Understanding inks for porous-electrode formation

Hatzell, Kelsey B.; Dixit, Marm B.; Berlinger, Sarah A.; Weber, Adam Z.

doi:10.1039/c7ta07255d

Cited by 97Supercapacitor Materials and FabricationNanomaterials and Printing TechnologiesElectrocatalysts for Energy Conversion

Understanding inks for porous-electrode formation

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Hatzell, Kelsey B., Dixit, Marm B., Berlinger, Sarah A., Weber, Adam Z.·2017·J. Mater. Chem. A

DOI 10.1039/c7ta07255d

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Abstract

Scalable manufacturing of high-aspect-ratio multi-material electrodes are important for advanced energy storage and conversion systems. There is a need to understand how one goes from a colloidal state through processing to a functional porous electrode. Such knowledge enables ink-engineering for electrode performance and durability optimization.

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The substrate and how the catalyst ink evolves into the final CL during the coating and drying process have a critical influence on the CL structure.
“When the catalyst ink is prepared, the substrate and how the catalyst ink will evolve into the final CL during the coating and drying process also have a critical influence on the CL structure.”
From Effect of Catalyst Ink and Formation Process on the Multiscale Structure of Catalyst Layers in PEM Fuel Cells (2022) · cites this paper as [35]
Through a brush, a low shear environment exists.
“through a brush, a low shear environment exists [35].”
From Effect of Catalyst Ink and Formation Process on the Multiscale Structure of Catalyst Layers in PEM Fuel Cells (2022) · cites this paper as [35]
The dispersion medium governs the ink properties, which ultimately govern the physical and mass transport properties of the catalyst layer.
“The dispersion medium governs the ink properties, which ultimately govern the physical and mass transport properties of the catalyst layer.”
From Full Parametric Study of the Influence of Ionomer Content, Catalyst Loading and Catalyst Type on Oxygen and Ion Transport in PEM Fuel Cell Catalyst Layers (2020) · cites this paper as [7]

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Authors: Hatzell, K. B., Dixit, M. B., Berlinger, S. A., & Weber, A. Z.
Affiliations: Vanderbilt University (US)
Lawrence Berkeley National Laboratory (US)
ORCID: Hatzell, Kelsey B.
Dixit, Marm B.
Berlinger, Sarah A.
Weber, Adam Z.
Venue: J. Mater. Chem. A
Publisher: Royal Society of Chemistry (RSC)
Published: 2017
Volume: 5
Issue: 39
Pages: 20527-20533
ISSN: 2050-7488 (ISSN-L)
2050-7496
DOI: 10.1039/c7ta07255d
OpenAlex: W2757017746
Cited by: 97
References: 77
Citations by year: 2026: 5 · 2025: 13 · 2024: 8 · 2023: 7 · 2022: 15 · 2021: 16 · 2020: 15 · 2019: 11 · 2018: 7
FWCI: 3.07
Type: journal article
Language: en
Open access: green
www.osti.gov
Locations: Journal of Materials Chemistry A (publishedVersion)
OSTI OAI (U.S. Department of Energy Office of Scientific and Technical Information) (submittedVersion)
eScholarship (California Digital Library) (submittedVersion)
Funders: Division of Chemical, Bioengineering, Environmental, and Transport Systems (1727863)
Fuel Cell Technologies Office (DE-AC02-05CH11231)
Topics: Physical Sciences › Materials Science › Electronic, Optical and Magnetic Materials › Supercapacitor Materials and Fabrication
Physical Sciences › Engineering › Electrical and Electronic Engineering › Nanomaterials and Printing Technologies
Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
Keywords: porous electrodes, high aspect ratio electrodes, colloidal inks, energy storage, energy conversion, electrode durability

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