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Evaluation of cation-exchanged zeolite adsorbents for post-combustion carbon dioxide capture
Open accessAbstract
A series of zeolite adsorbents has been evaluated for potential application in post-combustion CO2 capture using a new high-throughput gas adsorption instrument capable of measuring 28 samples in parallel. Among the zeolites tested, Ca-A exhibits the highest CO2 uptake (3.72 mmol g−1 and 5.63 mmol cm−3) together with an excellent CO2 selectivity over N2 under conditions relevant to capture from the dry flue gas stream of a coal-fired power plant. The large initial isosteric heat of adsorption of −58 kJ mol−1 indicates the presence of strong interactions between CO2 and the Ca-A framework. Neutron and X-ray powder diffraction studies reveal the precise location of the adsorption sites for CO2 in Ca-A and Mg-A. A detailed study of CO2 adsorption kinetics further shows that the performance of Ca-A is not limited by slow CO2 diffusion within the pores. Significantly, Ca-A exhibited a higher volumetric CO2 uptake and CO2/N2 selectivity than Mg2(dobdc) (dobdc4− = 1,4-dioxido-2,5-benzenedicarboxylate; Mg-MOF-74, CPO-27-Mg), one of the best performing adsorbents. The exceptional performance of Ca-A was maintained in CO2 breakthrough simulations.
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Metadata
- Authors
- Bae, T.-H., Hudson, M. R., Mason, J. A., Queen, W. L., Dutton, J. J., Sumida, K., Micklash, K. J., Kaye, S. S., Brown, C. M., & Long, J. R.
- Venue
- Energy Environ. Sci.
- Publisher
- Royal Society of Chemistry (RSC)
- Published
- 2013
- Volume
- 6
- Issue
- 1
- Pages
- 128-138
- ISSN
- 1754-5692 (ISSN-L)
- 1754-5706
- OpenAlex
- W2058236569
- Cited by
- 437
- References
- 67
- FWCI
- 32.34
- Type
- journal article
- Language
- en
- Open access
- green
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