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- Findingown data§ Electronically Programmable Photonic Molecule · p. 1
Ramsey interference is observed in the photonic molecule.
“We show signature two-level dynamics including microwave induced photonic Autler-Townes splitting, Stark shift, Rabi oscillation and Ramsey interference.”
- Also stated in: § Electronically Programmable Photonic Molecule · p. 3 · plain
“we measure photonic Ramsey interference by driving the system with detuned microwave pulses at 7.8 GHz.”
Quote in the paperSubstantial claim - Also stated in: § Electronically Programmable Photonic Molecule · p. 3 · plain
- Findingown data§ Electronically Programmable Photonic Molecule · p. 1
On-demand photon storage and retrieval is achieved in optical microresonators by reconfiguring the photonic molecule into a bright-dark mode pair.
“Leveraging the coherent control of optical energy, we show on-demand photon storage and retrieval in optical microresonators by reconfiguring the photonic molecule into a bright-dark mode pair.”
- Also stated in: § Electronically Programmable Photonic Molecule · p. 5 · plain
“Light can be deterministically stored and retrieved using the bright-dark mode pair and microwave control.”
Quote in the paperSubstantial claim - Also stated in: § Electronically Programmable Photonic Molecule · p. 5 · plain
- Findingown data§ Electronically Programmable Photonic Molecule · p. 2
The photonic molecule supports a pair of well-defined optical energy levels, evident from optical transmission measured using a tuneable telecom wavelength laser.
“The photonic molecule supports a pair of well-defined optical energy levels, which are evident from the optical transmission measured using a tuneable telecom wavelength laser (Fig. 1c; also, see Supplementary for full spectrum).”
Quote in the paperSubstantial claim - Findingown data§ Electronically Programmable Photonic Molecule · p. 1
Photonic AC Stark shift is observed in the photonic molecule.
“We show signature two-level dynamics including microwave induced photonic Autler-Townes splitting, Stark shift, Rabi oscillation and Ramsey interference.”
- Also stated in: § Electronically Programmable Photonic Molecule · p. 3 · plain
“When the microwave frequency is far detuned from the transition frequency, an effective dispersive effect in the level splitting is induced, analogous to the AC Stark shift in atomic systems (Fig. 2c).”
Quote in the paperSubstantial claim - Also stated in: § Electronically Programmable Photonic Molecule · p. 3 · plain
- Findingown data§ Electronically Programmable Photonic Molecule · p. 1
Rabi oscillation is observed in the photonic molecule.
“We show signature two-level dynamics including microwave induced photonic Autler-Townes splitting, Stark shift, Rabi oscillation and Ramsey interference.”
- Also stated in: § Electronically Programmable Photonic Molecule · p. 3 · plain
“In particular, for a peak drive voltage of V p = 1 . 1 V, we observe coherent Rabi oscillation with a frequency of 1.1 GHz, being 16% of the initial mode splitting.”
Quote in the paperSubstantial claim - Also stated in: § Electronically Programmable Photonic Molecule · p. 3 · plain
- Findingown data§ Electronically Programmable Photonic Molecule · p. 2
A microwave-optical coupling efficiency of g = 2π × 0.5 GHz/V is extracted from the asymptote of the anti-crossing.
“From the asymptote of the anti-crossing, a microwave-optical coupling efficiency of g = 2 π × 0 . 5 GHz/V is extracted.”
Quote in the paperSubstantial claim - Findingreasoning§ Electronically Programmable Photonic Molecule · p. 2
The extracted tuning/modulation efficiency g = 2π × 0.5 GHz/V is an order of magnitude larger than previously demonstrated in bulk electro-optic resonator systems.
“The extracted tuning/modulation efficiency g = 2 π × 0 . 5 GHz/V is an order of magnitude larger than previously demonstrated in bulk electro-optic resonator systems [32, 33]”
Quote in the paperNot a substantial claim0 of 2 sources checked- cites [32] Guarino, A., Poberaj, G., Rezzonico, D., Degl'Innocenti, R. & Gunter, P. Electro-optically tunable microring resonators in lithium niobate. Nat Photon. 1, 407–410 (2007). source
Not checked in the free run.
- cites [33] Witmer, J. D. et al. High-Q photonic resonators and electro-optic coupling using silicon-on-lithium-niobate. Sci. Rep. 7, 46313 (2017). source
Not checked in the free run.
- Findingown data§ Electronically Programmable Photonic Molecule · p. 1
Microwave-induced photonic Autler-Townes splitting is observed in the photonic molecule.
“We show signature two-level dynamics including microwave induced photonic Autler-Townes splitting”
- Also stated in: § Electronically Programmable Photonic Molecule · p. 3 · plain
“leading to microwave-induced photonic Autler-Townes splitting (Rabi splitting), shown in Fig. 2a.”
Quote in the paperSubstantial claim - Also stated in: § Electronically Programmable Photonic Molecule · p. 3 · plain
- Findingnone given§ Electronically Programmable Photonic Molecule · p. 4
Optical access to the dark optical mode can be granted by applying a microwave signal with frequency matched to the difference between the two optical modes.
“Notably, optical access to the dark optical mode can be granted by applying a microwave signal with frequency matched to the difference between the two optical modes (Fig. 4a).”
Quote in the paperSubstantial claim - Findingreasoning§ Electronically Programmable Photonic Molecule · p. 4
A large DC bias voltage (15 V) reconfigures the photonic molecule into a pair of bright and dark modes.
“To achieve this, we apply a large DC bias voltage (15 V) to reconfigure the photonic molecule into a pair of bright and dark modes.”
- Also stated in: § Electronically Programmable Photonic Molecule · p. 5 · plain
“The photonic molecule is programmed so that the resonance frequency of ring 1 is different from ring 2, resulting in bright and dark modes.”
Quote in the paperSubstantial claim - Also stated in: § Electronically Programmable Photonic Molecule · p. 5 · plain
- Findingown data§ Electronically Programmable Photonic Molecule · p. 2
Applying a DC bias voltage in the range of ±15 V to the microwave electrodes results in an avoided crossing curve.
“This is accomplished by applying a DC bias voltage in the range of ± 15 V to the microwave electrodes, which results in an avoided crossing curve shown in figure 1d.”
Quote in the paperSubstantial claim - Findingown data§ II. DEVICE AND EXPERIMENTAL SETUP DETAILS · p. 8
The normalized transmission spectrum of the photonic molecule shows pairs of two-level resonances separated by the free-spectral-range of the microring resonator (~2.2 nm).
“Figure S3 shows the normalized transmission spectrum of the photonic molecule, showing pairs of two-level resonances separated by the free-spectral-range of the microring resonator ( ∼ 2.2 nm).”
Quote in the paperNot a substantial claim - Findingown data§ Electronically Programmable Photonic Molecule · p. 2
The energy levels of the photonic molecule can be programmed by applying a DC electric field, equivalent to a DC Stark shift used to control energy levels in an atom.
“Building on this analogy, we show that the energy levels of the photonic molecule can be programmed by applying a direct current (DC) electric field, the effect equivalent to a DC Stark shift used to control the energy levels in an atom.”
Quote in the paperSubstantial claim - Findingown data§ D. Optical two-level dynamics · p. 11
Rabi oscillation was measured in real-time as the microwave signal is turned on.
“Rabi oscillation is measured in real-time as the microwave signal is turned on.”
Quote in the paperNot a substantial claim - Findingown data§ Electronically Programmable Photonic Molecule · p. 4
The microwave modulation results in an effective coupling between the bright and the dark mode, directly observed from the avoided crossing in the spectrum of the bright optical mode.
“The microwave modulation results in an effective coupling between the bright and the dark mode, which we directly observe from the avoided crossing in the spectrum of the bright optical mode (Fig. 4b).”
- Also stated in: § Electronically Programmable Photonic Molecule · p. 5 · hedged
“A microwave field applied to the system can induce an effective coupling between bright and dark modes, indicated by the avoided crossing observed in the optical transmission spectrum.”
Quote in the paperSubstantial claim - Also stated in: § Electronically Programmable Photonic Molecule · p. 5 · hedged
- Findingown data§ Electronically Programmable Photonic Molecule · p. 3
The splitting frequency Ω can be precisely controlled up to several gigahertz by controlling the amplitude of the microwave signals.
“In our system, the splitting frequency (Ω) can be precisely controlled up to several gigahertz by controlling the amplitude of the microwave signals (Fig. 2b).”
Quote in the paperSubstantial claim - Findingown data§ Electronically Programmable Photonic Molecule · p. 3
The photonic molecule can be used for unitary transformation of light in the frequency domain using Rabi oscillation and Ramsey interference.
“We demonstrate the photonic molecule can be used for unitary transformation of light in the frequency domain using Rabi oscillation and Ramsey interference (see Supplementary).”
Quote in the paperSubstantial claim - Findingown data§ Electronically Programmable Photonic Molecule · p. 5
The retrieved light from the dark mode measured at different time delays shows nearly twice the lifetime of the critically coupled bright mode.
“The retrieved light from the dark mode measured at different time delays. Inset: the extracted intensity of the retrieved light shows nearly twice the lifetime of the critically coupled bright mode.”
Quote in the paperSubstantial claim - Premisereasoning§ Electronically Programmable Photonic Molecule · p. 1
Conventional integrated photonic platforms have not been able to meet the requirements of long photon lifetime and fast modulation simultaneously.
“On the other hand, conventional integrated photonic platforms have not been able to meet the requirements of long photon lifetime and fast modulation simultaneously.”
Quote in the paperSubstantial claim - Interpretationreasoning§ Electronically Programmable Photonic Molecule · p. 3
The dispersive effect can be used to control the effective coupling strength between the energy levels of the photonic molecule, which are otherwise determined by geometric factors.
“Importantly, this effect can be used to control the effective coupling strength between the energy levels of the photonic molecule, which are otherwise determined by geometric factors.”
Quote in the paperSubstantial claim - Premisenone given§ Electronically Programmable Photonic Molecule · p. 4
To enable controllable write and read of photons into a resonator and from an external waveguide, the optical coupling strength needs to be altered faster than the cavity photon lifetime.
“To enable controllable write and read of photons into a resonator and from an external waveguide, the optical coupling strength needs to be altered faster than the cavity photon lifetime.”
Quote in the paperNot a substantial claim - Interpretationcitation§ Electronically Programmable Photonic Molecule · p. 2
The large tuning/modulation efficiency is due to the highly efficient overlap between microwave and optical fields enabled by the system.
“and is due to the highly efficient overlap between microwave and optical fields enabled by our system [34].”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [34] Rueda, A. et al. Efficient microwave to optical photon conversion: an electro-optical realization. Optica 3, 597–604 (2016). source
Not checked in the free run.
- Interpretationreasoning§ C. Autler-Townes Splitting and AC Stark Shifts · p. 9
Under continuous wave microwave modulation with frequency close to the optical two-mode splitting, each resonance of c1, c2 splits into two dips with splitting frequency W.
“Under a continuous wave microwave modulation with frequency close to the optical two-mode splitting, each resonance of c 1 , c 2 will further split into two dips with splitting frequency”
Quote in the paperSubstantial claim- The authors state this as an assumption: The nanophotonic two-level system under a coherent microwave drive can be described by the given Hamiltonian.
- Interpretationreasoning§ Electronically Programmable Photonic Molecule · p. 2
The electro-optic effect plays the role equivalent to that of an electric dipole moment in an atomic two-level system, where in both systems external electromagnetic fields are used to couple and address the energy levels.
“We note that in our system the electro-optic effect plays the role equivalent to that of an electric dipole moment in the case of an atomic two-level systems, where in both systems external electromagnetic fields are used to couple and address the energy levels.”
Quote in the paperSubstantial claim - Premiseown data§ Electronically Programmable Photonic Molecule · p. 2
When the optical coupling strength μ exceeds the optical loss rate γ of each cavity, the coupling leads to a normal mode splitting resulting in a frequency doublet consisting of a lower frequency symmetric (S) and a higher frequency antisymmetric (AS) optical mode.
“When the optical coupling strength µ exceeds the optical loss rate γ of each cavity, the coupling leads to a normal mode splitting resulting in a frequency doublet consisting of a lower frequency symmetric (S) and a higher frequency antisymmetric (AS) optical mode (Fig. 1a and c).”
Quote in the paperSubstantial claim - Premisecitation§ Electronically Programmable Photonic Molecule · p. 1
Ultra-high Q on-chip resonators have traditionally been realized in passive materials, such as silicon dioxide and silicon nitride, which can only be controlled electrically using slow thermal effect.
“On the other hand, ultra-high Q on-chip resonators have traditionally been realized in passive materials, such as silicon dioxide (SiO 2 ) [24, 25] and silicon nitride (Si 3 N 4 ) [26, 27], which can only be controlled electrically using slow thermal effect.”
Quote in the paperSubstantial claim0 of 4 sources checked- cites [24] Spreeuw, R. J. C., van Druten, N. J., Beijersbergen, M. W., Eliel, E. R. & Woerdman, J. P. Classical realization of a strongly driven two-level system. Phys. Rev. Lett. 65, 2642–2645 (1990). source
Not checked in the free run.
- cites [25] Karpiński, M., Jachura, M., Wright, L. J. & Smith, B. J. Bandwidth manipulation of quantum light by an electro-optic time lens. Nat. Photon. 11, 53–57 (2017). source
Not checked in the free run.
- cites [26] Armani, D. K., Kippenberg, T. J., Spillane, S. M. & Vahala, K. J. Ultra-high-Q toroid microcavity on a chip. Nature 421, 925–928 (2003). source
Not checked in the free run.
- cites [27] Lee, H. et al. Chemically etched ultrahigh-Q wedge-resonator on a silicon chip. Nat. Photon. 6, 369–373 (2012). source
Not checked in the free run.
- Premisereasoning§ Electronically Programmable Photonic Molecule · p. 1
A coherent photonic two-level system that can be programmed and dynamically controlled is still missing.
“However, the fundamental building block, a coherent photonic two-level system that can be programmed and dynamically controlled, is still missing.”
Quote in the paperSubstantial claim0 of 3 sources checked- cites [12] Chen, W., Özdemir, Ş. K., Zhao, G., Wiersig, J. & Yang, L. Exceptional points enhance sensing in an optical microcavity. Nature 548, 192–196 (2017). source
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- cites [13] O’Brien, J. L. Optical quantum computing. Science 318, 1567–1570 (2007). source
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- cites [14] Ramelow, S. et al. Strong nonlinear coupling due to induced photon interaction on a Si3N4 chip. Preprint at https://arxiv.org/abs/1802.10072 (2018).
Not checked in the free run.
- Interpretationreasoning§ Electronically Programmable Photonic Molecule · p. 2
The two new eigenmodes, separated in frequency by the optical coupling strength, are the energy states of the photonic molecule.
“The two new eigenmodes, separated in frequency by the optical coupling strength, are the energy states of the photonic molecule.”
Quote in the paperSubstantial claim - Interpretationreasoning§ Electronically Programmable Photonic Molecule · p. 3
The applied microwave signal drives a sequence of resonance enhanced sum- and difference-frequency generation (SFG and DFG) processes that result in energy of photons being changed several times (more than 10) before dissipation.
“In other words, using the language of nonlinear optics, applied microwave signal drives a sequence of resonance enhanced sum- and differencefrequency generation (SFG and DFG) processes that result in energy of photons being changed several times (more than 10 in Fig. 3c) before it is eventually dissipated due to the cavity photon loss (cavity life time ∼ 1.6 ns).”
Quote in the paperSubstantial claim - Study design and conductnone given§ Electronically Programmable Photonic Molecule · p. 4
The waveguide coupling is designed to be critically-coupled to a single resonator maximizing the transmission extinction ratio.
“In our experiment, the waveguide coupling is designed to be critically-coupled to a single resonator maximizing the transmission extinction ratio.”
Quote in the paperSubstantial claim - Interpretationown data§ Electronically Programmable Photonic Molecule · p. 2
The two optical energy levels are formed by the evanescent coupling of light from one resonator to another through a 500-nm gap.
“The two optical energy levels are formed by the evanescent coupling of light from one resonator to another through a 500-nm gap.”
Quote in the paperSubstantial claim - Interpretationnone given§ Electronically Programmable Photonic Molecule · p. 3
The number of photons that could populate each of the two levels is not limited to one, resembling an atomic ensemble.
“This situation is similar to an atomic two-level system under a strong coherent excitation, with an important difference that in our case the number of photons that could populate each of the two levels is not limited to one, resembling that of an atomic ensemble.”
Quote in the paperNot a substantial claim - Interpretationreasoning§ D. Optical two-level dynamics · p. 11
The oscillation of the output signal rotating at frequency δ corresponds to the population of c1 after dropping the fast rotating terms related to c2.
“So the oscillation of the output signal P out = ∣ ∣ ∣ s + √ γ ex / 2( c 1 + c 2 e iω m t ) ∣ ∣ ∣ 2 rotating at with the frequency δ corresponds to the population of c 1 after dropping the fast rotating terms related to c 2 .”
Quote in the paperNot a substantial claim- The authors state this as an assumption: The nanophotonic two-level system under a coherent microwave drive can be described by the given Hamiltonian.
- Interpretationreasoning§ E. Optical dark modes · p. 12
π-pulse control sequences can be implemented to achieve on-demand photon-storage and retrieval.
“Therefore, π -pulse control sequences can be implemented as described in the main text to achieve the on-demand photon-storage and retrieval.”
Quote in the paperSubstantial claim- The authors state this as an assumption: The nanophotonic two-level system under a coherent microwave drive can be described by the given Hamiltonian.
- May combine two claims. 26
- The quote only partly states this claim. 1
- Classified as probably not a substantial claim. 3
May combine two claims.
Findingown data§ Electronically Programmable Photonic Molecule · p. 2The two optical modes are separated by 2μ = 2π × 7 GHz and have cavity linewidths of γ = 2π × 96 MHz, corresponding to a loaded (intrinsic) quality factor of Q = 1.9×10^6 (Q_i = 2.5×10^6).
“In our case, the two optical modes are separated by 2 µ = 2 π × 7 GHz and have cavity linewidths of γ = 2 π × 96 MHz, corresponding to a loaded (intrinsic) quality factors of Q = 1 . 9 × 10 6 ( Q i = 2 . 5 × 10 6 ), thus forming a wellresolved two-level system (Fig. 1c).”
Quote in the paperSubstantial claimMay combine two claims.
Findingown data§ Electronically Programmable Photonic Molecule · p. 2The DC Stark effect can be achieved by applying a DC electric field to the two-level system, blue-shifting one ring and red-shifting the other, resulting in an anti-crossing curve due to optical coupling.
“DC Stark effect can be achieved by applying a DC electric field to the two-level system. The DC field blue-shifts one ring and red-shifts the other one. The resulting transmission spectra show an anti-crossing curve due to the optical coupling between the two rings.”
Quote in the paperSubstantial claimMay combine two claims.
Findingown data§ Electronically Programmable Photonic Molecule · p. 1The authors demonstrate a photonic molecule with two distinct energy levels and control it by external microwave excitation.
“In this work, we demonstrate a photonic molecule with two distinct energy-levels and control it by external microwave excitation.”
- Also stated in: § Electronically Programmable Photonic Molecule · p. 1 · plain
“In this work, we overcome the existing performance trade-off paradigm and realize a programmable photonic two-level system that can be dynamically controlled using gigahertz microwave signals (Fig. 1a).”
Quote in the paperSubstantial claim- Also stated in: § Electronically Programmable Photonic Molecule · p. 1 · plain
May combine two claims. The quote only partly states this claim.
Findingown data§ Electronically Programmable Photonic Molecule · p. 4The observed Rabi oscillation and Ramsey interference are in excellent agreement with theoretical predictions.
“The measurements are in excellent agreement with theoretical predictions (see Supplementary).”
Quote in the paperSubstantial claimMay combine two claims.
Findingnone given§ Electronically Programmable Photonic Molecule · p. 5The paper demonstrated coherent and dynamic control of a two-level photonic molecule with microwave fields and on-demand photon storage and retrieval.
“Our demonstration of the coherent and dynamic control of a two-level photonic molecule with microwave fields and on-demand photon storage and retrieval paves a path to a new paradigm of control over photons.”
Quote in the paperSubstantial claimMay combine two claims.
Findingreasoning§ Electronically Programmable Photonic Molecule · p. 2The S (AS) mode spatially spans both optical cavities, with the light in the two cavities being in- (out-of-) phase.
“The S (AS) mode spatially spans both optical cavities, with the light in the two cavities being in- (out-of-) phase.”
Quote in the paperSubstantial claimMay combine two claims.
Findingown data§ Electronically Programmable Photonic Molecule · p. 4In the bright-dark mode limit, one mode is mainly localized in the first ring and is optically bright and accessible to the input optical waveguide, while the other mode is mainly localized in the second ring and is optically dark and decoupled from the input optical waveguide by geometry.
“In this limit, one of the modes is mainly localized in the 1st ring (purple in Fig. 4a), and thus is still accessible to the input optical waveguide and is optically bright, while the other mode is mainly localized in the 2nd ring (black in Fig. 4a) and thus is decoupled from the input optical waveguide by geometry and becomes optically dark (See Supplementary for details).”
- Also stated in: § Electronically Programmable Photonic Molecule · p. 5 · plain
“As a result, bright mode can be accessed from the optical waveguide, while the dark mode cannot (forbidden by geometry).”
Quote in the paperSubstantial claim- Also stated in: § Electronically Programmable Photonic Molecule · p. 5 · plain
May combine two claims.
Findingown data§ Electronically Programmable Photonic Molecule · p. 3A large range of Rabi frequencies is achievable with low applied voltages, in excellent agreement with theoretical predictions.
“We find a large range of Rabi frequencies achievable with low applied voltages (Fig. 3a) to be in excellent agreement with theoretical predictions (Fig. 3b and Supplementary).”
Quote in the paperSubstantial claimMay combine two claims.
Findingown data§ Electronically Programmable Photonic Molecule · p. 4The optical coherence time is ∼1.6 ns for both Rabi and Ramsey oscillations, in agreement with the cavity decay time.
“The optical coherence time is ∼ 1 . 6 ns for both Rabi and Ramsey oscillations in agreement with the cavity decay time.”
Quote in the paperSubstantial claimMay combine two claims.
Findingown data§ Electronically Programmable Photonic Molecule · p. 4A dark mode lifetime of 2 ns is extracted, which is about two times the lifetime of the critically coupled bright mode.
“Tracking the intensity of the retrieved optical pulses stored in the dark mode, we extract a dark mode lifetime of 2 ns, which is about two times of the lifetime of the critically coupled bright mode as expected (Fig. 4d).”
- Also stated in: § Electronically Programmable Photonic Molecule · p. 5 · plain
“Inset: the extracted intensity of the retrieved light shows nearly twice the lifetime of the critically coupled bright mode.”
Quote in the paperSubstantial claim- Also stated in: § Electronically Programmable Photonic Molecule · p. 5 · plain
May combine two claims.
Findingnone given§ Electronically Programmable Photonic Molecule · p. 3The optical lifetime of the two-level system is ∼1.6 ns, much shorter than the coherence time of the laser (∼μs).
“As the optical lifetime of the two-level system ( ∼ 1.6 ns) is much shorter than the coherence time of the laser ( ∼ µ s)”
Quote in the paperSubstantial claimMay combine two claims.
Findingreasoning§ Electronically Programmable Photonic Molecule · p. 4Once the microwave signal is turned off, the photons are trapped in the dark mode and become decoupled from the waveguide, leaving cavity intrinsic dissipation as the only photon loss mechanism.
“Once the microwave signal is turned off, the photons are trapped in the dark mode and become decoupled from the waveguide leaving cavity intrinsic dissipation as the only photon loss mechanism.”
Quote in the paperSubstantial claimMay combine two claims.
Findingreasoning§ Electronically Programmable Photonic Molecule · p. 3The phase coherence time of the two energy levels obtained in the Ramsey measurement is dominated by cavity dissipation, in good agreement with that obtained from the Rabi oscillation.
“As the optical lifetime of the two-level system ( ∼ 1.6 ns) is much shorter than the coherence time of the laser ( ∼ µ s), the phase coherence time of the two energy levels obtained in this measurement is dominated by cavity dissipation in good agreement with that obtained from the Rabi oscillation.”
Quote in the paperNot a substantial claimMay combine two claims.
Findingnone given§ E. Optical dark modes · p. 12For a lithium niobate ring resonator fabricated close to its material loss limit (Q ~ 10^9), with δω = 20 GHz, μ = 1 GHz, θ = 0.05, and γex1 = 2 GHz, a tunable delay of more than 800 ns with a minimum of 500 ps steps and over 95% efficiency could be achieved.
“As an example, assuming a lithium niboate ring resonator can be fabricated close to its material loss limit ( Q ∼ 10 9 ), set δω = 20 GHz, µ = 1 GHz so θ = 0 . 05, and let γ ex1 = 2 GHz, one could achieve a tunable delay of more than 800 ns with a minimum of 500 ps steps (limited by output coupling bandwidth) and over 95% efficiency.”
Quote in the paperSubstantial claim- The authors state this as an assumption: A lithium niobate ring resonator can be fabricated close to its material loss limit (Q ~ 10^9).
May combine two claims.
Premisecitation§ Electronically Programmable Photonic Molecule · p. 1Electro-optic methods are ideally suited for controlling photonic two-level systems since they have fast response, can be programmed and allow for large scale integration.
“Electro-optic methods [15-21] are ideally suited for controlling photonic two-level systems since they have fast response, can be programmed and allow for large scale integration.”
Quote in the paperSubstantial claim0 of 7 sources checked- cites [15] Guo, X., Zou, C.-L., Jung, H. & Tang, H. X. On-chip strong coupling and efficient frequency conversion between telecom and visible optical modes. Phys. Rev. Lett. 117, 123902 (2016). source
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- cites [16] Sato, Y. et al. Strong coupling between distant photonic nanocavities and its dynamic control. Nat. Photon. 6, 56–61 (2012). source
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- cites [17] Clemmen, S., Farsi, A., Ramelow, S. & Gaeta, A. L. Ramsey interference with single photons. Phys. Rev. Lett. 117, 223601 (2016). source
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- cites [18] Xu, Q., Schmidt, B., Pradhan, S. & Lipson, M. Micrometre-scale silicon electro-optic modulator. Nature 435, 325–327 (2005). source
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- cites [19] Ayata, M. et al. High-speed plasmonic modulator in a single metal layer. Science 358, 630–632 (2017). source
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- cites [20] Shambat, G. et al. Ultra-low power fiber-coupled gallium arsenide photonic crystal cavity electro-optic modulator. Opt. Express 19, 7530–7536 (2011). source
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- cites [21] Enami, Y. et al. Hybrid polymer/sol-gel waveguide modulators with exceptionally large electro-optic coefficients. Nat. Photon. 1, 180–185 (2007). source
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May combine two claims.
Premisenone given§ Electronically Programmable Photonic Molecule · p. 4A static resonator can be used to slow down the propagation of a photon, but such slow-down is fundamentally limited by the frequency bandwidth of the resonator (delay-bandwidth product) and cannot be controlled on-demand.
“While a static resonator can be used to slow down the propagation of a photon, such slow-down is fundamentally limited by the frequency bandwidth of the resonator, i.e. the delay-bandwidth product, and cannot be controlled on-demand.”
Quote in the paperSubstantial claimMay combine two claims.
Premisecitation§ Electronically Programmable Photonic Molecule · p. 1Fast phase modulators can generate new optical frequencies but do not support distinct and long-lived optical modes.
“For example, fast phase modulators [9, 23] can generate new optical frequencies but they do not support distinct and long-lived optical modes.”
Quote in the paperSubstantial claim0 of 2 sources checked- cites [9] Lin, Q., Xiao, M., Yuan, L. & Fan, S. Photonic Weyl point in a two-dimensional resonator lattice with a synthetic frequency dimension. Nat. Commun. 7, 13731 (2016). source
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- cites [23] Wade, M. T., Zeng, X. & Popović, M. A. Wavelength conversion in modulated coupled-resonator systems and their design via an equivalent linear filter representation. Opt. Lett. 40, 107–110 (2015). source
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May combine two claims.
Premisecitation§ Electronically Programmable Photonic Molecule · p. 4The use of a dynamically-modulated resonator system can overcome the delay-bandwidth product constraint, enabling new functionalities such as optical buffering.
“In contrast, the use of a dynamically-modulated resonator system can overcome the delay-bandwidth product constraint, enabling new functionalities such as optical buffering [36].”
Quote in the paperSubstantial claim0 of 1 sources checked- cites [36] Casanova, J., Romero, G., Lizuain, I., García-Ripoll, J. J. & Solano, E. Deep strong coupling regime of the Jaynes–Cummings model. Phys. Rev. Lett. 105, 263603 (2010). source
Not checked in the free run.
Probably not a substantial claim: may not pass S2 (checkable), S3 (load-bearing).
Interpretationreasoning§ Electronically Programmable Photonic Molecule · p. 6Dynamically controlled two- and multi-level photonic systems have the potential to enable novel photonic technologies including topological photonics, advanced photonic computation concepts and on-chip optical quantum systems.
“Considering the high versatility and scalability of dynamically controlled two- and multi-level photonic systems, they have the potential to enable novel photonic technologies including topological photonics [3], advanced photonic computation concepts [21, 37] and on-chip optical quantum systems [9, 10].”
Quote in the paperNot a substantial claim0 of 5 sources checked- cites [3] Lu, L., Joannopoulos, J. D. & Soljačić, M. Topological photonics. Nat. Photon. 8, 821–829 (2014). source
Not checked in the free run.
- cites [21] Enami, Y. et al. Hybrid polymer/sol-gel waveguide modulators with exceptionally large electro-optic coefficients. Nat. Photon. 1, 180–185 (2007). source
Not checked in the free run.
- cites [37] Yanik, M. F. & Fan, S. Stopping light all optically. Phys. Rev. Lett. 92, 083901 (2004). source
Not checked in the free run.
- cites [9] Lin, Q., Xiao, M., Yuan, L. & Fan, S. Photonic Weyl point in a two-dimensional resonator lattice with a synthetic frequency dimension. Nat. Commun. 7, 13731 (2016). source
Not checked in the free run.
- cites [10] Chan, J. et al. Laser cooling of a nanomechanical oscillator into its quantum ground state. Nature 478, 89–92 (2011). source
Not checked in the free run.
Probably not a substantial claim: may not pass S2 (checkable), S3 (load-bearing).
Interpretationreasoning§ Electronically Programmable Photonic Molecule · p. 5With microwave control and possible integration of on-chip photonic components including filters, routers and modulators, a new generation of photonic-electronic systems with advanced functionalities can be put in practice.
“With microwave control and the possible integration of onchip photonic components including filters, routers and modulators, a new generation of photonic-electronic systems with advanced functionalities can be put in practice.”
Quote in the paperNot a substantial claimProbably not a substantial claim: may not pass S2 (checkable).
Interpretationreasoning§ Electronically Programmable Photonic Molecule · p. 5These results represent the initial step towards integrated electro-optic coherent manipulation of photonic states and energies.
“These results represent the initial step towards integrated electro-optic coherent manipulation of photonic states and energies, and could have immediate applications in signal processing and quantum photonics.”
Quote in the paperNot a substantial claimMay combine two claims.
Interpretationreasoning§ C. Autler-Townes Splitting and AC Stark Shifts · p. 10When the microwave frequency detuning to the two-mode resonances is much larger than the driving strength (δ ≫ Ω), the microwave modulation behaves as a weak perturbation and induces a shift of the optical energy levels.
“When the microwave frequency detuning to the two-mode resonances is much larger than the driving strength (i.e. δ ≫ Ω), the microwave modulation behaves as a weak perturbation. This perturbation induces a shift of the optical energy levels.”
Quote in the paperNot a substantial claim- The authors state this as an assumption: The nanophotonic two-level system under a coherent microwave drive can be described by the given Hamiltonian.
May combine two claims.
Premisecitation§ Electronically Programmable Photonic Molecule · p. 1Electrically active photonic platforms based on silicon, III-V materials, plasmonics, graphene, and polymers allow for fast electro-optic modulation at gigahertz frequencies, but suffer from dramatically reduced photon lifetimes compared to passive platforms.
“Electrically active photonic platforms based on silicon [16], III-V materials [12, 20], plasmonics [17], graphene [19], and polymers [28] allow for fast electro-optic modulation at gigahertz frequencies, but suffer from dramatically reduced photon lifetimes compared to passive platforms.”
Quote in the paperSubstantial claim0 of 4 sources checked- cites [16] Sato, Y. et al. Strong coupling between distant photonic nanocavities and its dynamic control. Nat. Photon. 6, 56–61 (2012). source
Not checked in the free run.
- cites [12] Chen, W., Özdemir, Ş. K., Zhao, G., Wiersig, J. & Yang, L. Exceptional points enhance sensing in an optical microcavity. Nature 548, 192–196 (2017). source
Not checked in the free run.
- cites [20] Shambat, G. et al. Ultra-low power fiber-coupled gallium arsenide photonic crystal cavity electro-optic modulator. Opt. Express 19, 7530–7536 (2011). source
Not checked in the free run.
- cites [17] Clemmen, S., Farsi, A., Ramelow, S. & Gaeta, A. L. Ramsey interference with single photons. Phys. Rev. Lett. 117, 223601 (2016). source
Not checked in the free run.
May combine two claims.
Interpretationreasoning§ Electronically Programmable Photonic Molecule · p. 5The longer dark mode lifetime is expected because the bright mode lifetime is affected by waveguide coupling, while the dark mode lifetime is determined by intrinsic losses only, as it is decoupled from the input waveguide.
“This is expected since the lifetime of the bright mode is affected by the waveguide coupling, while the lifetime of the dark mode is determined by the intrinsic losses of the resonator only, as it is decoupled from the input waveguide.”
Quote in the paperSubstantial claimMay combine two claims.
Interpretationown data§ Electronically Programmable Photonic Molecule · p. 3The observed Rabi oscillation corresponds to a rotation along the real axis of the energy Bloch sphere and indicates that light tunnels back and forth between the two optical modes at two different optical frequencies.
“The observed Rabi oscillation corresponds to a rotation along the real axis of the energy Bloch sphere (Fig. 3c, inset) and indicates that light tunnels back and forth between the two optical modes at two different optical frequencies.”
Quote in the paperSubstantial claimMay combine two claims.
Interpretationreasoning§ E. Optical dark modes · p. 12In the case of a bright-dark optical mode pair (high bias voltage, μ ≪ δω), c1 is composed by a large part of a1 with a small part of a2, and c2 has a large part of a2 with only a small part of a1.
“whereas in the case of a birght-dark optical mode pair, i.e. the bias voltage is high µ ≪ δω , a 1 , a 2 have a large frequency difference and in c 1 , c 2 basis, c 1 is composed by a large part of a 1 with small part of a 2 and c 2 has large part of a 2 while has only small part of a 1 .”
Quote in the paperNot a substantial claim- The authors state this as an assumption: The nanophotonic two-level system under a coherent microwave drive can be described by the given Hamiltonian.
May combine two claims.
Interpretationreasoning§ E. Optical dark modes · p. 12For c1, c2, the microwave modulation has a component that induces an exchange interaction and a component that induces a frequency modulation.
“This Hamiltonian indicate that for c 1 , c 2 , the microwave modulation has a component that induces an exchange interaction c 1 c † 2 + c † 1 c 2 and a component that induces a frequency modulation c † 2 c 2 -c † 1 c 1 .”
Quote in the paperNot a substantial claim- The authors state this as an assumption: The nanophotonic two-level system under a coherent microwave drive can be described by the given Hamiltonian.
May combine two claims.
Interpretationreasoning§ E. Optical dark modes · p. 12At large bias voltages, the access of mode c2 to the external waveguide is effectively controlled by the microwave drive Ω, and the lifetime for mode c2 becomes closer to that of the intrinsic cavity lifetime.
“From these equations of motion, we see that at large bias voltages, γ ex 2 → 0 and the access of mode c 2 to the external waveguide is effectively controlled by the microwave drive Ω. At the same time, the life time for mode c 2 becomes closer to that of the intrinsic cavity life time.”
Quote in the paperSubstantial claim- The authors state this as an assumption: The nanophotonic two-level system under a coherent microwave drive can be described by the given Hamiltonian.
May combine two claims.
Interpretationreasoning§ E. Optical dark modes · p. 12The conversion term is finite and suppressed by a factor sin θ = μ/δω, and the frequency modulation term is large but can be neglected under the high-Q approximation; the resulting Hamiltonian still has a similar form to the bright mode pairs, with a pre-factor sin θ in conversion efficiency.
“Here the conversion term is finite and is suppressed by a factor sin θ = µ δω and the term Ω cos( ω m t ) cos θ ( c † 2 c 2 -c † 1 c 1 ) is large, meaning that c 1 , c 2 are being frequency modulated. However, Since the modulation frequency is orders of magnitudes larger than the bandwidth of the optical modes, we can neglect this term under highQ approximation. The resulting Hamiltonian still has”
Quote in the paperSubstantial claim- The authors state this as an assumption: The nanophotonic two-level system under a coherent microwave drive can be described by the given Hamiltonian.
- The authors state this as an assumption: The high-Q approximation allows neglecting the frequency modulation term.
The paper relies on this without support.
To realize a fully unitary photonic two-level system with coherent electro-optic control, the photon lifetime of each energy state needs to be much longer than the time required to drive the system from one state to the other.
“To realize a fully unitary photonic twolevel system with coherent electro-optic control, the photon lifetime of each energy state needs to be much longer than the time required to drive the system from one state to the other.”
The paper relies on this without support.
To enable controllable write and read of photons into a resonator and from an external waveguide, the optical coupling strength needs to be altered faster than the cavity photon lifetime.
“To enable controllable write and read of photons into a resonator and from an external waveguide, the optical coupling strength needs to be altered faster than the cavity photon lifetime.”
The authors state this as an assumption.
The nanophotonic two-level system under a coherent microwave drive can be described by the given Hamiltonian.
“The nanophotonic two-level system under a coherent microwave drive can be described by a Hamiltonian with the form”
The authors state this as an assumption.
The high-Q approximation allows neglecting the frequency modulation term.
“we can neglect this term under highQ approximation.”
The authors state this as an assumption.
A lithium niobate ring resonator can be fabricated close to its material loss limit (Q ~ 10^9).
“assuming a lithium niboate ring resonator can be fabricated close to its material loss limit ( Q ∼ 10 9 )”
Claims other papers make about this one
Each is checked against this paper’s own text: does it say what the citing paper says it does?
In Z-cut microrings, modal phase matching using TM00 fundamental and TM20 second harmonic utilizes the largest nonlinear coefficient d33.
“For example, in Z-cut microrings, the fundamental wave is usually at fundamental quasi-TM (TM 00 ) mode, and the second harmonics can be at higher order quasi-TM (TM 20 ) mode.This conversion thus utilizes the largest nonlinear coefficient 𝑑𝑑 33 .”
From Integrated photonics on thin-film lithium niobate (2021) · cites this paper as [173]
Luo et al. demonstrated telecom-to-visible SHG with 1.5%/mW efficiency and DFG at telecom wavelengths in Z-cut microrings.
“With this approach, Luo et al. demonstrated telecom to visible SHG with a conversion efficiency of 1.5%/mW as well as DFG at telecom wavelengths [173].”
From Integrated photonics on thin-film lithium niobate (2021) · cites this paper as [173]
Intermodal phase matching in a microring resonator between the fundamental TM00 spatial mode at the fundamental frequency and TM20 higher order spatial mode at the second harmonic has been demonstrated.
“Intermodal phase matching in a microring resonator between the fundamental TM 00 spatial mode at the fundamental frequency and TM 20 higher order spatial mode at the second harmonic.”
From Integrated photonics on thin-film lithium niobate (2021) · cites this paper as [173]
Self-check
Percentages, sums and reported differences re-computed from the paper’s own numbers.
Each contradiction between two passages listed here was confirmed by an independent check.
Conflicting intrinsic quality factors
MinorThe Fig. 1 caption reports an intrinsic optical quality factor of 2.3 × 106, while the main text reports 2.5 × 106 for the same two-level system.
“which corresponds to a loaded (intrinsic) optical quality factor of 1 . 9 × 10 6 (2 . 3 × 10 6 ).”
“corresponding to a loaded (intrinsic) quality factors of Q = 1 . 9 × 10 6 ( Q i = 2 . 5 × 10 6 )”
Conflicting pulse descriptions for photon storage
MinorThe main text says a microwave π pulse transfers light into the dark mode, whereas the supplemental measurement method calls the first storage pulse a π/2 pulse.
“We excite the critically-coupled bright mode from the optical waveguide, and then apply a microwave π pulse to switch light from the bright to the dark mode (Fig.4c).”
“For the photon storage measurements, the pump light is synchronously turned off with the first π/ 2 pulse allowing for direct power readout of the retrieved light and prevent pump further leaking into the bright mode.”
Same photodetector model assigned incompatible bandwidths
MinorThe supplemental setup identifies the 1811A photodetector as a 12 GHz device, while the supplemental characterization section identifies that model as a 125 MHz device.
“The output optical signal, also coupled with a lensed fiber, is sent to a 12 GHz photodetector (New focus 1811A).”
“The DC transmission is measured on a 125 MHz photodetector (New Focus 1811A)”
Mode separation described as both μ and 2μ
MinorThe text identifies μ as the optical coupling strength and says the modes are separated by that strength, but elsewhere gives their separation as 2μ.
“The two new eigenmodes, separated in frequency by the optical coupling strength, are the energy states of the photonic molecule.”
“the two optical modes are separated by 2 µ = 2 π × 7 GHz”
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Integrated photonics on thin-film lithium niobate
Zhu, D., Shao, L., Yu, M., Cheng, R., Desiatov, B., Xin, C. J., Hu, Y., Holzgrafe, J., Ghosh, S., Shams-Ansari, A., et al. (2021) · Advances in Optics and Photonics · doi:10.1364/aop.411024 · Cited by 1,516 · see citing works
Self-citationLu, J., Surya, J. B., Liu, X., Bruch, A. W., Gong, Z., Xu, Y., & Tang, H. X. (2019) · Optica · doi:10.1364/optica.6.001455 · Cited by 445 · see citing works
Integrated lithium niobate photonics
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Toward 1% single-photon anharmonicity with periodically poled lithium niobate microring resonators
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Integrated Electro-Optics on Thin-Film Lithium Niobate
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Self-citationCavity electro-optics in thin-film lithium niobate for efficient microwave-to-optical transduction
Holzgrafe, J., Sinclair, N., Zhu, D., Shams-Ansari, A., Colangelo, M., Hu, Y., Zhang, M., Berggren, K. K., & Lončar, M. (2020) · Optica · doi:10.1364/optica.397513 · Cited by 136 · see citing works
Self-citationMcKenna, T. P., Witmer, J. D., Patel, R. N., Jiang, W., Van Laer, R., Arrangoiz-Arriola, P., Wollack, E. A., Herrmann, J. F., & Safavi-Naeini, A. H. (2020) · Optica · doi:10.1364/optica.397235 · Cited by 130 · see citing works
Fundamental electro-optic limitations of thin-film lithium niobate microring modulators
Bahadori, M., Goddard, L. L., & Gong, S. (2020) · Optics Express · doi:10.1364/oe.390179 · Cited by 44 · see citing works
2022 Roadmap on integrated quantum photonics
Moody, G., Sorger, V. J., Blumenthal, D. J., Juodawlkis, P. W., Loh, W., Sorace-Agaskar, C., Jones, A. E., Balram, K. C., Matthews, J. C. F., Laing, A., et al. (2022) · Journal of Physics: Photonics · doi:10.1088/2515-7647/ac1ef4 · Cited by 6 · see citing works
“The latter could be realized using an EO photonic molecule [77, 78], formed by coupling two electrically-driven resonators.”
BackgroundSelf-citationHolzgrafe, J., Sinclair, N., Zhu, D., Shams-Ansari, A., Colangelo, M., Hu, Y., Zhang, M., Berggren, K. K., & Loncar, M. (2020) · Conference on Lasers and Electro-Optics · doi:10.1364/cleo_qels.2020.fth4d.5 · Cited by 6 · see citing works
Self-citation
- Authors
- Zhang, M., Wang, C., Hu, Y., Shams-Ansari, A., Ren, T., Fan, S., & Lončar, M.
- Affiliations
- Harvard University (US)
- Stanford University (US)
- Corresponding author
- Lončar, Marko
- Venue
- Nature Photonics
- Published
- 2018-12-14
- Volume
- 13
- Issue
- 1
- Pages
- 36-40
- ISSN
- 1749-4885 (ISSN-L)
- 1749-4893
- OpenAlex
- W2890295555
- Cited by
- 255
- References
- 40
- Citations by year
- 2026: 25 · 2025: 34 · 2024: 28 · 2023: 45 · 2022: 25 · 2021: 39 · 2020: 36 · 2019: 20 · 2018: 1 · 2013: 1
- FWCI
- 11.09
- Type
- journal article
- Language
- en
- Open access
- green
- arxiv.org
- Licence
- www.springer.com/tdm (tdm)
- Locations
- Nature Photonics (publishedVersion)
- arXiv (Cornell University) (submittedVersion)
- Digital Access to Scholarship at Harvard (DASH) (Harvard University) (submittedVersion, cc-by)
- Figshare (submittedVersion, cc-by)
- arXiv (Cornell University)
- Topics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Photorefractive and Nonlinear Optics
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Quantum optics and atomic interactions
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Mechanical and Optical Resonators
- Keywords
- photonic molecules, coupled ring resonators, two-level system, Autler-Townes splitting, Stark shift, Rabi oscillations, Ramsey interference, electro-optic control, microwave signal processing
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Claims read by deepseek-v4.1-flash under definition version 3 (extract-v3) on 2026-10-07.
Classified by jev-1.13-20260917 (gold-guideline-v0.2) on 2026-10-07.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
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